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    华南晚奥陶世次火山岩的发现:早古生代与俯冲有关的英安岩?

    易立文 马昌前 王连训 赖中信 李湘玉 杨亚楠 吴飞 胡晏如

    易立文, 马昌前, 王连训, 赖中信, 李湘玉, 杨亚楠, 吴飞, 胡晏如, 2014. 华南晚奥陶世次火山岩的发现:早古生代与俯冲有关的英安岩?. 地球科学, 39(6): 637-653. doi: 10.3799/dqkx.2014.061
    引用本文: 易立文, 马昌前, 王连训, 赖中信, 李湘玉, 杨亚楠, 吴飞, 胡晏如, 2014. 华南晚奥陶世次火山岩的发现:早古生代与俯冲有关的英安岩?. 地球科学, 39(6): 637-653. doi: 10.3799/dqkx.2014.061
    Yi Liwen, Ma Changqian, Wang Lianxun, Lai Zhongxin, Li Xiangyu, Yang Ya'nan, Wu Fei, Hu Yanru, 2014. Discovery of Late Ordovician Subvolcanic Rocks in South China: Existence of Subduction-Related Dacite from Early Paleozoic?. Earth Science, 39(6): 637-653. doi: 10.3799/dqkx.2014.061
    Citation: Yi Liwen, Ma Changqian, Wang Lianxun, Lai Zhongxin, Li Xiangyu, Yang Ya'nan, Wu Fei, Hu Yanru, 2014. Discovery of Late Ordovician Subvolcanic Rocks in South China: Existence of Subduction-Related Dacite from Early Paleozoic?. Earth Science, 39(6): 637-653. doi: 10.3799/dqkx.2014.061

    华南晚奥陶世次火山岩的发现:早古生代与俯冲有关的英安岩?

    doi: 10.3799/dqkx.2014.061
    基金项目: 广东核工业地质局南岭贵东花岗岩体构造变形与铀矿成矿关系研究
    详细信息
      作者简介:

      易立文(1988-),博士研究生,研究方向为成因矿物学与矿床地球化学.E-mail: yiliwen1988@163.com

      通讯作者:

      马昌前,E-mail: cqma@cug.edu.cn

    • 中图分类号: P588.14

    Discovery of Late Ordovician Subvolcanic Rocks in South China: Existence of Subduction-Related Dacite from Early Paleozoic?

    • 摘要: 华南早古生代花岗岩广泛分布,但同时代的(次)火山岩却很罕见.本次研究采用LA-ICPMS锆石U-Pb定年方法,结合微区原位Hf同位素分析,对南岭广东韶关地区的河口、上洞英安岩进行了系统研究.结果表明英安岩形成于448.7±1.7 Ma,为晚奥陶世岩浆活动产物.岩石为斑状结构,常见石英碎斑或港湾状石英斑晶,基质为隐晶质,具有典型浅成岩石特征.地球化学资料表明,这些岩石属于高钾钙碱性英安岩.英安岩微量元素显示了轻稀土富集、高场强元素(Ta、Nb)亏损和极低的Cr、Ni含量等明显火山弧岩浆特征.同位素数据显示河口、上洞英安岩全岩ISr=0.709 0~0.714 0,εNd(t)=-8.9~-9.3,锆石εHf(t)变化范围为-8.06~-3.80,与华南加里东期主要花岗岩类同位素特征一致,具有壳源属性.二阶段Hf模式年龄范围为1.67~1.93 Ga,与Nd模式年龄结果1.91~1.94 Ga相近;表明河口、上洞英安岩来源于古元古代结晶基底地壳物质.河口、上洞奥陶纪英安岩的发现,进一步证明该区早古生代存在俯冲岩浆活动,为研究华南早古生代地质事件提供了新的证据.

       

    • 图  1  华南构造简图(a)和河口、上洞英安岩地质简图(b)

      a.据任纪舜等, 1980, 略修改;b.据1∶5万区域地质图

      Fig.  1.  Tectonic map of South China (a) and geological sketch map of Hekou and Shangdong dacite (b)

      图  2  华南晚奥陶世次火山岩显微特征

      港湾状石英(Qz)斑晶,正交偏光;b.石英斑晶破碎产生裂隙,正交偏光;c.斜长石(Pl)斑晶具环带构造及聚片双晶,正交偏光;d.绿泥石化(Chl)的黑云母呈挠曲片状,单偏光;e.基质具明显流动构造,单偏光;f.碳酸盐矿物(Cbn)和绿泥石呈角闪石假象,单偏光

      Fig.  2.  Microphotograph characters of Late Ordovician sub-volcanic rocks in South Chinaa

      图  3  华南晚奥陶世次火山岩锆石阴极发光图像

      Fig.  3.  CL images of zircons from Late Ordovician sub-volcanic rocks in South China

      图  4  华南晚奥陶世次火山岩锆石U-Pb谐和年龄

      Fig.  4.  Zircon U-Pb concordia diagram of zircons from Late Ordovician sub-volcanic rocks in South China

      图  5  华南晚奥陶世次火山岩锆石稀土元素球粒陨石标准化分布型式

      岩浆成因锆石据文献Rubatto, 2002;标准化所用原始地幔和球粒陨石数据据文献Sun and McDonough, 1989

      Fig.  5.  Chondrite-normalized REE patterns of zircons from Late Ordovician subvolcanic rocks in South China

      图  6  华南典型早古生代岩浆岩的TAS判别图(a)、K2O-SiO2判别图(b)和A/NK-A/CNK判别图(c)

      a.据文献Middlemost, 1994;虚线上方为碱性系列,下方为亚碱性系列;b.据文献Collins et al., 1982;c.据文献Maniar and Piccole, 1989; ANK=Al2O3/(Na2O+K2O);ACNK=Al2O3/(CaO+Na2O+K2O)

      Fig.  6.  TAS (a), K2O-SiO2 (b) and A/NK-A/CNK (c) diagram of typical Early Paleozoic dacites in South China

      图  7  华南晚奥陶世次火山岩与典型俯冲成因中酸性火山岩原始地幔标准化的微量元素分布型式(a)和稀土元素球粒陨石标准化分布型式(b)

      原始地幔和球粒陨石标准化据Sun and McDonough, 1989

      Fig.  7.  (a) Trace elements and (b) REE patterns spidergrams of Late Ordovician subvolcanic rocks in South China and typical subduction medium acidic volcanics

      图  8  华南典型加里东期岩浆岩εNd(t)-ISr关系(a)及εNd(t)-t关系(b)

      b.华南元古代地壳据沈渭洲等,1993

      Fig.  8.  Relations of εNd(t)-ISr and εNd(t)-t of typical Caledonian magmatic rocks in South China

      图  9  华南晚奥陶世次火山岩εHf(t)频数分布(a)、Lu-Hf同位素组成(b)及Hf地壳模式年龄概率分布(c)

      Fig.  9.  Initial hafnium isotope ratios, zircon Lu-Hf isotope relationship and Hf model age for Late Ordovician subvolcanic rocks in South China

      图  10  华南早古生代岩浆岩年龄分布位置及成岩年龄直方图

      图中Ⅰ、Ⅱ、Ⅲ为年龄阶梯分带代号,靠近华夏地块的弓形区域为一级阶梯,其岩浆活动集中在450 Ma;诸广山一带为二级阶梯,岩浆活动集中在430 Ma;最靠近扬子地块的雪峰山区域为三级阶梯,岩浆活动主要集中在410 Ma;数据来源据文献(李献华,1990周汉文等,1994王江海等,1999楼法生等,2005于津海等,2005柏道远等,2006彭松柏等,2006许德如等,2006; Wang et al., 2007刘锐等,2008曾雯等,2008程顺波等, 2009a, 2009b徐先兵等,2009张芳荣等, 2009, 2010李光来等,2010; Li et al., 2010, 2011; Liu et al., 2010a; Wan et al., 2010王彦斌等,2010; Yang et al., 2010张爱梅等,2010张菲菲等,2010张文兰等,2011)

      Fig.  10.  Age distribution and diagenetic ages of the Early Paleozoic granites in South China

      图  11  华南晚奥陶世次火山岩构造判别图(Harris et al., 1986)

      Fig.  11.  Recongnition diagram for Late Ordovician subvolcanic rocks in South China

      表  1  华南晚奥陶世次火山岩锆石LA-ICPMS U-Pb分析结果

      Table  1.   LA-ICPMS zircon U-Pb data for late ordovician sub-volcanic rocks in South China

      样品点号 Th(10-6) U(10-6) Th/U Pbt(10-6) 校正比率 校正年龄(Ma)
      207Pb/206Pb ±1σ 207Pb/235U ±1σ 206Pb/238U ±1σ 207Pb/206Pb ±1σ 207Pb/235U ±1σ 206Pb/238U ±1σ
      1 313 922 0.339 77.70 0.056 2 0.001 0 0.563 1 0.010 1 0.072 5 0.000 4 461 39 454 7 451 3
      2 275 513 0.536 45.20 0.056 1 0.001 2 0.559 8 0.011 5 0.072 5 0.000 6 454 44 451 7 451 3
      3 134 260 0.515 138.00 0.163 8 0.002 3 9.111 1 0.131 1 0.403 1 0.002 8 2 495 23 2 349 13 2 183 13
      4 179 356 0.699 31.11 0.059 0 0.001 4 0.587 6 0.014 1 0.072 1 0.000 5 569 52 469 9 449 3
      5 197 513 0.384 43.28 0.057 8 0.001 3 0.571 8 0.012 8 0.071 9 0.000 5 524 50 459 8 448 3
      6 150 289 0.519 25.25 0.057 2 0.001 6 0.569 8 0.015 3 0.072 5 0.000 7 498 66 458 10 451 4
      7 100 155 0.645 14.66 0.059 2 0.002 0 0.615 7 0.020 4 0.075 6 0.000 7 576 77 487 13 470 4
      8 151 322 0.469 27.75 0.052 6 0.001 2 0.525 8 0.011 3 0.072 5 0.000 6 322 50 429 8 451 4
      9 167 240 0.696 22.44 0.062 4 0.001 9 0.621 0 0.018 7 0.072 3 0.000 7 687 66 490 12 450 4
      10 196 331 0.592 29.76 0.054 1 0.001 3 0.541 3 0.012 9 0.072 3 0.000 6 372 56 439 8 450 3
      11 160 253 0.632 23.03 0.057 2 0.001 5 0.571 5 0.015 0 0.072 4 0.000 7 498 64 459 10 451 4
      12 178 364 0.489 34.88 0.054 6 0.001 3 0.587 3 0.013 7 0.077 9 0.000 6 394 58 469 9 483 3
      13 169 439 0.385 35.54 0.055 3 0.001 2 0.519 4 0.010 3 0.068 0 0.000 5 433 48 425 7 424 3
      14 314 336 0.935 32.30 0.054 1 0.001 4 0.528 2 0.013 1 0.070 7 0.000 5 376 59 431 9 440 3
      15 253 598 0.423 51.80 0.055 4 0.001 2 0.551 8 0.011 3 0.072 0 0.000 5 428 44 446 7 448 3
      16 158 282 0.560 25.24 0.052 3 0.001 5 0.519 1 0.014 5 0.072 0 0.000 6 298 65 425 10 448 3
      17 228 391 0.583 35.13 0.057 6 0.001 4 0.570 5 0.013 4 0.071 7 0.000 5 517 54 458 9 447 3
      18 203 366 0.555 32.97 0.054 6 0.001 5 0.541 8 0.014 1 0.072 0 0.000 6 394 63 440 9 448 4
      19 213 392 0.798 35.51 0.058 0 0.001 4 0.579 6 0.013 7 0.072 3 0.000 5 532 54 464 9 450 3
      20 135 360 0.375 32.14 0.053 6 0.001 3 0.562 0 0.013 3 0.075 9 0.000 6 354 54 453 9 472 4
      下载: 导出CSV

      表  2  华南晚奥陶世次火山岩单颗粒锆石微量元素分析结果(10-6)

      Table  2.   Contents of REE for zircons from Late Ordovician subvolcanic rocks in South China

      点号 1 2 3 4 5 6 7 8 9 10
      P 399.66 359.70 156.20 209.56 420.65 442.23 282.62 190.13 252.89 226.60
      Ti 2.05 3.56 6.38 3.18 5.33 4.43 9.27 2.96 7.98 16.91
      Nb 3.70 1.67 1.24 1.47 3.44 2.75 1.82 1.71 1.59 1.03
      La 0.44 0.04 0.02 0.02 0.00 0.01 0.10 0.00 0.01 0.15
      Ce 6.03 8.38 18.47 9.51 6.73 11.47 12.06 9.29 11.63 10.93
      Pr 0.26 0.12 0.02 0.03 0.05 0.08 0.07 0.02 0.07 0.10
      Nd 1.69 2.73 0.65 0.56 0.96 1.23 1.07 0.52 1.24 1.66
      Sm 2.66 7.40 1.28 1.63 3.35 3.28 2.55 1.21 3.42 3.03
      Eu 0.16 0.69 0.32 0.30 0.28 0.61 0.59 0.28 0.45 0.66
      Gd 19.66 49.40 6.92 10.00 24.46 22.37 16.03 10.38 19.12 20.80
      Tb 8.16 17.05 2.13 3.95 9.09 8.75 6.08 3.89 6.85 7.80
      Dy 113.00 209.12 27.26 52.28 122.86 117.40 75.35 51.62 83.79 97.58
      Ho 46.36 79.78 11.36 22.37 50.27 47.64 30.92 22.91 32.35 40.30
      Er 217.86 342.52 55.98 112.67 233.02 227.99 141.36 116.58 143.62 188.20
      Tm 45.92 67.76 13.38 25.56 48.24 49.08 30.29 27.43 29.12 41.59
      Yb 421.00 595.33 139.33 259.79 452.69 469.20 283.76 282.59 263.20 401.06
      Lu 80.09 109.60 29.16 54.54 88.33 92.70 56.08 61.14 51.09 82.59
      Ta 2.74 1.07 0.74 1.03 1.86 1.35 0.83 0.97 0.86 0.75
      Th 312.50 275.17 133.83 179.08 197.15 149.98 99.96 150.80 166.80 196.20
      U 922.34 513.19 260.35 356.49 512.67 289.18 154.55 321.71 240.27 331.08
      点号 11 12 13 14 15 16 17 18 19 20
      P 233.76 229.95 251.03 398.30 404.03 214.79 594.15 231.81 257.95 378.17
      Ti 3.85 2.31 3.28 11.91 2.63 3.51 8.11 3.47 2 135.64 4.19
      Nb 1.72 2.08 3.08 3.14 3.95 1.94 2.70 1.75 7.85 2.22
      La 0.02 0.01 0.00 0.01 0.12 0.00 0.14 0.00 0.12 0.02
      Ce 11.44 10.35 8.40 15.61 8.94 9.98 5.81 10.31 11.66 4.90
      Pr 0.05 0.02 0.03 0.14 0.07 0.02 0.12 0.03 0.10 0.04
      Nd 0.76 0.73 0.47 2.31 0.99 0.55 2.28 0.67 0.98 0.95
      Sm 2.77 1.70 1.57 5.39 2.89 2.11 5.17 1.53 2.46 2.75
      Eu 0.41 0.31 0.28 1.08 0.32 0.39 0.35 0.38 0.40 0.20
      Gd 17.28 12.70 13.37 32.61 23.97 12.41 31.15 11.94 14.01 19.29
      Tb 6.16 4.80 5.87 11.53 9.14 4.96 11.58 4.59 5.56 7.54
      Dy 76.58 68.00 79.16 142.65 121.65 63.09 144.99 60.43 71.52 97.44
      Ho 29.64 28.34 34.33 55.66 50.30 26.76 55.94 25.74 29.70 39.65
      Er 132.76 141.82 175.99 249.56 237.58 126.79 250.71 129.14 148.18 183.46
      Tm 27.13 32.73 40.11 49.71 50.02 28.18 51.63 29.06 33.08 38.30
      Yb 242.32 325.15 417.03 448.41 462.84 267.71 466.11 291.12 324.45 360.13
      Lu 46.83 67.78 86.58 85.65 91.77 54.59 89.21 62.41 67.17 70.97
      Ta 0.90 1.42 2.10 1.24 2.48 1.06 1.18 1.06 1.60 1.35
      Th 160.09 178.24 169.22 314.17 252.66 158.39 228.41 202.60 212.95 134.87
      U 252.54 363.72 438.53 336.30 597.79 281.54 391.17 365.80 392.12 360.07
      下载: 导出CSV

      表  3  华南晚奥陶世次火山岩主量元素分析结果(%)

      Table  3.   Major element data for Late Ordovician subvolcanic rocks in South China

      样品 SiO2 TiO2 Al2O3 Fe2O3 FeO MnO MgO CaO Na2O K2O P2O5 H2O+ CO2
      09GD47 71.35 0.46 13.55 0.75 3.12 0.07 1.06 1.87 2.82 3.60 0.10 0.97 0.08
      09GD18 70.05 0.47 13.88 0.64 3.37 0.08 1.11 3.16 2.71 2.96 0.11 1.14 0.13
      09GD19 68.34 0.55 14.25 0.63 3.98 0.09 1.45 3.77 2.58 2.91 0.13 0.97 0.15
      09GD20 69.53 0.38 14.10 2.97 1.30 0.08 0.40 2.13 2.53 3.05 0.10 1.58 1.67
      下载: 导出CSV

      表  4  华南晚奥陶世次火山岩微量元素分析结果(10-6)

      Table  4.   Trace element data for Late Ordovician subvolcanic rocks in South China

      样品 Li Be Sc V Cr Co Ni Cu Zn Ga Rb Sr Zr Nb Cs Ba Hf Ta Pb Th U
      09GD47 27.5 2.28 12.2 59.8 11.2 6.86 5.03 7.30 60.0 16.2 180 128 152 11.1 10.50 732 4.60 1.00 50.1 16.3 2.90
      09GD18 32.8 2.12 13.2 63.5 15.1 7.82 6.71 9.58 65.7 17.0 132 150 170 10.7 10.10 702 4.98 0.93 208.0 16.5 3.25
      09GD19 39.9 2.12 15.2 79.9 18.5 9.82 7.29 12.4 64.6 17.3 133 168 160 10.8 11.70 668 4.71 0.90 199.0 15.3 3.07
      09GD20 6.48 2.28 11.3 25.2 5.12 7.57 3.68 5.12 59.7 17.0 144 116 204 10.7 8.110 721 5.98 1.04 42.9 14.7 3.30
      下载: 导出CSV

      表  5  华南晚奥陶世次火山岩稀土元素分析结果(10-6)

      Table  5.   REE data for Late Ordovician subvolcanic rocks in South China

      样品 La Ce Pr Nd Sm Eu Gd Tb Dy Ho Er Tm Yb Lu Y REE LREE/HREE (La/Yb)N δEu δCe
      09GD47 41.6 78.2 8.75 32.8 6.61 1.17 6.04 0.98 5.86 1.16 3.52 0.50 3.26 0.49 34.1 191.0 7.76 12.02 0.60 0.74
      09GD18 48.7 86.5 9.90 37.2 7.22 1.36 6.78 1.08 6.56 1.28 3.75 0.54 3.54 0.50 37.5 214.9 7.94 12.95 0.63 0.71
      09GD19 46.9 85.6 9.81 37.5 7.35 1.32 6.76 1.08 6.35 1.26 3.59 0.51 3.38 0.47 35.7 211.9 8.05 13.09 0.60 0.72
      09GD20 38.4 69.2 8.19 32.4 6.89 1.50 6.91 1.14 7.00 1.41 4.24 0.59 4.13 0.60 41.7 182.6 6.01 8.77 0.71 0.70
      下载: 导出CSV

      表  6  华南晚奥陶世次火山岩全岩Sr-Nd同位素组成

      Table  6.   Whole-rock Sr-Nd compositions for Late Ordovician subvolcanic rocks in South China

      样品号 Rb(10-6) Sr(10-6) 87Rb/86Sr 87Sr/86Sr Isr εSr(t) Sm(10-6) Nd(10-6) 147Sm/147Nd 143Nd/144Nd INd εNd(t) TDM(Ga) T2DM(Ga) Sm/Nd
      09GD47 180 127.7 4.095 2 0.735 227 0.708 97 71.0 6.6 32.84 0.121 6 0.511 960 0.511 602 -8.9 1.96 1.91 0.20
      09GD18 132 149.9 2.546 9 0.729 150 0.712 82 125.7 7.2 37.23 0.117 2 0.511 928 0.511 583 -9.3 1.92 1.94 0.19
      09GD19 133 168.1 2.286 8 0.726 809 0.712 15 116.1 7.4 37.46 0.118 6 0.511 950 0.511 600 -8.9 1.92 1.91 0.20
      09GD20 144 116.1 3.596 4 0.737 243 0.714 19 145.1 6.9 32.42 0.128 5 0.511 973 0.511 594 -9.1 2.10 1.92 0.21
      下载: 导出CSV

      表  7  华南晚奥陶世次火山岩锆石Lu-Hf分析结果

      Table  7.   Zircon Lu-Hf isotopic compositions form Late Ordovician subvolcanic rocks in South China

      样品号 176Hf/177Hf ±2σ 176Lu/177Hf ±2σ 176Yb/177Hf ±2σ Hf(i) εHf(448) ±2σ TDM2(Ma) ±2σ
      1 0.282 327 0.000 014 0.000 947 0.000 004 0.025 335 0.000 143 0.282 319 -6.16 0.5 1 814 64
      2 0.282 299 0.000 028 0.000 954 0.000 010 0.023 209 0.000 261 0.282 291 -7.17 1.0 1 877 125
      3 0.282 336 0.000 014 0.000 774 0.000 007 0.019 551 0.000 088 0.282 329 -5.82 0.5 1 792 63
      4 0.282 273 0.000 012 0.000 919 0.000 009 0.023 983 0.000 220 0.282 266 -8.06 0.4 1 933 55
      5 0.282 285 0.000 018 0.000 728 0.000 009 0.018 501 0.000 200 0.282 279 -7.58 0.6 1 903 82
      6 0.282 301 0.000 016 0.001 275 0.000 010 0.034 589 0.000 307 0.282 290 -7.20 0.6 1 879 69
      7 0.282 396 0.000 021 0.001 224 0.000 010 0.032 350 0.000 248 0.282 386 -3.82 0.7 1 666 92
      8 0.282 378 0.000 007 0.001 001 0.000 002 0.025 514 0.000 047 0.282 370 -4.37 0.3 1 701 33
      9 0.282 329 0.000 014 0.000 740 0.000 004 0.020 343 0.000 061 0.282 323 -6.04 0.5 1 806 61
      10 0.282 432 0.000 016 0.001 096 0.000 008 0.027 277 0.000 220 0.282 423 -2.49 0.6 1 583 70
      11 0.282 356 0.000 014 0.001 088 0.000 004 0.027 168 0.000 120 0.282 347 -5.18 0.5 1 752 63
      12 0.282 343 0.000 016 0.000 905 0.000 002 0.024 177 0.000 091 0.282 335 -5.61 0.6 1 779 74
      下载: 导出CSV
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