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    大气颗粒物理化特征和影响效应的研究进展及展望

    邵龙义 王文华 幸娇萍 李卫军 牛红亚 侯聪 杨书申

    邵龙义, 王文华, 幸娇萍, 李卫军, 牛红亚, 侯聪, 杨书申, 2018. 大气颗粒物理化特征和影响效应的研究进展及展望. 地球科学, 43(5): 1691-1708. doi: 10.3799/dqkx.2018.422
    引用本文: 邵龙义, 王文华, 幸娇萍, 李卫军, 牛红亚, 侯聪, 杨书申, 2018. 大气颗粒物理化特征和影响效应的研究进展及展望. 地球科学, 43(5): 1691-1708. doi: 10.3799/dqkx.2018.422
    Shao Longyi, Wang Wenhua, Xing Jiaoping, Li Weijun, Niu Hongya, Hou Cong, Yang Shushen, 2018. Physicochemical Characteristics and Effects of Airborne Particles: Research Progress and Prospects. Earth Science, 43(5): 1691-1708. doi: 10.3799/dqkx.2018.422
    Citation: Shao Longyi, Wang Wenhua, Xing Jiaoping, Li Weijun, Niu Hongya, Hou Cong, Yang Shushen, 2018. Physicochemical Characteristics and Effects of Airborne Particles: Research Progress and Prospects. Earth Science, 43(5): 1691-1708. doi: 10.3799/dqkx.2018.422

    大气颗粒物理化特征和影响效应的研究进展及展望

    doi: 10.3799/dqkx.2018.422
    基金项目: 

    国家重点基础研究发展计划(973计划)项目 2013CB228503

    河北省自然科学基金项目 D2016402120

    国家自然科学基金项目 41571130031

    国家自然科学基金项目 41375145

    详细信息
      作者简介:

      邵龙义(1964-), 男, 教授, 主要从事沉积学和大气环境研究工作

    • 中图分类号: P57

    Physicochemical Characteristics and Effects of Airborne Particles: Research Progress and Prospects

    • 摘要: 大气颗粒物,尤其是细颗粒物PM2.5,是有毒和有害物质的载体,对人体健康具有重要的影响,同时大气颗粒物具有吸湿性、光学吸收和散射能力以及云凝结核活性等,对环境和气候变化具有重要的作用,大气颗粒物进一步的长距离输送还会对区域和全球地球化学循环产生重要影响.总结了当前大气颗粒物的物理化学特征研究进展,分析了离线和在线分析技术在大气颗粒物主要组分检测中的应用,阐述了大气颗粒物源解析技术的应用现状,以及由于大气颗粒物污染对环境、气候、人体健康和地球化学循环等产生的影响,最后展望未来大气颗粒物研究的重点问题.

       

    • 图  1  2000—2015年北京市PM2.5质量浓度季节变化特征

      Lang et al.(2017)

      Fig.  1.  Seasonal variations of PM2.5 mass concentrations in Beijing during 2000—2015

      图  2  透射电镜下大气颗粒物的单颗粒类型和混合状态

      a.NaCl颗粒和矿物颗粒的混合;b.飞灰集合体;c.金属Fe和硫酸盐形成的核壳结构;d.生物质颗粒;e.矿物颗粒和烟尘集合体的混合;f.烟尘集合体和硫酸盐的混合;g.硫酸盐和有机质等形成的核壳结构;h.硫酸盐和有机质混合,据Shao et al.(2017a)

      Fig.  2.  Morphologies and mixing states of individual particles in TEM images

      图  3  2013年1月重污染期间不同污染源对PM2.5的贡献(%)

      Huang et al.(2014)

      Fig.  3.  Source apportionment of PM2.5 during haze pollution in January, 2013

      图  4  入射太阳辐射的气溶胶及云的反射和吸收

      Bates et al.(2006)

      Fig.  4.  Optical reflection and absorption of aerosol and cloud under incoming solar radiation

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