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    纳米颗粒物:独具特性的地球化学组成

    杨毅 周立旻 钭斐昀 孙笑丽 刘敏 MichaelF. Hochella Jr.

    杨毅, 周立旻, 钭斐昀, 孙笑丽, 刘敏, MichaelF. Hochella Jr., 2018. 纳米颗粒物:独具特性的地球化学组成. 地球科学, 43(5): 1489-1502. doi: 10.3799/dqkx.2018.408
    引用本文: 杨毅, 周立旻, 钭斐昀, 孙笑丽, 刘敏, MichaelF. Hochella Jr., 2018. 纳米颗粒物:独具特性的地球化学组成. 地球科学, 43(5): 1489-1502. doi: 10.3799/dqkx.2018.408
    Yang Yi, Zhou Limin, Tou Feiyun, Sun Xiaoli, Liu Min, Michael F. Hochella Jr., 2018. Nanoparticle: A Unique Geochemical Composition in Environment. Earth Science, 43(5): 1489-1502. doi: 10.3799/dqkx.2018.408
    Citation: Yang Yi, Zhou Limin, Tou Feiyun, Sun Xiaoli, Liu Min, Michael F. Hochella Jr., 2018. Nanoparticle: A Unique Geochemical Composition in Environment. Earth Science, 43(5): 1489-1502. doi: 10.3799/dqkx.2018.408

    纳米颗粒物:独具特性的地球化学组成

    doi: 10.3799/dqkx.2018.408
    基金项目: 

    国家自然科学基金项目 41771506

    国家自然科学基金项目 41522111

    详细信息
      作者简介:

      杨毅(1979-), 女, 教授, 博士, 从事环境中纳米颗粒物的鉴别与行为研究

    • 中图分类号: P95

    Nanoparticle: A Unique Geochemical Composition in Environment

    • 摘要: 至少一维尺度上小于100 nm的颗粒物均称为纳米颗粒物,在人工纳米颗粒物产生的几十亿年前,地球已经通过其特有的生物地球化学过程合成各类天然纳米颗粒物.这些纳米颗粒物及其次生产物具有独特的理化特性,并参与各种地球化学过程,体现其非凡的地球化学意义.从地球化学的角度,解析了环境纳米颗粒物的定义和分类,重点阐述了风化壳与水体中天然和次生纳米颗粒物的形成,并在天然纳米颗粒物中区分了纳米矿物和矿物纳米颗粒物;同时,也讨论了大气纳米颗粒物的来源、成因与环境影响.该综述列举了目前环境中纳米颗粒物表征与鉴别的技术和方法,重点剖析了纳米颗粒物的地球化学功能和环境意义,并对该领域的研究前沿问题进行了概述.

       

    • 图  1  某发电厂煤灰中的Magnéli相氧化钛颗粒

      Yang et al.(2017).a.TEM图; b.高分辨TEM图,显示其超细的纹理条带; c.相应的电子衍射图

      Fig.  1.  Magnéli phase of Ti oxides in coal ash from a coal power plant

      图  2  煤灰蓄存池废水中的水合氧化铁SEM(a)和TEM图(b)

      Fig.  2.  SEM (a) and TEM (b) of ferrihydrite nanoparticles in a coal ash impoundment

      图  3  典型大气黑炭的SEM(a)、TEM(b)和高分辨率TEM(c)图

      高分辨TEM图显示其特有的类似洋葱结构

      Fig.  3.  SEM(a), TEM(b) and HR-TEM(c) images of soot particles

      图  4  某雾霾过程大气PM2.5中氧化铁(a)、富含Fe/Cr/Ni的纳米颗粒物(b)和氧化铝(c)纳米颗粒物团聚体的TEM图

      Fig.  4.  TEM images of Fe oxide (a), Fe/Cr/Ni enriched nanoparticles (b) and Al oxide (c) aggregations in PM2.5

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    • 收稿日期:  2017-10-27
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