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    高盐度卤水对CO2地质封存的影响: 以江汉盆地潜江凹陷为例

    李义连 房琦 柯怡兵 董建兴 杨国栋 马鑫

    李义连, 房琦, 柯怡兵, 董建兴, 杨国栋, 马鑫, 2012. 高盐度卤水对CO2地质封存的影响: 以江汉盆地潜江凹陷为例. 地球科学, 37(2): 283-288. doi: 10.3799/dqkx.2012.030
    引用本文: 李义连, 房琦, 柯怡兵, 董建兴, 杨国栋, 马鑫, 2012. 高盐度卤水对CO2地质封存的影响: 以江汉盆地潜江凹陷为例. 地球科学, 37(2): 283-288. doi: 10.3799/dqkx.2012.030
    LI Yi-lian, FANG Qi, KE Yi-bing, DONG Jian-xing, YANG Guo-dong, MA Xin, 2012. Effect of High Salinity on CO2 Geological Storage: A Case Study of Qianjiang Depression in Jianghan Basin. Earth Science, 37(2): 283-288. doi: 10.3799/dqkx.2012.030
    Citation: LI Yi-lian, FANG Qi, KE Yi-bing, DONG Jian-xing, YANG Guo-dong, MA Xin, 2012. Effect of High Salinity on CO2 Geological Storage: A Case Study of Qianjiang Depression in Jianghan Basin. Earth Science, 37(2): 283-288. doi: 10.3799/dqkx.2012.030

    高盐度卤水对CO2地质封存的影响: 以江汉盆地潜江凹陷为例

    doi: 10.3799/dqkx.2012.030
    基金项目: 

    国家自然科学基金项目 41072180

    详细信息
      作者简介:

      李义连(1965-),男,教授,主要从事二氧化碳地质储存技术以及地下水污染控制与修复的研究.E-mail: yl.li@cug.edu.cn

      通讯作者:

      房琦,E-mail: qifang.cug@foxmail.com

    • 中图分类号: X143;X52

    Effect of High Salinity on CO2 Geological Storage: A Case Study of Qianjiang Depression in Jianghan Basin

    • 摘要: 江汉盆地潜江凹陷卤水资源十分丰富,潜江组泥膏岩、泥岩和砂岩交替沉积,构成CO2地质储存的潜在场所.但是潜江组卤水层矿化度非常高,平均值高达283.25 g/L.以高盐度卤水为对象,探讨了高盐度卤水对CO2封存过程中产生的物理化学影响.结果表明,往高盐度卤水层中单纯地注入CO2会造成CO2溶解量和矿物捕集量的显著降低,不利于CO2的储存安全.高盐度会造成注入井附近发生盐岩大量沉淀,不利于CO2的持续注入,同时造成近井周围压力严重积累,降低了封闭安全系数.采用CO2与卤水联合注采模式,可有效缓解CO2单纯地注入过程中的压力严重积累和盐岩沉淀问题,实现资源和地下空间最大化利用,收获经济和环保的双重效益.

       

    • 图  1  潜江凹陷蚌湖向斜带王83井膏岩层与地层压力、孔隙度、温度随深度分布(据贾颖等(2011)修改)

      Fig.  1.  Distribution with depth of gypsum bed and formation pressure, porosity, temperture of the well Wang 83 of the Banghu synclines of Qianjiang depression, Jianghan basin

      图  2  CO2在卤水与纯水中溶解度比值随盐度变化(据Enick and Klara(1990)修改)

      Fig.  2.  CO2 solubility relative to pure water varies with salinity

      图  3  不同盐度条件下储层中(a)和盖层中(b)CO2矿化捕集量

      Fig.  3.  Total CO2 sequstered in mineral phases in the reservoir (a) and caprock (b) at different salinities

      图  4  不同盐度下固态饱和度(a)与流体压力(b)的变化曲线

      Fig.  4.  Solid saturation (a) and fluid pressure (b) at different salinities as function of the similarity variable

      图  5  不同模式下压力(a)、溶解CO2质量分数(b)随时间变化

      Fig.  5.  Pressure evolution (a) and CO2 dissolved fractions varies (b) with time considering different parameters

      表  1  江汉盆地潜江凹陷潜江组沉积地层及卤水层组划分(据于升松(1994)王庆胜(2011)修改)

      Table  1.   Sedimentary stratigraphy and brine formation division of Qianjiang depression, Jianghan basin

      表  2  潜北地区深层地下卤水化学成分(mg/L)(据于升松,1994)

      Table  2.   Chemical composition of deep saline in Qianbei area

      含量 Na Ca Mg K B Li Cl SO4 HCO3 CO3 Br I Rb
      最大值 134 500 2 830 898 6 830 448 108 198 000 36 700 5 764 1 680 913 25 19.3
      最小值 50 900 123 15 120 5 12 44 800 1 750 99 0 55 3.5 0.9
      平均值 110 473 899.4 173.8 1 457.5 145.5 58.9 160 000 9 665.8 1 018.4 1 482 364.7 11.9 3.68
      水样数 105 95 95 88 82 75 105 105 95 95 95 92 19
       
      含量 Cs Sr Mn Fe Cu Ag Pb Cr Ni Zn Mo Ga NO2 NO3 NH4
      最大值 10.1 63 1.2 1.8 1.2 0.006 0.06 0.012 0.12 1.2 0.02 1 100
      最小值 0.1 14 0.06 1.2 0.006 0.002 0.006 0 0 0.6 0 194
      平均值 1.22 34.3 0.64 1.5 0.23 0.003 6 0.038 0.006 0.036 0.84 0.003 0 0 30 734.5
      水样数 19 4 6 2 6 5 6 5 4 5 6 4 1 1 5
      下载: 导出CSV
    • Alkan, H., Cinar, Y., Ulker, E., 2011. Impact of capillary pressure, salinity and in situ condition on CO2 injection into saline aqfuiers. Transport in Porous Media, 84(3): 799-819. doi: 10.1007/s11242-010-9541-8
      Bacci, G., Korre, A., Durucan, S., 2011a. Experimental investigation into salt precipitation during CO2 injection in saline aquifers. Energy Procedia, 4: 4450-4456. doi: 10.1016/j.egypro.2011.02.399
      Bacci, G., Korre, A., Durucan, S., 2011b. An experimental and numerical investigation into the impact of dissolution/precipitation mechanisms on CO2 injectivity in the wellbore and far field regions. International Journal of Greenhouse Gas Control, 5(3): 579-588, doi: 10.1016/j.ijggc.2011.05.007
      Bachu, S., 2002. Sequestration of CO2 in geological media in response to climate change: road map for site selection using the transform of the geological space into the CO2 phase space. Energy Conversion Management, 43(1): 87-102. doi: 10.1016/S0196-8904(01)00009-7
      Enick, R.M., Klara, S.M., 1990. CO2 solubility in water and brine under reservoir conditions. Chem. Eng. Comm., 90: 23-33. doi: 10.1080/00986449008940574
      Fang, Z.X., 2002. Hydrocarbon exploration signification of intersalt sediments in Qianjiang saline lake basin. Acta Sedimentologica Sinica, 20(4): 608-613 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-CJXB200204011.htm
      Giorgis, T., Carpita, M., Battistelli, A., 2007.2D modelling of salt precipitation during the injection of dry CO2 in a depleted gas reservoir. Energy Conversion and Management, 48(6): 1816-1826. doi:/ 10.1016/j.enconman.2007.01.012
      Holloway, S., 2005. Underground sequestration of carbon dioxide—a viable greenhouse gas migration option. Energy, 30(11-12): 2318-2333. doi: 10.1016/j.energy.2003.10.23
      Jia, Y., Li, P.J., Fu, X., et al., 2011. Characteristics of gypsolyte-salt rock and its influence on formation pressure of Qianjiang Formation in Qianjiang depression. Geological Science and Technology Information, 30(4): 50-54 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTotal-DZKQ201104008.htm
      Kim, K.Y., Han, W.S., Oh, J., et al., 2011. Characteristics of salt-precipitation and the assoicated pressure build-up during CO2 storage in saline aquifers. Transport in Porous Media, 84(2), online first. doi: 10.1007/s11242-011-9909-4
      Lu, M.G., Chen, F.L., Liu, J., 2007. Characteristics of the Jianghan salt lake. China Mining Magazine, 16(4): 102-104 (in Chinese with English abstract). http://www.researchgate.net/publication/313661363_Characteristics_of_the_Jianghan_salt_lake
      Mert, M., Davidson, O., de Coninck H., et al., 2005. IPCC report on carbon dioxide capture and storage. Cambridge University Press, London.
      Pooladi-Darvish, M., Moghdam, S., Xu, D., 2011. Multiwell injectivity for storage of CO2 in aquifers. Energy Procedia, 4: 4252-4259. doi: 10.1016/j.egypro.2011.02.374
      Wang, Y.X., Mao, X.M., DePaolo, D., 2011. Nanoscale fluid-rock interaction in CO2 geological storage. Earth Science—Journal of China University of Geosciences, 36(1): 163-171 (in Chinese with English abstract). doi: 10.3799/dqkx.2011.017
      Wang, Q.S., 2011. The reservoir evaluation and development technology of nonsandstone reservoirs between salt beds in Qianjiang depression (Dissertation). China University of Geosciences, Beijing (in Chinese with English abstract).
      Yu, S.S., 1994. The hydrochemical characteristics of the deep brines in Jianghan basin, Hubei. Journal of Salt Lake Science, 2(1): 6-17 (in Chinese with English abstract). http://www.researchgate.net/publication/285511142_The_hydrochemical_characteristics_of_the_deep_brines_in_Jianghan_basin_Hubei
      Yuan, D.X., 1997. Modern karstology and global change study. Earth Science Frontiers, 4(1-2): 17-25 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-DXQY7Z1.003.htm
      Zhang, W., Li, Y.L., Omambia, A.N., 2010. Reactive transport modeling of effects of convective mixing on long-term CO2 geological storage in deep saline formations. International Journal of Greenhouse Gas Control, 5(2): 241-256. doi: 10.1016/j.ijggc.2010.10.007
      方志雄, 2002. 潜江盐湖盆地盐间沉积的石油地质特征. 沉积学报, 20(4): 608-613. doi: 10.3969/j.issn.1000-0550.2002.04.012
      贾颖, 李培军, 付鑫, 等, 2011. 潜江凹陷潜江组膏层特征及其对地层压力的影响. 地质科技情报, 30(4): 50-54. https://www.cnki.com.cn/Article/CJFDTOTAL-DZKQ201104008.htm
      卢明国, 陈凤玲, 刘俊, 2007. 江汉盐湖盆地沉积特征. 中国矿业, 16(4): 102-104. doi: 10.3969/j.issn.1004-4051.2007.04.032
      王庆胜, 2011. 潜江凹陷盐间非砂岩油藏评价与开发技术研究(学位论文). 北京: 中国地质大学.
      王焰新, 毛绪美, DePaolo, D., 2011. CO2地质储存的纳米尺度流体-岩石相互作用研究. 地球科学——中国地质大学学报, 36(1): 163-171. https://www.cnki.com.cn/Article/CJFDTOTAL-DQKX201101018.htm
      于升松, 1994. 湖北江汉盆地潜江凹陷深层地下卤水水文地球化学研究. 盐湖研究, 2(1): 6-17. https://www.cnki.com.cn/Article/CJFDTOTAL-YHYJ401.001.htm
      袁道先, 1997. 现代岩溶学和全球变化研究. 地学前缘, 4(1-2): 17-25. https://www.cnki.com.cn/Article/CJFDTOTAL-DXQY7Z1.003.htm
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    出版历程
    • 收稿日期:  2012-01-09
    • 刊出日期:  2012-03-15

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