Geochemistry and Geochronology of Mafic Rocks from Hongqiyingzi Group in Chongli Area of the Northern Hebei Province: Implications for the Late Neoarchean-Early Paleoproterzoic Tectonic Evolution of the North China Craton
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摘要: 崇礼地区红旗营子岩群位于华北克拉通北缘，该区红旗营子岩群的岩石组合、构造属性及时代归属对于探讨华北克拉通新太古代晚期－古元古代早期大地构造演化具有重要意义.本文对崇礼地区红旗营子岩群中的镁铁质岩石进行了野外、镜下岩相学、全岩地球化学、锆石U-Pb年代学及Hf同位素分析，并讨论其对华北克拉通北缘新太古代晚期－古元古代早期地壳演化的指示意义.研究区红旗营子岩群中的镁铁质岩石以夹层产出于表壳岩中，主要由斜长角闪岩和斜长辉石角闪岩组成.红旗营子镁铁质岩石主量元素中SiO2（40.17%~51.53%）、Na2O（1.52%~3.47%）和K2O（0.43%~1.23%）含量范围较大，具有较高的CaO（9.15%~12.68%）、MgO（5.90%~13.36%）和Al2O3（9.81%~20.92%）含量.镁铁质岩石轻稀土元素轻微富集，重稀土元素配分模式近平坦，大离子亲石元素Ba、U、K、Sr富集，高场强元素Th、Nb、Ta、Ti明显亏损.斜长角闪岩LA-ICP-MS锆石U-Pb测年显示207Pb/206Pb加权平均年龄为2 477±23 Ma（MSWD=3.1），上交点年龄为2 468±22 Ma，表明其形成于新太古代晚期－古元古代早期.斜长角闪岩锆石Hf同位素分析结果显示εHf（t）为负值（-5.2~0），一阶段模式年龄（TDM1）为2 673~2 783 Ma，二阶段模式年龄（TDM2）为2 880~3 074 Ma，均大于锆石的形成年龄，指示其来源于古老地壳物质的再循环.镁铁质岩石全岩地球化学分析结果显示其形成于岛弧相关环境.结合华北其他地区研究成果，本研究表明崇礼地区新太古代晚期－古元古代早期可能发生了一期与岛弧有关的岩浆事件.Abstract: The Hongqiyingzi Group in the Chongli area is located in the northern margin of the North China Craton. The rock association, structural characteristics and formation age of the Hongqiyingzi Group in the Chongli area are of great significance to study the tectonic evolution of the North China Craton from late Neoarchean to early Paleoproterozoic. In this paper, based on field, petrography, geochemistry, zircon U-Pb geochronology and Hf isotope analysis of these mafic rocks from the Hongqiyingzi Group in Chongli area, we study the origin and genesis of these rocks and discuss their tectonic implications on the late Neoarchean to early Paleoproterozoic crustal evolution of the North China Craton. The mafic rocks of the Hongqiyingzi Group are mainly composed of amphibolite and clinopyroxene amphibolite. The mafic rocks have a relatively wide range of geochemical compositions including SiO2 (40.17%－51.53%), Na2O (1.52%－3.47%) and K2O (0.43%－1.23%). These rocks have relatively high values of CaO (9.15%－12.68%), MgO (5.90%－13.36%) and Al2O3 (9.81%－20.92%), and are characterized by enrichment of large ion lithophile elements such as Ba, U, K, and Sr, depletion of high field strength elements such as Th, Nb, Ta, and Ti and flat heavy rare earth elements patterns. The LA-ICP-MS zircon U-Pb dating shows that the magmatic zircon of amphibolite was formed at 2 477±23 Ma, with the upper intercept age of 2 468±29 Ma, representing its formation age. The Hf isotopic analyses of amphibolite show that the εHf(t) values are negative (－5.2－0). The one-stage (TDM1) and two-stage Hf model ages (TDM2) are 2 673－2 783 Ma and 2 880－3 074 Ma, respectively, indicating that they were originated from recycling of the Archean crustal materials. In addition, the εHf(t) values of zircons suggest that a crustal accretion event occurred in the Neoarchean in the Chongli area. The geochemical characteristics indicate that these rocks were formed in an arc-related tectonic environment. Based on the research of other areas in the North China Craton, we suggest that a magmatic event related with arc environment may have occurred in the late Neoarchean to early Paleoproterozoic in the Chongli area.
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Key words:
- North China Craton /
- Hongqiyingzi Group /
- geochemistry /
- zircon U-Pb geochronology /
- Hf isotope /
- tectonic evolution
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图 1 华北克拉通大地构造单元划分（a）和崇礼地区地质图（b
Fig. 1. Tectonic subdivision of the North China Craton (a) and geological map of the Chongli area (b)
图 2 镁铁质岩石野外特征
a.似层状斜长角闪岩；b.透镜状斜长角闪岩；c.似层状斜长辉石角闪岩；d.透镜状斜长辉石角闪岩
Fig. 2. Field photos of mafic rocks
图 3 镁铁质岩石岩相学特征（正交偏光）
a、b.斜长角闪岩主要由角闪石、斜长石和黑云母组成；c、d.斜长辉石角闪岩主要由角闪石、辉石、斜长石和黑云母组成. Pl.斜长石；Am.角闪石；Aug.辉石；Bi.黑云母
Fig. 3. Photomicrographs of mafic rocks (crossed polarized light)
图 6 红旗营子镁铁质岩球粒陨石标准化REE配分图(a)；镁铁质岩原始地幔标准化微量元素蛛网图(b)
图a标准化值据Sun and McDonough, 1989；图b标准化值据McDonough and Sun, 1995
Fig. 6. Chondrite-normalized rare earth element diagrams of mafic rock (a); primitive mantle-normalized trace element diagrams of mafic rock (b)
图 7 SiO2-Zr/TiO2×0.000 1图解（a；据Winchester and Floyd, 1977）；FeOT/MgO-SiO2图解（b；据Miyashiro, 1974）
Fig. 7. SiO2-Zr/TiO2×0.000 1 diagram (a; modified from Winchester and Floyd, 1977); SiO2-FeOT/MgO diagram (b; modified from Miyashiro, 1974)
图 9 红旗营子镁铁质岩哈克图解（据Ajaji et al., 1998）
Fig. 9. Harker diagram of mafic rock in Chongli area (modified from Ajaji et al., 1998)
图 10 Th/Yb-Nb/Yb判别图（a；据Pearce, 2008）；Nb/Th-Nb判别图（b；据李曙光，1993）；La/Nb-La判别图（c；据李曙光，1993）
Fig. 10. Th/Yb versus Nb/Yb diagram (a; modified from Pearce, 2008); Nb/Th-Nb diagram (b; modified from Li, 1993); La/Nb versus La diagram (c; modified from Li, 1993)
表 1 锆石U⁃Pb同位素测年结果
Table 1. Zircon U⁃Pb dating data
样品号 (10-6) 同位素比值 年龄（Ma） CL-TW1 Th U Th/U 207Pb/206Pb 1σ 207Pb/235U 1σ 206Pb/238U 1σ 207Pb/206Pb 1σ 207Pb/235U 1σ 206Pb/238U 1σ RZ1 110 127 0.87 0.16174 0.00184 10.00894 0.16799 0.45163 0.00543 2 474 19 2 436 15 2 403 24 RZ2 85 30 2.84 0.14950 0.00346 9.28582 0.51360 0.43268 0.00713 2 340 39 2 367 51 2 318 32 RZ3 66 67 0.98 0.16828 0.00203 9.22057 0.17887 0.40191 0.00492 2 541 20 2 360 18 2 178 23 RZ4 70 192 0.37 0.16501 0.00187 9.60398 0.15877 0.43760 0.00526 2 508 19 2 398 15 2 340 24 RZ5 17 33 0.51 0.16119 0.00523 7.01405 0.51171 0.29565 0.00605 2 468 54 2 113 65 1 670 30 RZ6 182 209 0.87 0.16209 0.00214 9.52324 0.24028 0.43292 0.00512 2 478 22 2 390 23 2 319 23 RZ7 84 202 0.41 0.16044 0.00187 9.51457 0.17660 0.44133 0.00494 2 460 20 2 389 17 2 357 22 RZ8 50 86 0.59 0.16484 0.00202 10.24977 0.22114 0.44666 0.00509 2 506 20 2 458 20 2 380 23 RZ9 115 94 1.23 0.16180 0.00228 9.28046 0.26017 0.42462 0.00512 2 475 24 2 366 26 2 281 23 RZ10 53 45 1.18 0.16086 0.00211 10.48173 0.27312 0.46073 0.00612 2 465 22 2 478 24 2 443 27 RZ11 52 69 0.76 0.16635 0.00300 10.09918 0.41617 0.43968 0.00665 2 521 30 2 444 38 2 349 30 RZ12 107 100 1.07 0.15575 0.00262 9.41148 0.34769 0.41806 0.00606 2 410 28 2 379 34 2 252 28 RZ13 270 388 0.70 0.15999 0.00166 10.34474 0.15770 0.46436 0.00573 2 456 17 2 466 14 2 459 25 RZ14 79 160 0.50 0.16067 0.00190 10.10095 0.21283 0.46026 0.00586 2 463 20 2 444 19 2 441 26 
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表 2 崇礼镁铁质岩Lu-Hf同位素分析结果
Table 2. Lu-Hf isotopic analysis data of mafic rock in the Chongli area
样号 年龄(Ma) 176Yb/177Hf 176Lu/177Hf 176Hf/177Hf εHf(0) εHf(t) TDM1(Ma) TDM2(Ma) CL-TW1-1 2 474 0.010710 0.000356 0.281223 -54.77 -1.5 2 783 3 019 CL-TW1-2 2 340 0.012890 0.000464 0.281301 -52.02 -0.8 2 686 2 913 CL-TW1-3 2 541 0.012956 0.000419 0.281265 -53.31 -5.2 2 732 3 074 CL-TW1-4 2 508 0.006784 0.000271 0.281301 -52.02 0.0 2 673 2 880
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表 3 崇礼地区红旗营子岩群镁铁质岩石主量元素（%）和微量元素（10-6）分析结果
Table 3. Major (%) and trace elements (10-6) compositions of mafic rock in the Chongli area
样品号 CL-1 CL-2 CL-3 CL-4 CL-5 CL-6 CL-7 CL-8 岩性 斜长角闪岩 斜长角闪岩 斜长辉石角闪岩 斜长角闪岩 斜长角闪岩 斜长辉石角闪岩 斜长角闪岩 斜长角闪岩 GPS 115°04′37″E 115°03′58″E 115°09′24″E 115°08′31″E 115°09′14″E 115°12′49″E 115°15′21″E 115°26′18″E 41°01′4″N 41°00′58″N 41°01′30″N 41°01′05″N 41°00′12″N 41°01′22″N 41°01′56″N 41°01′55″N SiO2 47.85 45.46 40.17 51.53 46.96 43.48 50.53 45.36 TiO2 0.60 1.58 2.08 0.57 0.61 1.51 0.36 1.77 Al2O3 19.81 17.99 20.92 9.81 13.58 19.06 14.86 14.14 Fe2O3 2.67 4.15 4.70 2.30 6.76 2.46 1.49 4.22 FeO 6.52 8.72 8.83 6.48 8.85 5.84 6.88 8.62 MnO 0.13 0.19 0.11 0.18 0.19 0.11 0.19 0.19 MgO 6.79 5.90 7.31 13.36 7.95 9.16 10.12 8.93 CaO 9.21 9.60 10.28 10.24 9.15 12.68 9.42 10.44 Na2O 3.04 3.47 2.42 1.52 2.91 1.84 2.59 2.49 K2O 0.43 0.69 0.55 0.58 0.92 0.72 1.15 1.23 P2O5 0.058 0.300 0.056 0.130 0.071 0.100 0.032 0.390 LOI 2.71 1.75 2.38 3.12 1.94 2.86 2.26 2.06 Total 99.83 99.79 99.82 99.82 99.88 99.83 99.87 99.84 La 4.04 19.10 4.36 11.00 13.90 5.32 13.50 17.10 Ce 9.63 47.30 12.40 26.40 30.10 13.20 37.00 44.80 Pr 1.52 7.18 2.24 3.92 4.29 2.28 5.99 7.41 Nd 7.5 32.6 12.4 18.0 19.1 12.0 28.2 36.6 Sm 1.76 6.82 3.49 4.13 4.35 3.35 7.40 8.48 Eu 0.87 1.81 1.29 1.14 1.39 1.49 1.19 2.00 Gd 1.40 5.64 2.91 3.33 3.77 2.99 5.91 6.71 Tb 0.23 0.95 0.51 0.56 0.69 0.55 1.03 1.12 Dy 1.40 5.94 3.15 3.31 4.38 3.04 5.95 6.68 Ho 0.27 1.12 0.57 0.61 0.82 0.56 1.03 1.24 Er 0.75 3.26 1.56 1.71 2.42 1.47 2.78 3.50 Tm 0.11 0.49 0.23 0.26 0.40 0.21 0.41 0.53 Yb 0.70 2.98 1.28 1.52 2.41 1.26 2.31 3.01 Lu 0.11 0.44 0.19 0.23 0.39 0.19 0.34 0.45 ∑REE 30.28 135.67 46.55 76.05 88.32 47.93 113.00 139.73 LREE 25.32 114.84 36.15 64.52 73.05 37.67 93.24 116.49 HREE 4.96 20.83 10.40 11.53 15.27 10.26 19.76 23.24 LREE/HREE 5.10 5.51 3.47 5.60 4.79 3.67 4.72 5.01 (La/Sm)N 1.48 1.81 0.81 1.72 2.06 1.03 1.18 1.30 (La/Yb)N 4.14 4.60 2.44 5.19 4.14 3.03 4.19 4.08 La/Yb 4.14 4.61 2.44 5.17 4.13 3.04 4.17 4.09 Zr/Y 6.39 2.78 3.46 5.80 4.81 5.02 2.82 1.44 δEu 1.64 0.87 1.21 0.91 1.03 1.41 0.53 0.78 δCe 0.95 0.99 0.96 0.98 0.95 0.93 1.01 0.97 Ti 3 596 9 470 12 466 3 416 3 656 9 050 2 158 10 608 Cr 42.70 10.60 7.16 543.00 163.00 30.00 185.00 222.00 Rb 0.91 7.51 0.59 2.90 3.10 9.40 5.95 7.86 Ba 282 603 274 215 167 393 203 186 K 3 570 5 728 4 566 4 815 7 637 5 977 9 547 12 011 GPS 115°04′37″E 115°03′58″E 115°09′24″E 115°08′31″E 115°09′14″E 115°12′49″E 115°15′21″E 115°26′18″E 41°01′4″N 41°00′58″N 41°01′30″N 41°01′05″N 41°00′12″N 41°01′22″N 41°01′56″N 41°01′55″N Th 0.32 0.47 0.51 1.95 1.32 0.42 1.50 0.69 U 0.14 0.54 0.16 0.56 0.75 0.38 0.85 0.31 Zr 43.2 85.5 52.2 93.3 112.0 67.8 79.6 46.1 Hf 1.17 2.77 1.51 2.63 3.18 1.86 2.91 1.69 Sr 1 477 689 1 102 369 342 855 420 372 Y 6.76 30.80 15.10 16.10 23.30 13.50 28.20 32.00 Nb 1.13 6.31 2.61 3.20 13.40 2.84 7.69 6.57 Ta 0.19 0.23 0.15 0.20 0.87 0.13 0.44 0.40 Ga 17.6 22.3 22.3 13.1 19.0 14.6 19.6 19.1 Cr 42.70 10.60 7.16 543.00 163.00 30.00 185.00 222.00 V 161 254 370 155 170 218 298 179
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