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    扬子陆块北缘东河铂钯矿化超基性岩脉成岩时代与岩石成因:锆石年代学、地球化学和Sr-Nd-Hf同位素约束

    曹亮 陈林 段其发 周云 刘重芃 张利国

    曹亮, 陈林, 段其发, 周云, 刘重芃, 张利国, 2019. 扬子陆块北缘东河铂钯矿化超基性岩脉成岩时代与岩石成因:锆石年代学、地球化学和Sr-Nd-Hf同位素约束. 地球科学, 44(2): 366-386. doi: 10.3799/dqkx.2018.262
    引用本文: 曹亮, 陈林, 段其发, 周云, 刘重芃, 张利国, 2019. 扬子陆块北缘东河铂钯矿化超基性岩脉成岩时代与岩石成因:锆石年代学、地球化学和Sr-Nd-Hf同位素约束. 地球科学, 44(2): 366-386. doi: 10.3799/dqkx.2018.262
    Cao Liang, Chen Lin, Duan Qifa, Zhou Yun, Liu Chongpeng, Zhang Liguo, 2019. Geochronology and Petrogenesis of the Donghe Pt-Pd-Bearing Ultramafic Dykesin the Northern Margin of the Yangtze Block: Constraints from Zircon Geochronology, Geochemistry and Sr-Nd-Hf Isotpopes. Earth Science, 44(2): 366-386. doi: 10.3799/dqkx.2018.262
    Citation: Cao Liang, Chen Lin, Duan Qifa, Zhou Yun, Liu Chongpeng, Zhang Liguo, 2019. Geochronology and Petrogenesis of the Donghe Pt-Pd-Bearing Ultramafic Dykesin the Northern Margin of the Yangtze Block: Constraints from Zircon Geochronology, Geochemistry and Sr-Nd-Hf Isotpopes. Earth Science, 44(2): 366-386. doi: 10.3799/dqkx.2018.262

    扬子陆块北缘东河铂钯矿化超基性岩脉成岩时代与岩石成因:锆石年代学、地球化学和Sr-Nd-Hf同位素约束

    doi: 10.3799/dqkx.2018.262
    基金项目: 

    中国地质调查局扬子工程湘西-鄂西成矿带神农架-花垣地区地质矿产调查二级项目 DD20160029

    详细信息
      作者简介:

      曹亮(1982-), 男, 硕士研究生, 高级工程师, 从事矿床地质研究

    • 中图分类号: P581;P597

    Geochronology and Petrogenesis of the Donghe Pt-Pd-Bearing Ultramafic Dykesin the Northern Margin of the Yangtze Block: Constraints from Zircon Geochronology, Geochemistry and Sr-Nd-Hf Isotpopes

    • 摘要: 东河铂钯矿化超基性岩脉位于扬子陆块北缘房县东河地区,铂钯矿体产于超基性岩辉石岩脉中.LA-ICP-MS锆石U-Pb测年表明该超基性岩脉结晶侵位年龄为433.2±2.9 Ma,属于早志留世.地球化学特征上,岩石具有较低含量的SiO2(39.73%~47.46%,均值为41.41%)、中等偏低的Mg#(46.98~67.37)和高铝(11.25%~15.46%)的特征,整体上属于高铝质超基性岩类.微量和稀土元素方面,岩石具有较高的稀土总量、轻稀土富集和无明显的Eu正异常特征(∑REE=59.59×10-6~375.02×10-6,(LaN/YbN)=3.94~19.13,δEu=0.93~1.13),所有岩石富集Rb、Ba、Sr、Nb、Ti等元素,亏损K、Hf、P等元素,且具有显著不同于地壳的不相容元素组成.Sr、Nd、Hf同位素研究表明,东河超基性岩具有低的(87Sr/86Sr)i(0.703 26~0.704 15),正的εNdt)(4.37~5.27)和正的εHft)(7.29~10.26).综合研究表明:东河超基性岩来自亏损的岩石圈地幔源区,可能有富集岩石圈地幔组分的加入,原始岩浆在上升侵位过程中地壳物质的混染不明显.微量元素构造环境判别显示其形成于板内构造环境,通过分析表明东河地区在早志留世应处于被动大陆边缘,拉张伸展的状态,研究区出露的两期超基性岩床(脉)为岩石圈处于拉张状态下大陆裂谷早期阶段的产物.

       

    • 图  1  扬子地块与南秦岭造山带构造单元划分(a)及北大巴山地区基性火山岩分布(b)

      a.据董有浦等(2011); b.据邹先武等(2011); BKB.碧口地体;MCB.米仓山隆起;FPB.佛坪地体;WDB.武当地体;SNB.神农架地体;LMST.龙门山冲断褶皱带;MCT.米仓山冲断褶皱带:DBT.大巴山冲断褶皱带;CDT.川东冲断褶皱带;MLS.勉略缝合带;SDS.商丹缝合带;1.褶皱带;2.缝合线;3.冲断层;4.刚性地体;5.造山带;6.研究区; 7.扬子陆块区;8.扬子陆块北部陆缘区;9.前寒武隆起区;10.苦橄榄-碱性玄武岩;11.基性岩脉(墙);12.粗面岩;13.石英闪长岩;14.断层

      Fig.  1.  Sketch map of tectonic units of the South Qinling orogen and Yangtze block

      图  2  房县东河铂钯矿野外露头

      下部深色部分为辉石岩

      Fig.  2.  Fangxian Donghe platinum palladium fied outcrop

      图  3  扬子陆块北缘房县东河地区地质简图

      1.第四系;2.下第三系-白垩系;3.下寒武统-下志留统;4.志留系;5.辉绿玢岩;6.辉石岩;7.奥陶系;8.寒武系;9.武当群;10.逆断层;11.研究区;12.铂钯矿及取样位置

      Fig.  3.  Figure of geology Fangxian Donghe in northern margin of Yangtze platform

      图  4  东河超基性岩岩石标本及岩石镜下特征照片

      a.灰绿色块状构造变辉石岩;b.灰绿色含黄铁矿矿化块状构造角闪辉石岩;c.灰绿色块状角闪辉石岩;d.辉石式解理及简单双晶;e.不规则粒状角闪石,少量钛铁矿、磁铁矿;f.针状透闪石交代角闪石及辉石;g.透辉石、角闪石、绿帘石及绿泥石等沿边缘及裂隙交代普通辉石;h.棕褐色不规则粒状角闪石沿辉石、透辉石边缘及裂隙交代;i.发育聚片双晶结构的斜长石;j.辉石式解理及简单双晶;k.棕褐色不规则粒状角闪石沿辉石、透辉石边缘及裂隙交代,呈残余结构;l.不规则粒状斜长石被绿帘石、黝帘石及绿泥石等交代强烈呈假象结构; Aug.普通辉石;HbI.普通角闪石;PI.斜长石;Ab.钠长石;Di.透辉石;Mt.磁铁矿;Ilm.钛铁矿;Chl.绿泥石;Zo.黝帘石;Ep.绿帘石

      Fig.  4.  Rocks sample photographs and microphotographs of rocks of the ultramafic rocks in Donghe area

      图  5  扬子陆块北缘东河超基性岩锆石的CL图像和U-Pb年龄分析点(实线圆圈)及Lu-Hf同位素分析点(虚线圆圈)

      Fig.  5.  CL images of zircons from the Donghe ultramafic rocks in northern margin of Yangtze platform and the points for U-Pb analysis (the solid circles) and Lu-Hf isotope analysis (dashed circles)

      图  6  超基性岩锆石U-Pb谐和图(a)和加权平均年龄图(b)

      Fig.  6.  Zircon U-Pb concordia diagram (a) and weighted average age (b) for ultramafic rocks

      图  7  扬子陆块北缘东河超基性岩TAS分类图解

      Middlemost(1994); 镇坪辉绿岩数据来源于邹先武等(2011);北大巴碱性岩墙群数据来源于张成立等(2002);北大巴基性岩墙群数据来源于王存智等(2009);兰家畈基性火山岩数据来源于董云鹏等(1998)

      Fig.  7.  TAS nomination diagram for rock classification from the Donghe ultramafic rocks in northern margin of Yangtze platform

      图  8  东河超基性岩脉的球粒陨石标准化稀土配分图(a)和原始地幔标准化微量元素分布图(b)

      标准化值据Sun and McDonough(1989)

      Fig.  8.  Chondrite-normalized REE abundances (a) and primitive mantle-normalized trace element abundances (b) of the Donghe ultramafic rocks

      图  9  东河超基性岩(87Sr/86Sr)i-εNd(t)图解

      其中数字表示地壳物质参与的比例,计算采用的参数Nd(10-6)、εNd(t)、Sr(10-6)、(87Sr/86Sr)i值如下:软流圈地幔(DM)分别为1.2、+8、20和0.703;玄武岩分别为15、+8、200和0.704;上地壳(UCC)分别为30、-12、250和0.740,据Jahn et al.(2000);下地壳(LCC)分别为20、-15、230和0.708,据Wu et al.(2000)

      Fig.  9.  (87Sr/86Sr)i vs.εNd(t) diagram for the Donghe ultramafic rocks

      图  10  东河超基型脉岩锆石Hf同位素特征

      Fig.  10.  Zircon Hf isotopic features of the Donghe ultramafic dyke

      图  11  东河超基性岩143Nd/144Nd对87Sr/86Sr相关图解

      DM.亏损地幔,EMⅠ、EMⅡ.富集地幔,据Zindler and Hart(1986)

      Fig.  11.  143Nd/144Nd vs. 87Sr/86Sr plot for the Donghe ultramafic rocks

      图  12  东河超基性岩脉Th/Yb-Nb/Yb(a)、Ba/Th-TH/Nb(b)和Nb/Zr-Th/Zr(c)图解

      a.据Pearce(2008); b.据Hanyu et al.(2006); c.据Woodhead et al.(2001)

      Fig.  12.  Th/Yb-Nb/Yb (a), Ba/Th-TH/Nb (b) and Nb/Zr-Th/Zr (c) diagrams of the Donghe ultramafic rocks

      图  13  东河超基性岩脉构造环境判别图

      a.据Pearce(1979); b.据Wood(1979); c.据Meschede(1986); d.据Nisbet et al.(1977)

      Fig.  13.  Discrimination diagrams of tectonic settings for the Donghe ultramafic rocks

      表  2  东河超基性岩元素地球化学组成(主量元素:%;微量元素:10-6)

      Table  2.   Element compositions of the Donghe ultramafic rocks (major element: %; trace element: 10-6)

      样品编号 DH-B3 DH-B4 DH-B5 DH-B8 DH-B11 DH-B13 DH-B14 DH-B15 DH-B16 DH-B17
      样品名称 蚀变
      辉石岩
      蚀变
      辉石岩
      含长
      辉石岩
      角闪
      辉石岩
      蚀变
      辉石岩
      蚀变
      辉石岩
      蚀变
      辉石岩
      蚀变
      辉石岩
      蚀变
      辉石岩
      蚀变
      辉石岩
      SiO2 43.86 42.21 47.46 40.81 40.07 41.09 38.93 40.59 39.73 39.37
      Al2O3 4.55 8.90 7.05 8.47 11.09 14.40 9.80 11.25 15.46 11.38
      Fe2O3 7.32 8.10 4.79 7.74 8.21 9.03 10.08 5.92 11.86 10.52
      FeO 9.07 8.11 6.25 9.82 9.09 4.97 8.64 10.32 2.22 7.62
      CaO 12.77 13.44 17.06 12.82 13.41 16.58 14.40 11.70 20.59 12.38
      MgO 16.24 10.14 12.23 12.77 8.69 5.92 8.71 9.01 8.56 8.49
      K2O 0.093 0.652 0.202 0.455 0.887 0.377 0.190 0.295 0.088 1.30
      Na2O 0.391 1.54 1.18 0.593 1.32 1.33 0.491 2.00 0.880 1.18
      TiO2 3.62 4.24 2.20 4.12 4.73 3.28 6.33 5.26 3.70 4.05
      P2O5 0.054 0.238 0.189 0.066 0.621 1.04 0.041 0.723 0.780 0.614
      MnO 0.186 0.171 0.174 0.215 0.225 0.101 0.166 0.249 0.063 0.176
      LOI 1.98 2.70 1.33 2.20 1.39 2.22 2.34 2.11 2.41 2.36
      Total 98.69 98.79 99.02 98.62 98.62 99.03 98.71 98.60 99.27 98.75
      Na2O/K2O 4.20 2.36 5.84 1.30 1.49 3.53 2.58 6.78 10.00 0.91
      Mg# 64.90 54.00 67.37 57.56 48.46 54.36 50.20 50.66 50.06 46.98
      La 6.42 26.6 15.5 10.0 22.6 47.1 9.92 20.9 77.6 36.2
      Ce 19.7 66.9 43.0 27.6 60.0 118 20.8 56.5 157 74.0
      Pr 2.80 8.01 5.78 3.70 7.60 14.0 2.74 7.67 16.8 8.90
      Nd 14.6 36.3 28.8 18.5 36.6 64.1 14.2 38.8 71.0 42.4
      Sm 3.96 8.13 7.18 4.65 8.36 13.8 3.94 9.23 14.3 9.67
      Eu 1.22 2.34 2.23 1.59 2.69 4.54 1.34 3.23 4.80 3.03
      Gd 3.52 7.00 6.28 4.13 7.32 12.1 3.60 7.95 12.5 8.41
      Tb 0.58 1.08 1.01 0.68 1.12 1.80 0.60 1.22 1.86 1.30
      Dy 3.36 5.74 5.71 3.78 6.13 9.54 3.35 6.51 9.72 7.12
      Ho 0.60 1.01 1.02 0.68 1.07 1.67 0.58 1.13 1.68 1.26
      Er 1.40 2.36 2.39 1.57 2.45 3.83 1.34 2.61 4.00 2.93
      Tm 0.19 0.31 0.32 0.22 0.31 0.48 0.18 0.33 0.51 0.38
      Yb 1.10 1.77 1.92 1.29 1.78 2.68 1.00 1.89 2.91 2.17
      Lu 0.14 0.21 0.24 0.16 0.22 0.31 0.12 0.23 0.34 0.26
      Y 12.6 21.5 22.2 14.6 23.4 37.2 12.6 24.6 38.5 27.5
      ΣREE 59.59 167.76 121.38 78.55 158.25 293.95 63.71 158.20 375.02 198.03
      LREE 48.70 148.28 102.49 66.04 137.85 261.54 52.94 136.33 341.50 174.20
      HREE 10.89 19.48 18.89 12.51 20.40 32.41 10.77 21.87 33.52 23.83
      LREE/HREE 4.47 7.61 5.43 5.28 6.76 8.07 4.92 6.23 10.19 7.31
      LaN/YbN 3.94 10.16 5.46 5.24 8.58 11.88 6.70 7.47 18.02 11.27
      δEu 0.98 0.93 0.99 1.09 1.03 1.05 1.07 1.13 1.07 1.00
      δCe 1.09 1.07 1.06 1.06 1.07 1.07 0.92 1.05 0.98 0.95
      Pb 1.91 6.30 6.70 2.95 7.80 12.5 8.02 3.31 15.5 13.6
      Cr 1 050 413 819 570 144 21.8 9.77 180 22.5 212
      Ni 534 234 189 359 196 50.2 178 185 50.1 219
      Co 95.8 94.8 60.2 93.2 77.9 92.7 52.3 77.7 166 74.7
      Rb 4.12 18.0 5.65 12.1 21.3 8.57 5.50 7.87 3.05 39.8
      Sr 624 521 550 410 837 2 290 1 120 806 3 820 1 300
      Ba 51.5 76.8 145 46.9 28.6 24.3 30.2 59.9 26.4 36.2
      V 350 451 324 438 540 516 620 417 499 462
      Sc 61.8 55.9 73.3 56.8 58.4 26.8 56.1 40.7 22.5 39.5
      Nb 14.6 32.6 10.2 16.2 25.3 47.6 22.8 35.2 83.6 36.9
      Ta 0.21 1.24 0.50 0.36 0.77 1.84 0.90 1.69 4.19 1.48
      Zr 87.1 193 113 119 127 213 114 102 351 138
      Hf 1.98 4.94 3.24 3.03 3.50 5.10 3.13 2.61 9.30 3.72
      U 0.10 0.62 0.11 0.18 0.20 0.79 0.14 0.14 2.30 0.43
      Th 0.86 2.31 0.94 1.36 1.29 3.52 0.80 0.82 7.95 1.12
      下载: 导出CSV

      表  3  东河地区超基性岩锆石原位Hf同位素组成

      Table  3.   Zircon Lu-Hf isotopic compositions of the Donghe ultramafic rocks

      点号 176Yb/177Hf 176Lu/177Hf 176Hf/177Hf 年龄(Ma) (176Hf/177Hf)i εHf(0) εHf(t) fLu/Hf tDM t2DM
      DH1-1 0.015 200 0.000 413 0.282 748 0.000 014 430 0.282 745 -0.85 8.52 -0.99 703 873
      DH1-2 0.012 661 0.000 364 0.282 775 0.000 017 421 0.282 737 -1.17 8.03 -0.99 714 898
      DH1-3 0.037 026 0.001 121 0.282 761 0.000 034 447 0.282 760 -0.28 9.42 -0.98 683 829
      DH1-4 0.032 398 0.000 885 0.282 756 0.000 017 434 0.282 778 0.35 9.77 -0.99 656 794
      DH1-5 0.027 753 0.000 773 0.282 755 0.000 019 436 0.282 761 -0.18 9.22 -0.98 682 833
      DH1-6 0.027 525 0.000 733 0.282 751 0.000 016 426 0.282 744 -0.71 8.39 -0.97 708 877
      DH1-7 0.019 274 0.000 530 0.282 753 0.000 016 433 0.282 706 -2.12 7.20 -0.98 759 958
      DH1-8 0.022 381 0.000 621 0.282 796 0.000 020 442 0.282 782 0.50 10.09 -0.98 652 782
      DH1-9 0.019 556 0.000 540 0.282 741 0.000 016 427 0.282 781 0.46 9.72 -0.98 654 794
      DH1-10 0.028 259 0.000 765 0.282 735 0.000 018 435 0.282 772 0.11 9.58 -0.99 665 809
      DH1-11 0.017 352 0.000 474 0.282 776 0.000 015 423 0.282 752 -0.39 8.61 -0.97 698 861
      DH1-12 0.010 994 0.000 321 0.282 739 0.000 016 441 0.282 749 -0.57 8.90 -0.97 701 858
      DH1-13 0.022 548 0.000 619 0.282 712 0.000 015 435 0.282 749 -0.60 8.77 -0.98 700 861
      DH1-14 0.019 478 0.000 535 0.282 764 0.000 016 489 0.282 744 -0.74 9.79 -0.98 705 837
      DH1-15 0.016 175 0.000 447 0.282 782 0.000 016 441 0.282 749 -0.67 8.90 -0.98 698 857
      DH1-16 0.024 815 0.000 683 0.282 767 0.000 016 427 0.282 791 0.85 10.08 -0.98 640 771
      DH1-17 0.036 630 0.000 999 0.282 752 0.000 016 430 0.282 737 -1.10 8.23 -0.98 715 891
      DH1-18 0.025 703 0.000 689 0.282 712 0.000 016 441 0.282 729 -1.31 8.19 -0.98 728 903
      DH1-19 0.019 464 0.000 528 0.282 786 0.000 018 430 0.282 772 0.14 9.47 -0.99 665 811
      DH1-20 0.020 349 0.000 563 0.282 785 0.000 015 432 0.282 707 -2.12 7.22 -0.98 757 957
      下载: 导出CSV

      表  4  东河超基性岩脉全岩Sr-Nd同位素组成

      Table  4.   Whole-rock isotope compositions of the Donghe ultramafic rocks

      样品号 Rb(10-6) Sr (10-6) 87Rb/86Sr 87Sr/86Sr (87Sr/86Sr)i εSr(t) Sm(10-6) Nd(10-6) 147Sm/ 144Nd 143Nd/ 144Nd εNd(t) INd fSm/Nd tDM(Ga) t2DM(Ga)
      DH-B3 1.574 52.14 0.087 010 0.703 88 5 0.703 34 -9.2 3.781 14.03 0.163 0 0.512 782 4.68 0.512 320 -0.17 1.111 0.792
      DH-B4 18.170 471.30 0.111 100 0.704 22 3 0.703 53 -6.5 7.820 35.28 0.134 1 0.512 705 4.78 0.512 325 -0.32 0.855 0.784
      DH-B5 4.454 486.90 0.026 370 0.704 02 5 0.703 86 -1.9 6.866 27.99 0.148 4 0.512 760 5.05 0.512 339 -0.25 0.914 0.761
      DH-B8 12.670 368.00 0.099 180 0.703 87 3 0.703 26 -10.4 4.404 17.53 0.152 0 0.512 755 4.76 0.512 324 -0.23 0.980 0.785
      DH-B11 4.512 1 006.00 0.012 920 0.704 23 7 0.704 15 2.3 3.780 13.90 0.164 5 0.512 813 5.21 0.512 347 -0.16 1.050 0.749
      DH-B13 7.335 703.20 0.030 060 0.703 71 2 0.703 52 -6.7 8.882 37.71 0.142 5 0.512 713 4.47 0.512 309 -0.28 0.939 0.809
      DH-B14 21.550 720.40 0.086 190 0.704 17 4 0.703 64 -5.0 8.193 36.16 0.137 1 0.512 718 4.86 0.512 329 -0.30 0.863 0.777
      DH-B15 6.942 2 148.00 0.009 312 0.704 04 2 0.703 98 -0.1 13.780 65.28 0.127 7 0.512 696 4.96 0.512 334 -0.35 0.808 0.770
      DH-B16 2.164 2 945.00 0.002 117 0.704 06 3 0.704 05 0.9 14.550 73.34 0.120 0 0.512 690 5.27 0.512 350 -0.39 0.751 0.744
      DH-B17 43.320 1 207.00 0.103 400 0.704 40 1 0.703 76 -3.3 9.849 43.50 0.137 0 0.512 692 4.37 0.512 304 -0.30 0.914 0.818
      下载: 导出CSV
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