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    大别山金河桥超高压榴辉岩石榴石中的水

    蒋素会 王志民 陈仁旭 郑永飞 朱琳

    蒋素会, 王志民, 陈仁旭, 郑永飞, 朱琳, 2020. 大别山金河桥超高压榴辉岩石榴石中的水. 地球科学, 45(4): 1168-1186. doi: 10.3799/dqkx.2019.132
    引用本文: 蒋素会, 王志民, 陈仁旭, 郑永飞, 朱琳, 2020. 大别山金河桥超高压榴辉岩石榴石中的水. 地球科学, 45(4): 1168-1186. doi: 10.3799/dqkx.2019.132
    Jiang Suhui, Wang Zhimin, Chen Renxu, Zheng Yongfei, Zhu Lin, 2020. Water of Garnet in Eclogite from Jinheqiao Area in the Dabie Orogen. Earth Science, 45(4): 1168-1186. doi: 10.3799/dqkx.2019.132
    Citation: Jiang Suhui, Wang Zhimin, Chen Renxu, Zheng Yongfei, Zhu Lin, 2020. Water of Garnet in Eclogite from Jinheqiao Area in the Dabie Orogen. Earth Science, 45(4): 1168-1186. doi: 10.3799/dqkx.2019.132

    大别山金河桥超高压榴辉岩石榴石中的水

    doi: 10.3799/dqkx.2019.132
    基金项目: 

    中科院先导项目 XDB18020303

    国家自然科学基金项目 41590624

    国家自然科学基金项目 41873033

    详细信息
      作者简介:

      蒋素会(1993-), 女, 硕士研究生, 主要研究名义上无水矿物中水.E-mail:jshsx@mail.ustc.edu.cn

      通讯作者:

      陈仁旭(1981-)

    • 中图分类号: P595

    Water of Garnet in Eclogite from Jinheqiao Area in the Dabie Orogen

    • 摘要: 名义上无水矿物的水含量研究对于认识俯冲带流体活动和地球动力学具有重要意义.对大别山金河桥榴辉岩中石榴石进行了傅里叶变换红外光谱分析和主微量元素分析,结果表明石榴石含有分子水和结构羟基,分别为 < 1×10-6~1 946×10-6和< 1×10-6~1 347×10-6.石榴石羟基含量与Ca、Na、Ti、Zr和Pr正相关,而与Si负相关,表明羟基结合机制以水榴石替代为主并伴有其他机制.分子水主要为初始水或折返过程中羟基转化形成.石榴石总水含量为 < 1×10-6~3 293×10-6,最大值对应于峰期超高压石榴石水储存能力.水在峰期石榴石中可达到饱和.石榴石变化的水含量受原岩性质、流体可获得性、压力和温度等多种因素控制,但主要由折返过程中降压脱水导致.石榴石平均总水含量为749×10-6~1 164×10-6,是俯冲板片向地幔水传输的重要介质.

       

    • 图  1  大别山地质简图及采样位置

      Lin et al. (2009)Wei et al. (2013)修改

      Fig.  1.  Geological maps of Dabie orogen (a, b) and study area (c) with sample location

      图  2  金河桥榴辉岩野外露头照片

      a.块状榴辉岩;b.条带状榴辉岩

      Fig.  2.  Photos of Jinheqiao eclogite in the field

      图  3  金河桥榴辉岩岩相学照片

      a.样品16DB20;b.样品16DB25;c.样品16DB27-1;d.样品16DB27-4;e.样品16DB27-2;f.样品16DB27-7.Grt.石榴石;Omp.绿辉石;Qtz.石英;Ms.白云母;Zo.黝帘石;Rt.金红石;Amp.角闪石

      Fig.  3.  Petrographic photos of Jinheqiao eclogite

      图  4  金河桥榴辉岩中石榴石端员组分的三元图解

      Alm.铁铝榴石;Grs.钙铝榴石;Pyr.镁铝榴石;Sps.锰铝榴石;And.钙铁榴石

      Fig.  4.  End member components of garnet in Jinheqiao eclogite

      图  5  金河桥榴辉岩中石榴石稀土元素配分图解

      球粒陨石标准化值来自Sun and McDonough (1989)

      Fig.  5.  Chondrite-normalized REE patterns of garnets for Jinheqiao eclogite

      图  6  金河桥榴辉岩中石榴石代表性红外吸收光谱

      吸收度标准化到1 cm厚度

      Fig.  6.  Representative FTIR spectra of garnet in Jinheqiao eclogite

      图  7  金河桥榴辉岩石榴石M型水含量与I型羟基水含量相关性图解

      Fig.  7.  Relationship between contents of M-type H2O and I-type OH in garnet from Jinheqiao eclogite

      图  8  金河桥榴辉岩石榴石M型水含量与III型羟基水含量相关性图解

      Fig.  8.  Relationship between contents of M-type H2O and III-type OH in garnet from Jinheqiao eclogite

      图  9  金河桥榴辉岩石榴石M型水含量与羟基水含量相关性图解

      Fig.  9.  Contents of structural hydroxyl due to band type I, II and III, respectively, plotted against the amount of molecular water (M-type) in garnet from Jinheqiao eclogite

      图  10  金河桥榴辉岩石榴石不同种型水含量统计

      Fig.  10.  Histograms illustrating distribution and contents of different types of water in garnet from Jinheqiao eclogite

      图  11  石榴石水含量剖面

      Fig.  11.  The distribution of water content in the same garnet grains

      图  12  金河桥榴辉岩石榴石组成与水含量之间关系图解

      Fig.  12.  Relationship between composition and water content of garnet from Jinheqiao eclogite

      表  1  金河桥榴辉岩矿物含量(%)

      Table  1.   Contents of minerals in Jinheqiao eclogite(%)

      样品编号 构造 绿辉石 石榴石 白云母 石英 角闪石 金红石 帘石 锆石 磷灰石 后成合晶
      16DB20-1 块状 50 35 4 2 1 1 1 < 1 < 1 4
      16DB25-2 块状 58 27 2 5 1 1 0 < 1 < 1 4
      16DB27-1 块状 56 37 1 1 1 1 0 < 1 < 1 1
      16DB27-4 块状 50 37 1 2 3 1 0 < 1 < 1 4
      16DB27-2 条带状 35 54 2 3 2 1 0 < 1 < 1 1
      16DB27-7 条带状 20 54 1 20 1 1 0 < 1 < 1 1
      下载: 导出CSV

      表  2  金河桥榴辉岩石榴石代表性主量元素组成

      Table  2.   Representative garnet major element compositions for Jinheqiao eclogite

      Sample 16DB27-4 16DB27-2 16DB27-7
      Spot Grt3 Grt8 Grt19 Grt22 Grt26 Grt1 Grt13 Grt18 Grt22 Grt29 Grt1 Grt18 Grt24 Grt27 Grt39
      SiO2 39.30 38.94 40.05 38.68 38.17 39.02 38.77 38.67 38.87 39.36 40.04 38.74 39.55 39.40 38.98
      TiO2 0.01 0.00 0.00 0.02 0.01 0.01 0.00 0.03 0.05 0.00 0.03 0.04 0.00 0.02 0.00
      Al2O3 22.21 22.42 21.80 22.49 23.85 22.30 22.47 22.44 22.23 22.53 22.33 24.22 22.63 22.26 22.37
      Cr2O3 0.07 0.00 0.01 0.02 0.06 0.07 0.08 0.06 0.03 0.05 0.05 0.03 0.04 0.05 0.09
      FeO 19.23 18.93 19.56 18.59 17.54 20.13 18.97 19.88 18.75 19.45 18.99 18.95 19.91 18.91 20.79
      MnO 0.42 0.40 0.38 0.37 0.37 0.44 0.32 0.42 0.41 0.35 0.42 0.41 0.35 0.39 0.39
      MgO 7.93 8.81 9.41 9.20 8.95 9.18 8.27 8.52 9.15 9.56 9.56 9.73 10.21 10.73 9.46
      CaO 10.46 9.93 8.64 10.13 9.86 8.29 10.09 9.46 9.86 8.60 8.49 7.66 7.01 7.48 7.62
      Total 99.63 99.43 99.85 99.50 98.81 99.43 98.98 99.47 99.33 99.90 99.92 99.77 99.71 99.22 99.71
      Atom per 12 O
      Si 3.00 2.96 3.03 2.94 2.90 2.97 2.97 2.95 2.96 2.98 3.02 2.90 2.99 2.98 2.97
      Ti 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00
      Al iv 0.00 0.04 0.00 0.06 0.10 0.03 0.03 0.05 0.04 0.02 0.00 0.10 0.01 0.02 0.03
      Al vi 1.99 1.98 1.94 1.96 2.04 1.98 2.00 1.98 1.96 1.99 1.98 2.05 2.00 1.97 1.97
      Cr 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.01
      Fe2+ 1.22 1.19 1.21 1.15 1.17 1.27 1.22 1.25 1.16 1.22 1.20 1.26 1.26 1.17 1.30
      Fe3+ 0.00 0.02 0.03 0.03 0.00 0.01 0.00 0.02 0.03 0.01 0.00 0.00 0.00 0.02 0.02
      Mn 0.03 0.03 0.02 0.02 0.02 0.03 0.02 0.03 0.03 0.02 0.03 0.03 0.02 0.03 0.02
      Mg 0.90 1.00 1.06 1.04 1.01 1.04 0.94 0.97 1.04 1.08 1.07 1.09 1.15 1.21 1.07
      Ca 0.85 0.81 0.70 0.83 0.80 0.68 0.83 0.77 0.80 0.70 0.68 0.61 0.57 0.61 0.62
      Total 8.00 8.02 7.99 8.04 8.05 8.02 8.01 8.02 8.02 8.01 7.99 8.04 8.01 8.01 8.02
      Almandine 40.5 38.1 39.6 35.7 36.6 41.2 39.6 40.0 36.9 39.7 40.1 40.5 41.8 38.2 42.0
      Andradite 0.20 0.95 1.30 1.73 0.00 0.75 0.00 0.82 1.69 0.54 0.00 0.00 0.00 1.16 1.0
      Grossular 28.1 26.4 22.4 26.3 27.5 21.8 27.7 25.2 25.4 22.7 22.8 21.1 18.9 19.0 19.7
      Pyrope 30.1 33.7 35.9 35.5 35.0 35.1 31.8 32.9 35.1 36.2 36.0 37.4 38.5 40.6 36.2
      Spessartine 0.91 0.86 0.82 0.80 0.82 0.96 0.71 0.92 0.89 0.75 0.91 0.89 0.75 0.84 0.8
      Uvarovite 0.22 0.00 0.02 0.07 0.19 0.21 0.24 0.18 0.09 0.15 0.15 0.10 0.13 0.14 0.3
      Sample 16DB27-4 16DB27-2 16DB27-7
      Spot Grt3 Grt8 Grt19 Grt22 Grt26 Grt1 Grt13 Grt18 Grt22 Grt29 Grt1 Grt18 Grt24 Grt27 Grt39
      SiO2 38.99 39.72 39.45 39.93 39.41 39.41 39.37 39.33 39.09 38.77 39.35 38.87 39.20 39.35 39.04
      TiO2 0.00 0.00 0.00 0.04 0.00 0.00 0.02 0.00 0.00 0.01 0.02 0.04 0.02 0.00 0.03
      Al2O3 22.52 22.70 22.52 22.53 22.63 22.72 22.62 22.34 22.51 22.33 21.98 22.36 21.54 21.90 21.94
      Cr2O3 0.03 0.07 0.06 0.08 0.01 0.04 0.06 0.07 0.04 0.05 0.05 0.03 0.03 0.00 0.06
      FeO 18.00 17.72 19.81 18.17 19.66 19.34 18.83 19.24 21.48 21.84 21.34 21.60 23.56 22.04 21.65
      MnO 0.39 0.39 0.38 0.37 0.39 0.35 0.39 0.39 0.46 0.53 0.42 0.37 0.44 0.41 0.38
      MgO 9.55 10.10 9.18 10.13 9.60 10.38 11.04 10.03 9.68 8.79 7.70 7.75 6.23 7.29 7.77
      CaO 9.61 8.57 8.24 8.66 7.56 7.44 6.80 8.10 6.31 7.50 8.68 8.25 9.03 9.20 8.76
      Total 99.07 99.27 99.65 99.90 99.25 99.69 99.13 99.49 99.58 99.81 99.54 99.27 100.04 100.19 99.63
      Atom per 12 O
      Si 2.96 2.99 2.99 3.00 2.99 2.97 2.98 2.98 2.98 2.96 3.01 2.98 3.02 3.01 2.99
      Ti 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00
      Al iv 0.04 0.01 0.01 0.00 0.01 0.03 0.02 0.02 0.02 0.04 0.00 0.02 0.00 0.00 0.01
      Al vi 1.98 2.01 2.00 1.99 2.01 2.00 1.99 1.98 2.00 1.98 1.98 2.01 1.96 1.97 1.98
      Cr 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00 0.00
      Fe2+ 1.13 1.14 1.27 1.14 1.27 1.22 1.19 1.20 1.37 1.38 1.37 1.40 1.50 1.39 1.37
      Fe3+ 0.01 0.00 0.00 0.00 0.00 0.00 0.00 0.02 0.00 0.02 0.00 0.00 0.02 0.02 0.01
      Mn 0.02 0.02 0.02 0.02 0.02 0.02 0.02 0.03 0.03 0.03 0.03 0.02 0.03 0.03 0.02
      Mg 1.08 1.13 1.04 1.13 1.08 1.17 1.24 1.13 1.10 1.00 0.88 0.89 0.72 0.83 0.89
      Ca 0.78 0.69 0.67 0.70 0.61 0.60 0.55 0.66 0.52 0.61 0.71 0.68 0.75 0.75 0.72
      Total 8.02 8.00 8.00 8.00 8.00 8.01 8.01 8.01 8.01 8.02 7.99 8.01 7.99 8.00 8.00
      Almandine 36.3 38.0 42.1 38.1 42.3 39.7 38.8 39.1 44.8 44.3 45.7 46.7 49.7 46.0 45.5
      Andradite 0.63 0.00 0.00 0.00 0.00 0.04 0.05 0.90 0.00 0.97 0.00 0.00 0.78 0.86 0.71
      Grossular 25.7 23.0 22.2 23.0 20.5 20.1 18.3 21.0 17.2 19.6 23.7 22.6 24.3 24.4 23.1
      Pyrope 36.5 38.0 34.7 37.8 36.3 39.3 41.8 38.0 36.9 33.8 29.5 29.7 24.2 27.8 29.7
      Spessartine 0.84 0.83 0.82 0.79 0.83 0.75 0.83 0.84 0.99 1.16 0.91 0.80 0.96 0.90 0.82
      Uvarovite 0.10 0.20 0.19 0.23 0.03 0.13 0.18 0.20 0.13 0.14 0.16 0.09 0.09 0.00 0.19
      下载: 导出CSV
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