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    阿尔泰南缘乌拉斯沟铜矿床S-Pb-Sr-Nd-C-H-O同位素特征及其对成矿物质和流体来源限定

    卢琦园 郑义 王成明 王岳军

    卢琦园, 郑义, 王成明, 王岳军, 2018. 阿尔泰南缘乌拉斯沟铜矿床S-Pb-Sr-Nd-C-H-O同位素特征及其对成矿物质和流体来源限定. 地球科学, 43(9): 3141-3153. doi: 10.3799/dqkx.2018.135
    引用本文: 卢琦园, 郑义, 王成明, 王岳军, 2018. 阿尔泰南缘乌拉斯沟铜矿床S-Pb-Sr-Nd-C-H-O同位素特征及其对成矿物质和流体来源限定. 地球科学, 43(9): 3141-3153. doi: 10.3799/dqkx.2018.135
    Lu Qiyuan, Zheng Yi, Wang Chengming, Wang Yuejun, 2018. S-Pb-Sr-Nd-C-H-O Isotopic Geochemistry of the Wulasigou Cu Deposit in the South Altay: Constraints for the Fluid and Metal Sources. Earth Science, 43(9): 3141-3153. doi: 10.3799/dqkx.2018.135
    Citation: Lu Qiyuan, Zheng Yi, Wang Chengming, Wang Yuejun, 2018. S-Pb-Sr-Nd-C-H-O Isotopic Geochemistry of the Wulasigou Cu Deposit in the South Altay: Constraints for the Fluid and Metal Sources. Earth Science, 43(9): 3141-3153. doi: 10.3799/dqkx.2018.135

    阿尔泰南缘乌拉斯沟铜矿床S-Pb-Sr-Nd-C-H-O同位素特征及其对成矿物质和流体来源限定

    doi: 10.3799/dqkx.2018.135
    基金项目: 

    珠江科技新星项目 201710010027

    广东省引进人才创新创业团队项目 2016ZT06N331

    国家自然科学基金项目 41502068

    广东省自然科学基金杰出青年基金项目 2018B030306021

    科技部国家重点研发计划项目 2016YFC0600408

    详细信息
      作者简介:

      卢琦园(1995-), 男, 硕士研究生, 主要从事矿床学方面的研究

      通讯作者:

      郑义

    • 中图分类号: P611

    S-Pb-Sr-Nd-C-H-O Isotopic Geochemistry of the Wulasigou Cu Deposit in the South Altay: Constraints for the Fluid and Metal Sources

    • 摘要: 新疆乌拉斯沟铜矿床位于阿尔泰造山带南缘克兰盆地内,为近年来新发现的矿床,受NW向断裂控制的脉状矿体产于泥盆系康布铁堡组变质火山岩系中,目前其成矿流体和成矿物质来源尚不明确.在细致的矿床地质研究基础上,通过开展S-Pb-Sr-Nd-C-H-O同位素分析,根据野外和显微镜下观察,可将乌拉斯沟铜矿床的形成划分为黄铁矿-磁铁矿-石英、黄铜矿-绿泥石-绿帘石-石英及石英-碳酸盐阶段.同位素分析结果显示:乌拉斯沟铜矿硫化物样品δ34S值为0.1‰~3.2‰,平均为1.6‰,落入未矿化围岩δ34S值范围(-4.7‰~18.68‰),矿石硫可能源自康布铁堡组.成矿晚阶段的方解石样品δ13CV-PDB‰=-1.1‰,δ18OV-PDB‰=-20.3‰,海相碳酸盐地层和有机碳是可能的碳质来源.8件黄铁矿的Pb同位素为206Pb/204Pb=17.939~18.508(平均18.255),207Pb/204Pb=15.519~15.674(平均15.578),208Pb/204Pb=37.881~38.653(平均38.209),与康布铁堡组围岩类似.初始ISr(220 Ma)为0.710 4~0.711 7,平均值为0.711 1,初始143Nd/144Nd值为0.512 002~0.512 240(平均0.512 103).矿石Sr-Nd-Pb同位素组成均指示乌拉斯沟铜矿成矿物质可能主要源自围岩康布铁堡组,并可能有外来成矿物质的加入.流体的δDV-SMOW变化于-103.8‰~-92‰(平均值为-99.2‰),石英和方解石矿物的δ18OV-SMOW值集中在9.4‰~11.5‰(平均值为10.4‰),δ18OH2O值为2.1‰~4.2‰(平均值为3.1‰),结合流体包裹体物理化学特征,成矿热液可能来源于变质水,但可能受到大气降水的影响而偏移.因此,乌拉斯沟铜矿成矿物质主要来源于赋矿围岩的变质脱挥发分作用,这与造山型矿床的成矿机制吻合.

       

    • 图  1  研究区大地构造背景和区域地质及矿产分布

      a.研究区大地构造背景;b.阿尔泰南缘阿尔泰南缘克兰盆地区域地质及矿产分布.据Zheng et al.(2012)及其引文

      Fig.  1.  Tectonic background and regional geology and mineral distribution of the study area

      图  2  乌拉斯沟铜矿床矿区地质简图(a)及A1-A2勘探线剖面(b)

      Zheng et al.(2012)及其引文

      Fig.  2.  Geological sketch and exploration line A1-A2 of the Wulasigou Cu deposit

      图  3  乌拉斯沟铜矿床硫同位素组成

      Fig.  3.  S isotopic composition of pyrite and wall rocks in the Wulasigou Cu deposit

      图  4  乌拉斯沟铜矿床成矿流体δ18O-δD组成

      底图据Taylor(1974)

      Fig.  4.  δ18O-δD isotopic composition of the ore-forming fluid in the Wulasigou Cu deposit

      图  5  乌拉斯沟铜矿金属硫化物及围岩初始Sr、Nd同位素图解

      Fig.  5.  Initial Sr-Nd isotopic composition of sulfides and wall rocks in the Wulasigou deposit

      图  6  乌拉斯沟矿石硫化物及围岩铅同位素图解

      Fig.  6.  Pb isotopic diagram of sulfides and wall rocks of the Wulasigou Cu deposit

      表  1  乌拉斯沟铜矿床硫化物及围岩硫同位素组成

      Table  1.   S isotopic composition of sulfide and wall rocks in the Wulasigou Cu deposit

      序号 样品编号 δ34SV-CDT(‰) 测试样品 数据来源
      1 10WL-09 1.7 黄铁矿 本文
      2 10WL-12 2.9 黄铁矿 本文
      3 10WL-Q5B 2.0 黄铁矿 本文
      4 10WL-13 3.2 黄铁矿 本文
      5 10WL-Q1 1.0 黄铁矿 本文
      6 10WL-Q8B 0.7 黄铁矿 本文
      7 10WL-Q4 0.1 黄铁矿 本文
      8 10WL-Q3 1.3 黄铁矿 本文
      9 10TMZK-34A 5.6 无矿化大理岩 Niu et al., 2017
      10 SL-30 7.5 无矿化绿片岩 Niu et al., 2017
      11 TM-26 7.5 未矿化大理岩 Niu et al., 2017
      12 SL-38 16.5 未矿化凝灰岩 Niu et al., 2017
      13 SL-37 16.4 未矿化凝灰岩 Niu et al., 2017
      14 SL-15 18.7 未矿化凝灰岩 Niu et al., 2017
      15 10DD-13 -4.7 无矿化灰岩 Niu et al., 2017
      16 TM-51 -19.3 矿化绿泥片岩 Niu et al., 2017
      17 TM-01 -24.1 浸染矿化砂岩 Niu et al., 2017
      18 TM-06 -16.8 矿化绿泥片岩 Niu et al., 2017
      19 TM-14 -13.7 矿化绿泥片岩 Niu et al., 2017
      下载: 导出CSV

      表  2  乌拉斯沟铜矿床氢氧同位素组成

      Table  2.   δ18O-δD isotopic composition of quartz in the Wulasigou Cu deposit

      序号 样品编号 岩性 δDV-SMOW(‰) δ18OV-SMOW(‰) δ18OH2O(‰) T(℃)
      1 WL-Q1 石英 / 9.4 2.1 289
      2 WL-Q3 石英 -103.8 10.8 3.5 289
      3 WL-Q4 石英 -103.7 10.4 3.1 289
      4 WL-Q8B 石英 / 10.1 2.8 289
      5 WL-13 石英 -92.0 10.5 3.2 289
      6 WL-09 石英 / 10.7 3.4 289
      7 WL-12 石英 -94.8 11.5 4.2 289
      8 WL-Q5B 石英 -101.6 9.7 2.4 289
      下载: 导出CSV

      表  3  乌拉斯沟铜矿床碳同位素组成

      Table  3.   C isotopic composition of the Wulasigou Cu deposit

      样品编号 矿物/岩石 δ13CV-PDB(‰) δ18OV-PDB(‰) δ18OV-SMOW(‰) 数据来源
      10WL-0-5C 方解石 -1.1 -20.3 9.9 本文
      DDZK-7 大理岩 -1.2 -15.8 14.7 Niu et al., 2017
      10TMZK-37B 大理岩 2.7 -18.5 11.9 Niu et al., 2017
      10TMZK-34A 大理岩 2.2 -20.5 9.7 Niu et al., 2017
      10DD-13 灰岩 -1.6 -15.8 14.6 Niu et al., 2017
      10SK-11A 灰岩 -1.7 -16.3 14.1 Niu et al., 2017
        注:本次测试只获得1件成矿晚阶段的方解石样品(样品编号10WL-0-5C),δ13CV-PDB(‰)=-1.1‰,δ18OV-PDB(‰)=-20.3‰.Niu et al.(2017)获得围岩C同位素值介于-1.7‰~2.7‰(平均值为2.1‰),其中大理岩δ13CV-PDB为-1.2‰~2.7‰(平均值为1.2‰),灰岩δ13CV-PDB为-1.6‰~-1.7‰(平均值-1.7‰).
      下载: 导出CSV

      表  4  乌拉斯沟矿床金属硫化物及围岩Sr同位素组成

      Table  4.   Sr isotopic composition of sulfides and wall rocks in the Wulasigou deposit

      样品号 样品名称 Rb(10-6) Sr(10-6) 87Rb/86Sr 87Sr/86Sr ISr(220 Ma)
      10WL-09 黄铁矿 0.03 0.37 0.246 8 0.712 3 0.711 6
      10WL-12 黄铁矿 0.13 1.52 0.239 4 0.712 0 0.711 3
      10WL-Q5B 黄铁矿 0.09 1.16 0.229 4 0.712 4 0.711 7
      10WL-13 黄铁矿 0.24 0.79 0.889 4 0.713 6 0.710 8
      10WL-Q1 黄铁矿 0.05 0.68 0.194 4 0.712 0 0.711 4
      10WL-Q8B 黄铁矿 0.10 1.42 0.207 0 0.710 7 0.710 1
      10WL-Q4 黄铁矿 0.04 0.73 0.160 6 0.710 9 0.710 4
      10WL-Q3 黄铁矿 0.05 0.51 0.278 0 0.712 4 0.711 5
      平均值(n=8) 0.711 1
      样品号 样品名称 Rb(10-6) Sr(10-6) 87Rb/86Sr 87Sr/86Sr ISr(220 Ma)
      10SKY-09 方解石 0.14 341.0 0.001 2 0.720 5 0.720 5
      10SKY-07 方解石 0.13 459.0 0.000 8 0.717 3 0.717 3
      10SKY-05 方解石 0.22 511.0 0.001 3 0.714 2 0.714 2
      10SKY-02 方解石 0.06 315.0 0.000 6 0.717 2 0.717 2
      10TMZK 大理岩 0.84 103.0 0.023 6 0.713 1 0.713 0
      10DD-13 灰岩 107.00 372.0 0.833 5 0.710 9 0.708 3
      10TM-11 晶屑凝灰岩 97.80 12.3 23.08 5 0.809 8 0.737 6
      10SK-10 晶屑凝灰岩 51.10 33.4 4.429 4 0.742 3 0.728 5
      10SK-3a 钙质粉砂岩 146.00 49.8 8.467 1 0.754 2 0.727 7
      SL-30 绿片岩 6.98 348.0 0.058 1 0.711 8 0.711 6
      平均值(n=10) 0.719 6
        注:表中的87Rb/86Sr是根据实测的样品元素含量和同位素比值计算所得,成矿年龄采用黑云母Ar-Ar年龄220 Ma(Zheng et al., 2012),将测得的87Sr/86Sr同位素比值返算回220 Ma时的87Sr/86Sr比值ISr(220 Ma);初始Sr计算公式:ISr=(87Sr/86Sr)m-(87Rb/86Sr)m(eλt-1).
      下载: 导出CSV

      表  5  乌拉斯沟铜矿金属硫化物及围岩Nd同位素组成

      Table  5.   Nd isotopic composition of sulfides and wall rocks in the Wulasigou deposit

      样品号 样品名称 Sm(10-6) Nd(10-6) 147Sm/144Nd 143Nd/144Nd (143Nd/144Nd)i εNd
      10WL-09 黄铁矿 0.35 1.00 0.209 1 0.512 444 0.512 143 -9.7
      10WL-12 黄铁矿 0.22 0.80 0.161 5 0.512 473 0.512 240 -7.8
      10WL-Q5B 黄铁矿 0.09 0.25 0.204 4 0.512 387 0.512 093 -10.6
      10WL-13 黄铁矿 0.39 2.19 0.106 0 0.512 325 0.512 172 -9.1
      10WL-Q1 黄铁矿 0.05 0.20 0.139 5 0.512 233 0.512 031 -11.8
      10WL-Q8B 黄铁矿 0.24 1.23 0.120 4 0.512 260 0.512 087 -10.8
      10WL-Q4 黄铁矿 0.17 0.67 0.148 3 0.512 216 0.512 002 -12.4
      10WL-Q3 黄铁矿 0.05 0.19 0.168 0 0.512 300 0.512 058 -11.3
      平均值(n=8) 0.512 103 -10.4
      10SKY-09 方解石 0.16 0.53 0.179 1 0.512 470 0.512 212 -12.4
      10SKY-07 方解石 0.25 0.63 0.239 9 0.512 681 0.512 336 -11.4
      10SKY-05 方解石 1.04 2.79 0.225 1 0.512 632 0.512 308 -11.6
      10SKY-02 方解石 0.54 1.28 0.254 8 0.512 640 0.512 273 -13.0
      10TMZK 大理岩 0.43 1.87 0.140 0 0.512 450 0.512 248 -10.8
      10DD-13 灰岩 3.73 18.6 0.121 7 0.512 322 0.512 147 -12.4
      10TM-11 晶屑凝灰岩 3.09 15.8 0.117 9 0.512 550 0.512 380 -7.7
      10SK-10 晶屑凝灰岩 7.82 39.8 0.118 7 0.512 499 0.512 328 -8.8
      10SK-3a 钙质粉砂岩 7.24 36.8 0.119 1 0.512 559 0.512 388 -7.6
      SL-30 绿片岩 4.27 15.2 0.169 8 0.512 881 0.512 636 -3.9
      平均值(n=10) 0.512 326 -10.2
        注:表中的147Sm/144Nd是根据实测的样品元素含量和同位素比值计算所得,成矿年龄采用黑云母Ar-Ar成矿年龄220 Ma(Zheng et al., 2012),将测得的143Nd/144Nd同位素比值返算回220 Ma时的(143Nd/144Nd)i(220 Ma)εNd(t)值;初始Nd计算公式:(143Nd/144Nd)=(143Nd/144Nd)m-(147Sm/144Nd)m(eλt-1),其中λ=0.006 54×10-9 a-1.计算过程中,球粒陨石均一储库(CHUR)Nd同位素参数采用143Nd/144Nd=0.512 638(Goldstein et al., 1984),147Sm/144Nd=0.196 7(Jacobsen and Wasserburg, 1984).
      下载: 导出CSV

      表  6  乌拉斯沟矿床金属硫化物及围岩Pb同位素组成

      Table  6.   Pb isotopic composition of sulfides and wall rocks in the Wulasigou deposit

      样品号 样品名称 206Pb/
      204Pb
      207Pb/
      204Pb
      208Pb/
      204Pb
      10WL-09 黄铁矿 18.255 15.570 38.123
      10WL-12 黄铁矿 18.449 15.648 38.537
      10WL-Q5B 黄铁矿 18.199 15.519 37.888
      10WL-13 黄铁矿 18.455 15.674 38.653
      10WL-Q1 黄铁矿 18.508 15.611 38.436
      10WL-Q8B 黄铁矿 18.087 15.545 37.881
      10WL-Q4 黄铁矿 18.145 15.526 37.901
      10SK-06 黄铁矿 17.939 15.528 38.250
      平均值(n=8) 18.255 15.578 38.209
      10TMZK 大理岩 18.066 15.510 37.762
      10DD-13 灰岩 18.102 15.506 37.813
      10TM-11 晶屑凝灰岩 18.651 15.551 38.576
      10SK-10 晶屑凝灰岩 18.674 15.551 38.541
      10SK-3a 钙质粉砂岩 18.850 15.584 38.707
      SL-30 绿片岩 18.265 15.528 38.070
      平均值(n=6)
      下载: 导出CSV
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