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    相山西部牛头山铅锌矿化体成矿物质来源:原位硫同位素的制约

    刘斌 陈卫锋 方启春 唐湘生 毛玉锋 孙立强 高爽 严永杰 魏欣 凌洪飞

    刘斌, 陈卫锋, 方启春, 唐湘生, 毛玉锋, 孙立强, 高爽, 严永杰, 魏欣, 凌洪飞, 2020. 相山西部牛头山铅锌矿化体成矿物质来源:原位硫同位素的制约. 地球科学, 45(2): 389-399. doi: 10.3799/dqkx.2018.395
    引用本文: 刘斌, 陈卫锋, 方启春, 唐湘生, 毛玉锋, 孙立强, 高爽, 严永杰, 魏欣, 凌洪飞, 2020. 相山西部牛头山铅锌矿化体成矿物质来源:原位硫同位素的制约. 地球科学, 45(2): 389-399. doi: 10.3799/dqkx.2018.395
    Liu Bin, Chen Weifeng, Fang Qichun, Tang Xiangsheng, Mao Yufeng, Sun Liqiang, Gao Shuang, Yan Yongjie, Wei Xin, Ling Hongfei, 2020. Study on In-Situ Sulfur Isotope Compositions of Sulfides: Implication for the Source of Pb-Zn Mineralized Body of Niutoushan in the Xiangshan Area. Earth Science, 45(2): 389-399. doi: 10.3799/dqkx.2018.395
    Citation: Liu Bin, Chen Weifeng, Fang Qichun, Tang Xiangsheng, Mao Yufeng, Sun Liqiang, Gao Shuang, Yan Yongjie, Wei Xin, Ling Hongfei, 2020. Study on In-Situ Sulfur Isotope Compositions of Sulfides: Implication for the Source of Pb-Zn Mineralized Body of Niutoushan in the Xiangshan Area. Earth Science, 45(2): 389-399. doi: 10.3799/dqkx.2018.395

    相山西部牛头山铅锌矿化体成矿物质来源:原位硫同位素的制约

    doi: 10.3799/dqkx.2018.395
    基金项目: 

    国家重点研发计划项目"深地资源勘查开采"专项 2017YFC0602601

    核工业地质局科研项目 201631

    详细信息
      作者简介:

      刘斌(1991-), 男, 硕士生, 主要从事铀矿床地球化学方面的研究

      通讯作者:

      凌洪飞

    • 中图分类号: P611

    Study on In-Situ Sulfur Isotope Compositions of Sulfides: Implication for the Source of Pb-Zn Mineralized Body of Niutoushan in the Xiangshan Area

    • 摘要: 近年来,在相山铀矿田的西部牛头山地区深部发现了铅锌矿化体,其成因机制不明.为探讨牛头山铅锌矿化体物质来源,开展了硫化物原位硫同位素分析研究.根据硫化物矿物之间的充填和包裹关系判断,铅锌矿化体金属硫化物形成的先后顺序是:黄铁矿形成最早,方铅矿和闪锌矿次之,细脉状黄铜矿形成最晚.利用LA-MC-ICP-MS技术对矿化体中几种金属硫化物分别进行了系统的原位硫同位素分析.结果显示:黄铁矿、闪锌矿、方铅矿、细脉状黄铜矿的δ34S值介于-4.8‰~+5.4‰之间,各硫化物矿物之间硫同位素未达到完全平衡分馏,利用黄铁矿δ34S值得到的矿化流体δ34SΣS值(总硫同位素组成)近似为+3.7‰,与共生矿物对(闪锌矿-方铅矿)图解法得到的闪锌矿和方铅矿沉淀时矿化流体的δ34SΣS值(+3.2‰)相近,表明形成牛头山铅锌矿化体的矿化流体δ34SΣS值大约为+3.7‰,为岩浆硫.结合前人的岩浆岩年龄数据,我们判断该铅锌矿化体金属硫化物的硫可能主要来自次火山岩相花岗斑岩岩浆热液.同一薄片中闪锌矿δ34S值高于共生的方铅矿,表明两者硫同位素基本平衡,利用共生矿物对(闪锌矿-方铅矿)硫同位素温度计计算得出平衡温度为197~476℃,与前人通过脉石矿物流体包裹体得到的铅锌矿化流体温度基本一致.相山火山盆地与相邻的北武夷黄岗山、梨子坑等产铅锌矿的火山盆地具有相似的成矿条件及成矿物质来源,使相山火山盆地具有良好的铅锌多金属找矿前景.

       

    • 图  1  相山铀矿田地质简图(据谢国发等,2014修改)

      图中方框为钻探剖面(图 2)所在区

      Fig.  1.  Simplified geologic map of the Xiangshan uranium ore field

      图  2  牛头山26线矿体剖面图(据吴志坚和胡志华,2014修改)

      Fig.  2.  Cross-section of ore body found in exploration line No.26 in Niutoushan Pb-Zn mineralization

      图  3  牛头山铅锌矿化体中主要金属硫化物的分布和结构关系(手标本a-c、显微镜照片d-i)

      图中圆圈代表原位硫同位素测点位置;a.黄铁矿;b.块状矿石;c.块状矿石;d.乳滴状黄铜矿与闪锌矿呈“固溶体”出溶结构;e.细脉状黄铜矿充填闪锌矿解理面中;f.方铅矿与闪锌矿紧密共生;;g.闪锌矿交代黄铁矿;h.方铅矿充填交代黄铁矿;i.黄铜矿包裹方铅矿;Py.黄铁矿;Gn.方铅矿;Sp.闪锌矿;Cp.黄铜矿;Apy.毒砂;Sd.菱铁矿;Q.石英.

      Fig.  3.  Distribution and structure of sulfide minerals from the Niutoushan Pb-Zn mineralization

      图  5  牛头山铅锌矿化体硫同位素组成直方图

      Fig.  5.  Histogram of the δ34Svalues of sulfide minerals from the Niutoushan Pb-Zn mineralization

      图  4  牛头山铅锌矿化体δ34SΣS Pinckney法图解

      Sp.闪锌矿,Gn.方铅矿

      Fig.  4.  The Pinckney method of δ34SΣS from the Niutoushan Pb-Zn mineralization

      表  1  牛头山铅锌矿化体金属硫化物硫同位素组成(‰)

      Table  1.   The sulfur isotope compositions of sulfide minerals from the Pb-Zn mineralization (‰)

      序号 样品编号 采样位置(m) 样品类型 测试矿物 δ34S(‰)
      1 ZK26-101-2-1 -1 045 细脉状矿石 黄铁矿 +5.3
      2 ZK26-101-2-1 -1 045 细脉状矿石 闪锌矿 +3.5
      3 ZK26-101-2-2 -1 045 细脉状矿石 方铅矿 -0.2
      4 ZK26-101-2-4 -1 045 细脉状矿石 黄铁矿 +3.6
      5 ZK26-101-2-5 -1 045 细脉状矿石 闪锌矿 +3.8
      6 ZK26-101-2-5 -1 045 细脉状矿石 方铅矿 +1.7
      7 ZK26-101-4-1 -1 051 细脉状矿石 黄铁矿 +4.0
      8 ZK26-101-4-1 -1 051 细脉状矿石 方铅矿 -1.7
      9 ZK26-101-4-2 -1 051 细脉状矿石 黄铁矿 +5.3
      10 ZK26-101-4-3 -1 051 细脉状矿石 黄铁矿 +4.5
      11 ZK26-101-4-4 -1 051 细脉状矿石 闪锌矿 +4.0
      12 ZK26-101-12-1-A -1 074 块状矿石 黄铁矿 +4.0
      13 ZK26-101-12-1-B -1 074 块状矿石 黄铁矿 +3.7
      14 ZK26-101-12-2 -1 074 块状矿石 黄铁矿 +3.9
      15 ZK26-101-12-3 -1 074 块状矿石 黄铁矿 +4.0
      17 ZK26-101-12-5 -1 074 块状矿石 黄铁矿 +3.8
      18 ZK26-101-14-1 -1 077 块状矿石 方铅矿 +3.9
      19 ZK26-101-14-1 -1 077 块状矿石 细脉状黄铜矿 -4.8
      20 ZK26-101-14-2 -1 077 块状矿石 闪锌矿 +3.9
      21 ZK26-101-14-2 -1 077 块状矿石 方铅矿 +2.6
      22 ZK26-101-14-2 -1 077 块状矿石 细脉状黄铜矿 -0.9
      23 ZK26-101-14-2 -1 077 块状矿石 闪锌矿 +5.4
      24 ZK26-101-14-3 -1 077 块状矿石 黄铁矿 +3.3
      25 ZK26-101-14-3 -1 077 块状矿石 细脉状黄铜矿 -3.8
      26 ZK26-101-14-4 -1 077 块状矿石 细脉状黄铜矿 +1.9
      27 ZK26-101-14-4 -1 077 块状矿石 闪锌矿 +3.5
      28 ZK26-101-14-4 -1 077 块状矿石 方铅矿 +2.5
      29 ZK26-101-15-1 -1 078 块状矿石 黄铁矿 +3.6
      30 ZK26-101-15-2 -1 078 块状矿石 黄铁矿 +3.7
      31 ZK26-101-15-2 -1 078 块状矿石 方铅矿 +0.1
      32 ZK26-101-15-3 -1 078 块状矿石 闪锌矿 +3.4
      33 ZK26-101-15-3 -1 078 块状矿石 细脉状黄铜矿 +1.4
      34 ZK26-101-15-4 -1 078 块状矿石 闪锌矿 +3.7
      35 ZK26-101-15-4 -1 078 块状矿石 细脉状黄铜矿 +2.6
      36 ZK26-101-15-5 -1 078 块状矿石 黄铁矿 +3.6
      37 ZK26-101-17-1 -1 080 块状矿石 黄铁矿 +4.4
      38 ZK26-101-17-2 -1 080 块状矿石 细脉状黄铜矿 +2.0
      39 ZK26-101-17-3 -1 080 块状矿石 方铅矿 +0.9
      40 ZK26-101-17-3 -1 080 块状矿石 闪锌矿 +4.2
      41 ZK26-101-17-4 -1 080 块状矿石 细脉状黄铜矿 +3.3
      下载: 导出CSV

      表  2  牛头山铅锌矿化体硫同位素地质温度

      Table  2.   Sulfur isotope geo-thermometer of sulfide from the Niutoushan Pb-Zn mineralization

      样品编号 岩性 Sp(‰) Gn(‰) △Sp-Gn 平衡温度(℃)
      ZK26-101-2-5 细脉状矿石 3.8 1.7 2.1 316
      ZK-26-101-14-2 块状矿石 3.9 2.6 1.3 476
      ZK-26-101-14-2 块状矿石 5.4 2.5 2.9 229
      ZK-26-101-17-3 块状矿石 4.2 0.9 3.3 197
      下载: 导出CSV

      表  3  牛头山、生米坑及蔡家坪铅锌矿床基本特征

      Table  3.   Typical characteristics of Niutoushan, Lengshuikeng and shengminkeng Pb-Zn deposits

      矿床 牛头山 生米坑 蔡家坪
      岩性 流纹英安岩 粗面斑岩 流纹斑岩
      岩石类型 S型
      稀土模式 轻重稀土分异明显,轻稀土富集,Eu负异常
      成岩年龄 135 Ma 138 Ma 137 Ma
      成矿年龄 121 Ma 135 Ma 135 Ma
      成矿温度 197~476℃ 302~558℃ 292~490℃
      成矿物质来源(S同位素) 岩浆热液 岩浆热液 岩浆热液
      注:牛头山成岩成矿数据引自:杨水源等(2010);成矿年龄数据与刘军港讨论获得;生米坑数据引自:罗平等(2009)张家箐等(2012);蔡家坪数据引自:代堰锫等(2011)徐庆胜等(2014).
      下载: 导出CSV
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