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    华北平原与大同盆地原生高碘地下水赋存主控因素的异同

    王雨婷 李俊霞 薛肖斌 田小伟 迟秀成

    王雨婷, 李俊霞, 薛肖斌, 田小伟, 迟秀成, 2021. 华北平原与大同盆地原生高碘地下水赋存主控因素的异同. 地球科学, 46(1): 308-320. doi: 10.3799/dqkx.2019.261
    引用本文: 王雨婷, 李俊霞, 薛肖斌, 田小伟, 迟秀成, 2021. 华北平原与大同盆地原生高碘地下水赋存主控因素的异同. 地球科学, 46(1): 308-320. doi: 10.3799/dqkx.2019.261
    Wang Yuting, Li Junxia, Xue Xiaobin, Tian Xiaowei, Chi Xiucheng, 2021. Similarities and Differences of Main Controlling Factors of Natural High Iodine Groundwater between North China Plain and Datong Basin. Earth Science, 46(1): 308-320. doi: 10.3799/dqkx.2019.261
    Citation: Wang Yuting, Li Junxia, Xue Xiaobin, Tian Xiaowei, Chi Xiucheng, 2021. Similarities and Differences of Main Controlling Factors of Natural High Iodine Groundwater between North China Plain and Datong Basin. Earth Science, 46(1): 308-320. doi: 10.3799/dqkx.2019.261

    华北平原与大同盆地原生高碘地下水赋存主控因素的异同

    doi: 10.3799/dqkx.2019.261
    基金项目: 

    国家自然科学基金项目 41502230

    详细信息
      作者简介:

      王雨婷(1996-), 女, 硕士研究生, 主要从事地下水污染与防治方面的研究工作.ORCID:0000-0002-9462-9736.E-mail:cugwyt@cug.edu.cn

      通讯作者:

      李俊霞, ORCID:0000-0001-5191-3166.E-mail:jxli@cug.edu.cn

    • 中图分类号: P641.1

    Similarities and Differences of Main Controlling Factors of Natural High Iodine Groundwater between North China Plain and Datong Basin

    • 摘要: 原生高碘地下水在我国有广泛分布,为查明不同区域地下水碘赋存机理的异同,通过选取我国大同盆地以及华北平原为代表性区域,完成区域地下水样品系统性采集及水化学、碘形态测试工作,对区域地下水水环境及其演化特征完成详细刻画.结果表明:大同盆地地下水总碘含量为2.86~1 286 μg/L,华北平原地下水总碘含量为2.40~1 106 μg/L,分别约有50.0%及49.5%地下水碘含量超过(GB19380- 2016)《水源性高碘地区和高碘病区的划定》中界定的100 μg/L国家标准.地下水水环境特征表明,在大同盆地,第四纪河湖相沉积所形成的,富含有机质、偏碱性、还原性、Na-HCO3型水环境,利于赋存于固相介质上的碘以碘离子的形式进入地下水中,沿地下水流向,富集于盆地中心排泄区;在华北平原,由第四纪6次海侵形成的冲湖积、海积松散沉积物中富含Na、Cl、I等元素,其偏碱性、还原性、Na-Cl型水环境及低水力坡度的平缓地形利于赋存在固相介质上的碘以碘离子的形式进入地下水,沿地下水流向富集于沿海排泄区.控制两个地区高碘地下水形成的相同因素是偏碱性及偏还原的地下水环境,且该环境下碘的主要赋存形态均为碘离子,但大同盆地高碘地下水形成主要受富有机质环境影响,而华北平原高碘地下水形成的主要受富碘的海相沉积控制.

       

    • 图  1  研究区及采样点分布

      Fig.  1.  Location of the study area and sampling sites

      图  2  大同盆地AA’水文地质剖面(a)和华北平原BB’水文地质剖面(b)

      a.引自Guo and Wang(2005); b.张兆吉和费宇红(2009)

      Fig.  2.  Hydrogeological cross⁃section along the AA' line of Datong basin (a) and BB' line of NCP (b)

      图  3  大同盆地(左)及华北平原(右)地下水样piper三线图

      Fig.  3.  Piper diagram of groundwater samples from Datong basin (left) and NCP (right)

      图  4  大同盆地(左)及华北平原(右)聚类分析树状图

      Fig.  4.  Parameters clustering analysis of Datong basin (left) and NCP (right)

      图  5  大同盆地与华北平原总碘含量与Cl/Br摩尔比关系

      Fig.  5.  Iodine concentration vs. Cl/Br molar ratio of groundwater samples from Datong basin and NCP

      图  6  大同盆地与华北平原地下水pH (a)、Eh(b)、I-(c)含量与I含量关系图; (d)大同盆地与华北平原地下水总碘与TOC及HCO3-含量关系图; (e)大同盆地三类地下水样总碘与TOC及HCO3-含量关系图

      Fig.  6.  The relationship between iodine and pH(a), Eh(b), I-(c) of groundwater from Datong basin and NCP; (d) variation of TOC with HCO3- with different iodine concentration; (e) relationships of total iodine with TOC and HCO3- contents in three kinds of groundwater samples in Datong basin

      表  1  研究区地下水化学组分

      Table  1.   Chemical composition of groundwater samples from study area

      参数 大同盆地(n=82) 华北平原(n=96)
      最小值 最大值 中间值 均值 最小值 最大值 中间值 均值
      TDS
      (mg/L)
      373.2 8 533.0 1 337.0 2 383.0 370.9 7 590.0 1 060.0 1 240.0
      TOC
      (mg/L)
      < 0.01 92.14 5.45 2.65 0.13 37.90 0.86 2.23
      Eh (mV) -189.0 224.0 112.0 83.06 -228.50 139.60 34.40 9.79
      pH 6.90 9.73 7.82 7.91 6.46 8.79 8.00 7.89
      K+(mg/L) 0.49 79.37 2.70 4.55 0.13 8.12 1.05 1.40
      Na+(mg/L) 10.57 2
      208.00
      259.20 506.70 8.57 1 953.00 282.80 344.30
      Ca2+(mg/L) 3.86 442.80 38.34 56.77 < 0.01 393.90 17.85 42.47
      Mg2+(mg/L) 13.26 498.90 42.10 92.35 0.83 522.40 14.75 34.35
      HCO3-(mg/L) 181.3 1 842.0 519.8 615.1 142.7 916.8 366.0 387.5
      Cl-(mg/L) 8.57 3
      214.00
      155.90 509.40 9.16 1
      874.00
      151.10 251.80
      Br-(μg/L) 22.48 3
      611.00
      423.00 801.00 16.46 4
      035.00
      381.20 609.60
      SO42-(mg/L) 3.63 2
      395.00
      196.40 523.10 < 0.01 2
      159.00
      84.45 178.50
      Cl/Br(摩尔比) 171.30 3
      725.00
      1
      042.00
      1
      230.00
      147.00 5
      637.00
      937.00 1
      143.00
      Fe(mg/L) < 0.01 3.47 0.06 0.18 < 0.01 3.46 0.09 0.30
      Fe2+(mg/L) < 0.01 0.45 0.05 0.08 < 0.01 0.56 0.01 0.02
      I(μg/L) 2.86 1
      286.00
      105.60 230.40 2.40 1
      106.00
      93.82 198.10
      I-(μg/L) 1.28 1
      157.00
      50.89 168.30 < 0.01 854.00 63.40 164.70
      IO3-(μg/L) < 0.01 999.30 5.720 46.08 < 0.01 292.80 0.66 20.38
      下载: 导出CSV

      表  2  大同盆地与华北平原旋转因子载荷矩阵

      Table  2.   Matrix of rotated factor loadings of Datong basin and NCP

      因子 大同盆地 华北平原
      F1 F2 F3 F1 F2 F3 F4 F5
      TDS 0.937 0.307 0.091 0.420 0.873 0.154 -0.018 0.129
      Na+ 0.820 0.481 0.142 0.736 0.477 -0.178 -0.203 0.265
      Ca2+ 0.793 -0.347 -0.214 -0.204 0.709 0.463 0.344 -0.144
      Mg2+ 0.955 -0.079 -0.044 -0.149 0.829 0.373 0.180 -0.124
      Cl- 0.958 0.149 -0.040 0.621 0.610 -0.133 -0.090 0.253
      Br- 0.704 0.527 -0.205 0.569 0.605 -0.100 -0.337 0.108
      Cl/Br摩尔比 0.696 -0.246 0.278 -0.042 -0.051 0.018 0.919 0.091
      SO42- 0.921 0.139 0.090 0.008 0.926 0.063 0.009 -0.040
      HCO3- 0.180 0.842 0.194 0.100 0.230 0.769 0.126 0.020
      TOC 0.037 0.825 0.205 -0.041 0.045 0.858 0.020 -0.052
      pH -0.449 0.546 -0.078 0.083 -0.386 -0.420 -0.640 0.114
      I 0.112 0.850 -0.294 0.891 0.004 -0.014 -0.029 0.166
      I- 0.055 0.796 -0.415 0.913 -0.002 -0.021 -0.027 -0.038
      Eh 0.047 -0.108 0.700 -0.738 -0.020 0.064 -0.070 0.371
      Fe 0.074 0.177 -0.814 0.620 -0.015 0.150 -0.048 -0.053
      IO3- 0.085 0.225 0.615 -0.019 -0.015 -0.051 0.047 0.939
      特征值 6.102 3.970 2.080 4.069 3.984 1.973 1.596 1.275
      贡献率(%) 38.1 24.8 13.0 25.4 24.9 12.3 10.0 8.0
      累计贡献率(%) 38.1 63.0 75.9 25.4 50.3 62.7 72.6 80.6
      注:黑体数字表示较高因子载荷.
      下载: 导出CSV
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    • 收稿日期:  2019-10-22
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