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    达里诺尔湖水体稳定氢、氧同位素组成变化对结冰过程的响应

    李文宝 李畅游 刘晓旭 甄志磊 胡其图 刘志娇

    李文宝, 李畅游, 刘晓旭, 甄志磊, 胡其图, 刘志娇, 2015. 达里诺尔湖水体稳定氢、氧同位素组成变化对结冰过程的响应. 地球科学, 40(12): 2081-2090. doi: 10.3799/dqkx.2015.184
    引用本文: 李文宝, 李畅游, 刘晓旭, 甄志磊, 胡其图, 刘志娇, 2015. 达里诺尔湖水体稳定氢、氧同位素组成变化对结冰过程的响应. 地球科学, 40(12): 2081-2090. doi: 10.3799/dqkx.2015.184
    Li Wenbao, Li Changyou, Liu Xiaoxu, Zhen Zhilei, Hu Qitu, Liu Zhijiao, 2015. Changes of Stable Oxygen and Hydrogen Isotopes and Their Responses to Freezing Process in Dali-Nor Lake in Cold-Arid Areas of China. Earth Science, 40(12): 2081-2090. doi: 10.3799/dqkx.2015.184
    Citation: Li Wenbao, Li Changyou, Liu Xiaoxu, Zhen Zhilei, Hu Qitu, Liu Zhijiao, 2015. Changes of Stable Oxygen and Hydrogen Isotopes and Their Responses to Freezing Process in Dali-Nor Lake in Cold-Arid Areas of China. Earth Science, 40(12): 2081-2090. doi: 10.3799/dqkx.2015.184

    达里诺尔湖水体稳定氢、氧同位素组成变化对结冰过程的响应

    doi: 10.3799/dqkx.2015.184
    基金项目: 

    国家自然科学基金重点项目 51339002

    国家自然科学基金项目 51269013

    国家自然科学基金项目 51469025

    中国博士后科学基金资助项目 2014M562495XB

    内蒙古自治区自然基金项目 2012MS0615

    详细信息
      作者简介:

      李文宝(1980-), 男, 副教授, 博士, 主要从事环境地球化学、第四纪地质学等研究工作.E-mail: tianshitd@126.com

      通讯作者:

      李畅游, E-mail: nndlichangyou@163.com

    • 中图分类号: P592

    Changes of Stable Oxygen and Hydrogen Isotopes and Their Responses to Freezing Process in Dali-Nor Lake in Cold-Arid Areas of China

    • 摘要: 利用自然界中广泛分布的环境同位素进行湖泊水体演化过程分析已经成为现代湖泊科学的重要研究方向.通过采集内蒙古达里诺尔湖(简称"达里湖") 2013年1月份的湖冰、湖水, 2012年夏季湖水与湖区大气降水等, 共分析了77个样品中稳定氢(H)、氧(O)同位素值的变化情况, 在此基础上对达里湖水体稳定H、O同位素组成变化及其对结冰过程的响应进行了详细分析, 结果显示: (1)伴随结冰过程的完成, 各站点深层冰体(厚度~65 cm)中δD、δ18O值比表层冰体(厚度~15 cm)中的值出现不同幅度的偏重.而冰下水体中δD、δ18O平均值则比冰体中的平均值分别偏轻约13.85‰、2.23‰.在冰层形成的快速与稳定阶段, δD、δ18O值的变化幅度也存在差异.同时, 冬季外源水体的输入对各站点间同位素值差异的影响比夏季更明显; (2)夏季湖水、冬季湖水与湖冰的同位素值均落在全球大气降水线与湖区大气降水线之外, 显示湖泊冰封之前, 蒸发对湖泊水体同位素偏移存在一定程度的影响; 而冬季湖水与湖冰的同位素值基本位于同一斜率区间, 且全部落在夏季湖水同位素值的右侧, 显示两者之间并不存在明显的蒸发分馏作用, 造成上述现象的因素只能归结于结冰过程.

       

    • 图  1  内蒙古地区气候特征及达里湖取样点分布

      a.内蒙古地区现代年均降水分布,左上小图中单位为mm/a;b.达里湖流域及取样点分布

      Fig.  1.  Characteristic of local climate in Inner Mongolia and sample sites in Dali-Nor Lake

      图  2  不同厚度冰层中δD、δ18O同位素值分布特征

      a.达里湖不同厚度冰层中δD的分布特征;b.为达里湖不同厚度冰层中δ18O的分布特征; 图中黑色圆点为H、O同位素值变化示意,各站位样品中H、O同位素的具体数值以图中给出的大小为准

      Fig.  2.  Distribution of δD and δ18O in different layers of lake ice

      图  3  结冰过程中湖冰生长速率、冰体密度及冰体δD、δ18O值变化

      a.湖泊结冰过程中冰体的生长速率(张岩等,2012);b.湖泊结冰过程中冰体密度变化(李志军等,2009);c.湖泊不同厚度冰层中δD变化;d.湖泊不同厚度冰层中δ18O变化.图中阴影条带代表本文湖泊冰体样品采集深度范围,图b~d中黑色实线为实验数据范围,虚线代表各个参数的可能趋势外延趋势,不代表实际变化情况,仅供参考;A7、E2为采样点

      Fig.  3.  Changes of ice grown rate, ice density and δD, δ18O value during the freezing process

      图  4  达里湖冬季湖水与冬季湖冰及夏季湖水中δD、δ18O值变化对比

      a.达里湖冬季湖冰与冰下水体中δD、δ18O值对比;b.达里湖冬季冰下水体与夏季湖水中δD、δ18O值对比.图中实验结果间的连接虚线不代表各点间具体的变化趋势

      Fig.  4.  Comparison of δD, δ18O values of lake water between winter and summer

      图  5  达里湖湖水(冬季、夏季)、湖冰及湖区大气降水等的同位素组成

      GMWL为全球降水曲线(Craig, 1961);LMWL为达里湖区域夏季降水曲线,根据2012年7—9月份达里湖区域大气降水样品的稳定同位素值计算,其公式为:δD=7.71δ18O-0.06,R2=0.897 5

      Fig.  5.  δD-δ18O relation of waters (winter and summer), ice and precipitation in Dali-Nor Lake

      表  1  2013年1月达里湖湖水(冰)取样站点位置

      Table  1.   Sample locations of lake ice and water in the Dali-Nor Lake during January 2013

      序号 站点名称 经度(°) 纬度(°) 水深(m) 冰厚(m)
      1 A7 116.695 9 43.370 8 3.0 0.92
      2 B4 116.598 7 43.332 6 6.8 1.01
      3 C5 116.632 9 43.300 5 8.5 0.93
      4 C7 116.722 3 43.300 0 7.3 1.01
      5 D4 116.603 6 43.267 7 1.7 1.12
      6 D6 116.666 9 43.266 7 7.0 1.21
      7 E1 116.501 2 43.233 6 8.1 0.90
      8 E2 116.516 9 43.216 9 9.5 1.06
      9 E5 116.633 9 43.233 4 7.8 1.10
      下载: 导出CSV

      表  2  达里湖不同厚度冰层间δD、δ18O同位素差值变化

      Table  2.   The change of ΔδD and Δδ18O between different layers of lake ice

      厚度 取样点
      A7 B4 C5 C7 D4 D6 E1 E2 E5
      ΔδD(‰) 35~15 cm 2.50 -0.46 -0.43 2.75 0.69 0.58 2.86 5.46 1.15
      65~15 cm 2.69 1.32 0.28 3.03 0.97 0.51 4.55 8.23 5.45
      Δδ18O(‰) 35~15 cm 0.44 -0.23 0.20 0.72 0.23 -0.03 0.17 1.13 -0.03
      65~15 cm 0.62 0.44 0.15 0.35 0.15 0.08 0.57 1.72 1.77
      下载: 导出CSV

      表  3  达里湖区域降水及湖水中δD、δ18O平均值

      Table  3.   The average value of δD, δ18O in precipitation, lake water and ice

      夏季降水 夏季湖水 冬季湖水 冬季湖冰 冬季平均(湖冰+湖水)
      δD -64.23 -37.66 -41.15(-36.55)* -27.30 -34.23
      δ18O -8.33 -3.38 -2.24(-1.49)* -0.009 -1.123
      注:带“*”的表示括号内数值为去掉A7、E2两点以后的冬季湖泊水体各站位的δD、δ18O的平均值.
      下载: 导出CSV
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    • 收稿日期:  2015-04-03
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