Discovery of Neoproterozoic A-Type Granite in Northern Yangtze Craton and Its Tectonic Significance
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摘要: 对大磊山片麻状花岗岩的研究可以为新元古代罗迪尼亚超大陆在扬子克拉通北缘裂解提供约束.在详细野外地质调查和岩相学工作基础上，对该片麻状花岗岩进行了系统的锆石U-Pb定年、全岩地球化学和锆石原位Lu-Hf同位素分析，研究发现，这些片麻状花岗岩富硅(SiO2=73.18%~77.40%)、碱(Na2O+K2O=8.07%~8.70%)、贫铝(Al2O3=12.11%~13.92%)和镁(MgO=0.10%~0.34%)，富集LILE、Ga、Rb、Th，Zr和Hf元素具明显正异常，Nb、Sr、P、Ti等元素具明显负异常，表现出后造山A型花岗岩(A2型)的特征.这些花岗岩中，锆石均具典型的震荡环带，Th/U比值均大于0.5，为岩浆成因；两个样品的LA-ICP-MS(laser ablation inductively coupled plasma mass spectrometry)锆石的谐和分别是：801.3±3.0 Ma(MSWD=0.62，n=21) 和796.1±6.3 Ma(MSWD=1.70，n=15)，其中一个样品继承锆石谐和年龄为845.0±12.0 Ma(MSWD=1.30，n=6)，表示他们是新元古代岩浆结晶产物.锆石εHf(t)值变化于-7.5~+8.0，正εHf(t)值对应的亏损地幔单阶段模式年龄(tDM1)为1 242~1 059 Ma，负εHf(t)值对应的地壳两阶段模式年龄(tDM2)为1 636~1 981 Ma，显示该地区存在的最古老物质是古元古代(老至1 981 Ma).这些数据结果表明形成大磊山A型花岗岩的初始物质主要为元古代古老地壳物质，暗示该岩浆源自于壳幔混合作用，幔源端元可能源自于伸展拉张背景下地幔岩浆上涌.结合区域研究成果认为，该A型花岗岩的形成与罗迪尼亚超大陆聚合后-裂解中的陆缘弧后拉张环境所引起的深部古元古代地壳拉张垮塌有关.Abstract: Researches on the Daleishan gneissic granites can constrain Neoproterozoic Rodinia supercontinent breakup in the northern margin of Yangtze craton. In this paper, zircon U-Pb dating, in-situ Lu-Hf isotope and whole-rock geochemical compositions analyses are presented for the Daleishan gneissic granites in the northern margin of the Yangtze craton. The results show that the Daleishan gneissic granites have high contents of SiO2 (73.18%-77.40%) and alkali (8.07%-8.70%), but low contents of Al2O3 (12.11%-13.92%) and MgO (0.10%-0.34%), and display enrichment in Ga, Rb, Th, Zr, Hf but depletion in Nb, Sr, P, Ti, which indicates the post-orogenic A-type affinity. Zircons selected from two Daleishan gneissic granitic samples show typical oscillatory zone structure with high ratios of Th/U (greater than 0.5), exhibiting the magmatic zircon genesis. LA-ICP-MS (laser ablation inductively coupled plasma mass spectrometry) zircon U-Pb data from the two samples yield Neoproterozoic crystallization ages of 801.3±3.0 Ma (MSWD=0.62) and 796.1±6.3 Ma (MSWD=1.70), respectively, which are interpreted to represent the intrusion time. In-situ Hf isotopic compositions show that the two gneissic granitic samples have wide range of εHf(t) values that are indicative of a heterogeneity property. εHf(t) values of these zircon ranges from -7.5 to +8.0, with the positive εHf(t) values, coinciding with the single phase model age (tDM1) of the depleted mantle of (1 242-1 059 Ma), and the negative εHf(t) values coinciding with two-phase model age (tDM2) of the crustal of (1 636-1 981 Ma), suggesting that the oldest existing material in the region belongs to Paleoproterozoic (as old as 1 981 Ma). These data show that the source materials of the Daleishan A-type granites were usually derived from Palaeoproterozoic ancient crust. The magmatic source of the granites was originated from the crust-mantle migmatization, and the mantle composition could have been generated from the upwelling of the mantle magma in the extensional background. Combining with the pre-existing regional publications, it is proposed that the Daleishan A-type granite was formed at the crustal extensional background in the continental back-arc setting associated with the assembly-break up process of the Rodinia supercontinent.
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图 1 扬子克拉通北缘大地构造简图(a)和研究区大地构造格架(b)
图a中CYB.华夏陆块，YZB.扬子陆块，COO.中央造山带，NCC.华北克拉通；a.据杨巍然等(2000)；b.据Yang et al.(2000)和Xu et al.(2009)
Fig. 1. Simplified tectonic map of the northern Yangtze craton (a) and tectonic framework of the research area (b)
图 2 研究区地质简图及年代学样品位置(a)和花岗岩地层剖面(b)
Fig. 2. Geological map of the research area and geochronological sample location (a) and geological profile of the granite stratigraphy (b)
图 3 大磊山片麻状花岗岩样品野外特征及镜下照片
Fig. 3. Field and microscopic photos of the Daleishan gneissic granite
图 4 大磊山岩体片麻状花岗岩SiO2-(Na2O+K2O)(a)和SiO2-K2O(b)判别图解
a.据Le Maitre(1989); b.实线据Peccerillo et al.(1976)，虚线据Middlemost(1985); 红色圆圈代表中粗粒片麻状花岗岩，黑色圆圈代表细粒片麻状花岗岩
Fig. 4. Discrimination diagrams SiO2-(Na2O+K2O) (a) and SiO2-K2O (b)for Daleishan gneissic granite
图 5 大磊山岩体片麻状花岗岩稀土元素配分图(a)和微量元素蛛网图(b)球粒陨石和原始地幔标准化值
据Sun and McDonough(1989); 红色填充圆圈为中粗粒片麻状花岗岩，黑色方形为细粒片麻状花岗岩
Fig. 5. (a) Chondrite-and (b) primitive mantle-normalized diagrams for gneissic granite of the Daleishan area
图 6 (a)细粒(D6597) 和(b)中-粗粒(PM301/1) 片麻状花岗岩样品锆石阴极发光、LA-MS-ICP-MS测年及Hf同位素分析点
实心圆圈为U-Pb分析点，虚线圈为Lu-Hf同位素分析点
Fig. 6. Cathodolominescence (CL) images、LA-MS-ICP-MS dating and Hf isotopic analysis of zircons for (a) fine-grain sample D6597 and (b) medium-coarse sample PM301/1 of Daleishan gneissic granite zircon
图 7 (a)细粒(D6597) 和(b)中-粗粒(PM301/1) 片麻状花岗岩样品LA-ICP-MS锆石U-Pb谐和图
Fig. 7. Concordia plots showing the geochronological results of the LA-ICP-MS zircon U-Pb of (a) fine-grain sample D6597 and (b) medium-coarse sample PM301/1 of Daleishan gneissic granite
图 9 样品PM301/1(a)成岩和(b)残留锆石εHf(t)值分布
Fig. 9. εHf(t)values of diagenetic zircon (a) and residual zircons (b) for sample PM301/1
图 10 大磊山岩体片麻状花岗岩(a)10 000×Ga/Al-Ce和(b)10 000×Ga/Al-Zr判别图解
据Whalen et al.(1987)；红色圆圈代表中粗粒片麻状花岗岩，黑色圆圈代表细粒片麻状花岗岩
Fig. 10. Dicrimination diagrams of (a) 10 000×Ga/Al-Ce and (10 000×Ga/Al-Zr) for the Daleishan gneissic granite
图 11 大磊山岩体片麻状花岗岩εHf(t)-成岩年龄(t)图解
红色为样品D6597，黑色为样品PM301/1
Fig. 11. Age (t) versus εHf(t) values diagrams for the Daleishan gneissic granite
图 12 (a)Y/Nb-Ce/N和(b)Nb-Y-Ce判别图解
A1.非造山环境; A2.后碰撞环境; OIB.洋岛; IAB.岛弧; 图据Eby et al.(1992)，Pearce et al.(1984); 黑色圆圈代表细粒片麻状花岗岩，红色圆圈代表中粗粒片麻状花岗岩
Fig. 12. Dicrimination diagrams of (a) Y/Nb-Ce/ Nb and (b) Nb-Y-Ce for the Daleishan gneissic granite
表 1 大磊山岩体片麻状花岗岩主量(%)及微量元素(10-6)分析结果
Table 1. Major (%) and trace element (10-6) compositions of the Daleishan gneissic granite
岩性样号 中粗粒片麻状花岗岩 细粒片麻状花岗岩 D3034/1 D2114/1 D3155/1 D4213/1 D3016/1 D6597/1 D3155/1 D3006/1 SiO2 75.59 74.55 76.20 74.70 73.18 77.40 76.34 76.79 TiO2 0.16 0.11 0.19 0.21 0.26 0.10 0.09 0.09 Al2O3 13.06 13.92 12.70 13.50 13.83 12.11 12.35 12.26 Fe2O3 0.89 1.24 1.02 1.07 1.80 0.39 0.41 0.73 FeO 0.37 0.25 0.32 0.58 0.68 0.67 0.49 0.59 FeOT 1.17 1.37 1.24 1.54 2.30 1.02 0.85 1.25 MnO 0.06 0.02 0.03 0.04 0.11 0.02 < 0.01 0.02 MgO 0.21 0.25 0.31 0.34 0.31 0.19 0.10 0.15 CaO 0.60 0.13 0.19 0.64 0.68 0.10 0.21 0.08 Na2O 3.50 4.28 3.49 3.92 3.89 2.77 3.33 3.63 K2O 4.69 4.14 4.78 4.24 4.19 5.84 5.37 4.77 P2O5 0.03 0.03 0.04 0.05 0.06 0.01 0.01 < 0.01 LOI 0.64 0.90 0.58 0.57 0.80 0.35 0.71 0.52 Rb 184.40 188.10 180.54 147.00 107.64 197.59 229.00 188.50 Ba 421.55 419.80 233.65 1164.35 761.70 179.13 179.13 268.69 Th 18.51 20.34 26.94 12.85 8.50 24.00 24.50 26.60 U 1.94 2.09 1.73 1.60 1.42 5.45 2.85 4.88 Nb 19.03 12.32 20.87 12.30 18.12 15.80 20.90 19.60 Sr 50.89 40.78 28.14 89.60 64.51 18.80 25.60 34.20 Nd 31.50 15.52 28.07 32.70 56.47 33.60 49.20 18.30 Zr 128.00 160.50 131.50 179.00 300.20 119.00 139.00 126.00 Hf 3.42 4.59 5.06 4.80 9.43 4.70 5.60 5.20 Yb 4.17 3.30 4.05 2.89 4.52 2.94 5.74 5.00 Lu 0.67 0.55 0.62 0.42 0.70 0.51 0.85 0.77 Y 36.20 30.41 30.68 23.50 49.56 20.40 60.30 39.80 La 38.95 21.99 43.14 43.20 66.11 28.60 58.10 20.90 Ce 82.05 38.44 100.30 91.00 92.46 80.60 93.00 33.80 Pr 8.69 4.44 8.47 8.89 14.74 10.80 13.75 5.15 Nd 31.5 15.52 28.07 32.70 56.47 33.60 49.20 18.30 Sm 5.98 3.23 4.90 5.79 10.44 6.62 10.40 4.09 Eu 0.57 0.45 0.52 0.92 1.26 0.35 0.59 0.24 Gd 5.38 3.36 4.50 4.60 9.34 3.79 9.70 3.88 Tb 1.01 0.73 0.80 0.72 1.57 0.59 1.64 0.73 Dy 6.13 4.79 4.75 4.26 8.41 3.71 9.91 5.33 Ho 1.31 1.02 1.08 0.92 1.79 0.78 1.98 1.28 Er 3.93 3.01 3.37 2.53 4.83 2.32 5.56 4.09 Tm 0.64 0.50 0.61 0.41 0.74 0.39 0.88 0.70 Yb 4.17 3.30 4.05 2.89 4.52 2.94 5.74 5.00 Lu 0.67 0.55 0.62 0.42 0.70 0.51 0.85 0.77 ΣREE 191.00 101.32 205.18 199.25 273.40 175.60 261.30 104.26 LREE/HREE 7.21 4.87 9.37 10.90 7.57 10.68 6.21 3.79 LaN/YbN 6.70 4.78 7.63 10.72 10.48 6.98 7.26 3.00 δEu 0.30 0.41 0.33 0.53 0.38 0.20 0.18 0.18 
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表 2 大磊山岩体片麻状花岗岩D6597 LA-ICP-MS岩浆锆石U-Pb定年结果
Table 2. LA-ICP-MS zircon U-Pb data of the gneissic granite sample D6597 in the Daleishan granitoid
点号 含量(10-6) Th/U U-Th-Pb同位素比值±1σ 同位素年龄(Ma)±1σ 232Th 238U 207Pb/206Pb 207Pb/235U 206Pb/238U 207Pb/206Pb 207Pb/235U 206Pb/238U D6597-01 531.90 490.23 1.085 0.065 3±0.002 4 1.173 2±0.043 6 0.130 2±0.001 3 783.34±77.77 788.12±20.36 789.03±7.37 D6597-02 408.63 444.65 0.919 0.068 9±0.002 2 1.261 7±0.040 6 0.133 0±0.001 4 894.45±66.67 828.69±18.24 804.98±7.93 D6597-03 640.43 553.35 1.157 0.067 8±0.001 9 1.215 5±0.033 0 0.130 4±0.001 1 861.11±56.64 807.72±15.13 790.34±6.45 D6597-04 1 998.20 430.26 4.644 0.064 7±0.001 9 1.180 2±0.034 9 0.132 4±0.001 1 764.82±62.96 791.41±16.25 801.41±6.27 D6597-05 796.04 892.36 78.250 0.101 7±0.002 7 1.733 2±0.044 8 0.124 3±0.001 1 1 654.63±48.92 1 020.95±16.66 755.40±6.18 D6597-06 467.19 309.26 1.511 0.068 1±0.002 6 1.235 9±0.046 4 0.133 3±0.001 4 872.22±79.63 817.03±21.10 806.60±8.00 D6597-07 621.16 600.89 1.034 0.068 7±0.001 8 1.247 7±0.033 8 0.132 0±0.001 1 900.00±55.55 822.37±15.28 799.28±6.22 D6597-08 596.53 460.37 1.296 0.066 0±0.002 1 1.199 7±0.037 3 0.132 3±0.001 1 805.56±66.66 800.45±17.23 801.12±6.34 D6597-09 1341.2 966.65 5.488 0.049 8±0.003 3 0.133 7±0.008 5 0.019 8±0.000 3 187.12±149.06 127.38±7.61 126.26±1.72 D6597-10 513.78 546.20 91.760 0.087 9±0.002 6 1.687 8±0.051 0 0.138 6±0.001 3 1 379.94±55.56 1 003.93±19.26 836.70±7.39 D6597-11 388.97 447.97 0.868 0.063 4±0.002 3 1.158 8±0.041 5 0.133 1±0.001 5 720.38±79.62 781.41±19.53 805.25±8.4 D6597-12 569.85 598.38 0.952 0.067 7±0.001 9 1.248 9±0.035 5 0.133 8±0.001 2 858.94±59.26 822.89±16.04 809.54±7.07 D6597-13 897.38 414.37 2.166 0.062 6±0.002 2 1.142 9±0.038 9 0.132 7±0.001 3 694.46±74.07 773.90±18.43 803.51±7.27 D6597-14 638.29 593.35 1.076 0.065 3±0.001 7 1.196 5±0.031 7 0.132 3±0.001 1 783.34±55.55 798.98±14.65 800.92±6.08 D6597-15 483.17 584.33 0.827 0.070 0±0.001 8 1.2833±0.0316 0.132 5±0.001 1 927.78±56.48 838.34±14.05 802.37±6.11 D6597-16 908.71 596.97 1.522 0.067 3±0.002 1 1.224 3±0.035 6 0.131 8±0.001 1 850.00±69.44 811.74±16.26 798.00±6.40 D6597-17 1 211.20 391.78 3.091 0.064 2±0.001 9 1.1904±0.034 7 0.133 8±0.001 3 746.30±62.96 796.17±16.08 809.78±7.48 D6597-18 366.78 265.91 1.379 0.065 6±0.002 5 1.2028±0.044 1 0.133 8±0.001 4 792.28±81.47 801.89±20.33 809.55±7.97 D6597-19 284.32 241.60 1.177 0.061 3±0.002 7 1.110 1±0.047 6 0.131 2±0.001 4 650.02±94.43 758.22±22.90 794.85±7.91 D6597-20 412.69 315.25 1.309 0.062 4±0.002 4 1.131 9±0.043 4 0.132 2±0.001 4 700.01±81.47 768.64±20.68 800.19±8.00 D6597-21 567.14 491.47 1.154 0.0656±0.002 4 1.190 3±0.046 6 0.131 6±0.001 2 792.28±77.77 796.09±21.61 797.15±6.68 D6597-22 439.25 468.36 0.938 0.063 8±0.002 6 1.159 0±0.050 7 0.132 2±0.001 1 744.45±85.18 781.50±23.86 800.56±6.42 D6597-23 423.42 455.92 0.929 0.061 4±0.002 7 1.114 0±0.054 7 0.132 7±0.001 2 651.56±87.95 760.11±26.27 803.46±7.04 D6597-24 306.31 293.09 1.045 0.062 2±0.003 5 1.133 8±0.07 1 0.133 4±0.001 4 679.64±113.87 769.54±33.78 807.03±8.07
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表 3 大磊山岩体片麻状花岗岩PM301/1 LA-ICP-MS岩浆锆石U-Pb定年结果
Table 3. 3LA-ICP-MS zircon U-Pb data of the gneissic granite sample PM301/1 in the Daleishan granitoid
点号 含量(10-6) Th/U U-Th-Pb同位素比值±1σ 同位素年龄(Ma)±1σ 232Th 238U 207Pb/206Pb 207Pb/235U 206Pb/238U 207Pb/206Pb 207Pb/235U 206Pb/238U PM302/1-01 493.22 509.06 0.969 0.070 5±0.002 2 1.260 2±0.037 7 0.128 7±0.001 2 942.6±63.0 828.0±17.0 780.5±6.9 PM302/1-02 463.13 282.87 1.637 0.068 2±0.002 9 1.213 0±0.050 8 0.128 8±0.001 7 875.9±88.1 806.6±23.3 781.1±9.8 PM302/1-03 229.98 234.10 0.982 0.072 5±0.003 3 1.333 2±0.058 9 0.133 2±0.000 2 999.1±91.5 860.3±25.6 805.9±11.6 PM302/1-04 302.45 266.40 1.135 0.071 4±0.002 8 1.285 2±0.048 3 0.130 6±0.001 7 968.5±84.3 839.2±21.5 791.2±9.8 PM302/1-05 978.17 367.85 2.659 0.066 5±0.002 9 1.205 2±0.054 9 0.129 6±0.001 8 821.9±91.5 803.0±25.3 785.5±10.3 PM302/1-06 547.85 490.63 1.117 0.065 7±0.002 6 1.308 9±0.050 0 0.142 8±0.001 6 798.2±78.7 849.7±22.0 860.5±8.9 PM302/1-07 407.41 251.32 1.621 0.063 3±0.002 7 1.157 7±0.047 7 0.132 5±0.001 5 720.4±86.1 780.9±22.5 802.2±8.6 PM302/1-08 396.84 384.01 1.033 0.069 6±0.002 2 1.263 7±0.037 5 0.131 7±0.001 2 916.7±65.6 829.6±16.8 797.6±7.0 PM302/1-09 333.75 379.50 0.879 0.064 7±0.002 3 1.180 0±0.040 7 0.132 2±0.001 4 764.8±75.9 791.3±19.0 800.4±7.8 PM302/1-10 1033.79 352.16 2.936 0.067 9±0.002 6 1.297 5±0.049 0 0.138 0±0.001 6 877.8±77.8 844.6±21.7 833.2±9.3 PM302/1-11 288.34 250.45 1.151 0.064 2±0.003 1 1.203 6±0.054 4 0.137 7±0.002 2 750.0±103.7 802.2±25.1 831.7±12.4 PM302/1-12 84.01 106.6 0.788 0.075 0±0.005 5 1.409 8±0.091 7 0.141 0±0.002 5 1 069.4±146.3 893.1±38.7 850.2±14.1 PM302/1-13 603.18 257.29 2.344 0.071 3±0.003 0 1.284 1±0.054 0 0.131 7±0.001 5 964.8±87.0 838.7±24.0 797.5±8.6 PM302/1-14 265.49 342.78 0.775 0.065 7±0.002 6 1.208 8±0.046 4 0.134 5±0.001 4 794.4±82.6 804.6±21.3 813.7±8.2 PM302/1-15 494.92 515.50 0.960 0.075 0±0.002 9 1.330 4±0.051 5 0.128 8±0.001 2 1 133.3±79.6 859.1±22.4 781.3±7.0 PM302/1-16 456.10 398.82 1.144 0.065 5±0.002 7 1.199 7±0.050 4 0.132 6±0.0018 790.7±87.0 800.4±23.2 802.6±10.1 PM302/1-17 417.77 404.34 1.033 0.066 7±0.002 5 1.2183±0.045 3 0.133 0±0.001 8 827.8±79.6 809.0±20.7 804.7±10.2 PM302/1-18 218.38 295.86 0.738 0.065 5±0.002 9 1.194 9±0.052 3 0.133 0±0.001 6 790.7±92.6 798.2±24.2 804.7±8.8 PM302/1-19 418.33 407.06 1.028 0.064 3±0.002 2 1.239 5±0.041 1 0.140 4±0.001 3 750.0±78.7 818.7±18.6 846.8±7.3 PM302/1-20 228.57 211.42 1.081 0.060 7±0.003 1 1.111 0±0.055 2 0.134 1±0.001 8 627.8±105.4 758.7±26.6 811.5±10.0 PM302/1-21 243.23 272.66 0.892 0.064 7±0.002 8 1.222 7±0.053 1 0.138 3±0.002 4 764.8±60.2 811.0±24.3 834.9±13.6
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表 4 大磊山岩体片麻状花岗岩D6597岩浆锆石Hf同位素组成
Table 4. Lu-Hf isotope compositions of the gneissic granite sample D6597 in the Daleishan granitoid
点号 176Hf/177Hf 1σ 176Lu/177Hf 1σ 176Yb/177Hf 1σ t(Ma) εHf(0) 1σ εHf(t) 1σ tDM1 (Ma) tDM2 (Ma) fLu/Hf 1 0.282 125 0.000 017 0.001 091 0.000 008 0.033 252 0.000 48 796 -22.87 0.8 -5.87 0.84 1 590.61 1 901.71 -0.97 2 0.282 275 0.000 027 0.001 962 0.000 043 0.061 676 0.001 86 796 -17.56 1.09 -1.02 1.13 1 413.81 1 635.68 -0.94 3 0.282 558 0.000 037 0.003 757 0.000 032 0.118 907 0.000 55 796 -7.579 1.41 8.02 1.44 1 059.84 1 136.98 -0.89 4 0.282 112 0.000 026 0.001 013 0.000 016 0.028 364 0.000 68 796 -23.33 1.04 -6.30 1.08 1 605.60 1 924.94 -0.97 5 0.282 176 0.000 019 0.001 063 0.000 002 0.030 677 0.000 28 861 -21.09 0.84 -2.68 0.88 1 519.65 1 778.22 -0.97 6 0.282 249 0.000 024 0.001 529 0.000 058 0.045 529 0.001 37 796 -18.51 0.98 -1.74 1.04 1 435.15 1 674.98 -0.95 7 0.282 245 0.000 025 0.002 027 0.000 026 0.059 721 0.000 38 833 -18.64 1.01 -1.36 1.05 1 459.81 1 683.41 -0.94 8 0.282 135 0.000 021 0.001 050 0.000 006 0.030 248 0.000 10 832 -22.52 0.91 -4.73 0.95 1 575.37 1 867.56 -0.97 9 0.282 175 0.000 021 0.001 107 0.000 009 0.031 941 0.000 40 796 -21.13 0.9 -4.14 0.94 1 522.64 1 806.71 -0.97 10 0.282 215 0.000 020 0.001 211 0.000 009 0.036 462 0.000 55 796 -19.69 0.87 -2.76 0.91 1 469.94 1 730.81 -0.96
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表 5 大磊山岩体片麻状花岗岩PM301-1岩浆锆石Hf同位素组成
Table 5. Lu-Hf isotope compositions of the gneissic granite sample PM301-1 in the Daleishan granitoid
点号 176Hf/177Hf 1σ 176Lu/177Hf 1σ 176Yb/177Hf 1σ t(Ma) εHf(0) 1σ εHf(t) 1σ tDM1 (Ma) tDM2 (Ma) fLu/Hf 1 0.282 420 0.000 032 0.003 008 0.000 059 0.091 968 0.001 575 781 -12.5 1.2 3.2 1.3 1 242 1 390 -0.91 2 0.282 105 0.000 019 0.001 089 0.000 028 0.029 445 0.000 898 806 -23.6 0.8 -6.4 0.9 1 619 1 937 -0.97 3 0.282 146 0.000 026 0.001 103 0.000 007 0.031 471 0.000 352 791 -22.2 1.0 -5.3 1.1 1 563 1 865 -0.97 4 0.282 510 0.000 035 0.003 061 0.000 047 0.091 394 0.001 780 786 -9.3 1.4 6.5 1.4 1 110 1 212 -0.91 5 0.282 242 0.000 023 0.001 584 0.000 010 0.047 003 0.000 394 861 -18.8 1.0 -0.6 1.0 1 447 1 666 -0.95 6 0.282 167 0.000 026 0.001 228 0.000 013 0.034 397 0.000 292 800 -21.4 1.0 -4.4 1.1 1 538 1 823 -0.96 7 0.282 488 0.000 034 0.003 183 0.000 031 0.095 571 0.000 469 833 -10.0 1.3 6.6 1.3 1 146 1 245 -0.90 8 0.282 182 0.000 028 0.001 306 0.000 053 0.038 229 0.001 508 832 -20.9 1.1 -3.2 1.2 1 520 1 784 -0.96 9 0.282 228 0.000 031 0.001 816 0.000 022 0.054 271 0.000 568 802 -19.2 1.2 -2.5 1.2 1 475 1 721 -0.95 10 0.282 241 0.000 027 0.001 609 0.000 071 0.046 716 0.001 961 798 -18.8 1.1 -2.0 1.1 1 449 1 691 -0.95 11 0.282 085 0.000 022 0.000920 0.000 008 0.026 532 0.000 377 781 -24.3 0.9 -7.5 1.0 1 639 1 981 -0.97 12 0.282 126 0.000 023 0.001 195 0.000 008 0.035 452 0.000 332 803 -22.8 1.0 -5.8 1.0 1 594 1 901 -0.96 13 0.282 221 0.000 029 0.001 675 0.000 113 0.053 218 0.004 902 805 -19.5 1.1 -2.6 1.2 1 479 1 729 -0.95 14 0.282 161 0.000 022 0.001 111 0.000 007 0.032 048 0.000 136 847 -21.6 0.9 -3.5 1.0 1 541 1 812 -0.97 15 0.282 196 0.000 025 0.001 712 0.000 024 0.046 725 0.000 816 812 -20.4 1.0 -3.3 1.1 1 516 1 776 -0.95
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