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    Volume 36 Issue 6
    Jun.  2011
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    MEN Wu, LIU Guang-shan, CHEN Min, HUANG Yi-pu, 2011. 224Ra in the Seawater of the East China Sea. Earth Science, 36(6): 999-1008. doi: 10.3799/dqkx.2011.106
    Citation: MEN Wu, LIU Guang-shan, CHEN Min, HUANG Yi-pu, 2011. 224Ra in the Seawater of the East China Sea. Earth Science, 36(6): 999-1008. doi: 10.3799/dqkx.2011.106

    224Ra in the Seawater of the East China Sea

    doi: 10.3799/dqkx.2011.106
    • Received Date: 2011-03-18
      Available Online: 2021-11-10
    • Publish Date: 2011-06-15
    • 224Ra in the seawater of the East China Sea (ECS) were measured using Mn-fiber adsorption—emanation method. The content level and distribution feature of 224Ra in sea water in summer and winter were studied. The 224Ra activities were < LLD~5.88Bq/m3 with an average of 0.85Bq/m3 in the summer and < LLD~7.50Bq/m3 with an average of 0.72Bq/m3 in the winter. Both seasons 224Ra in the surface water have similar distribution and decreased rapidly with the increasing distance from the coast. The high 224Ra activity at 0.5-7.5Bq/m3 is located within 30-100km offshore and the lowest activity at < 0.13Bq/m3 was in the Kuroshio Current. The 224Ra concentrations in the middle shelf are 0.13-0.5Bq/m3. The vertical distributions showed two different characteristics. The horizontal and vertical eddy diffusion coefficients calculated by the one-dimensional state model of 224Ra were (7.1-88.9)×106cm2/s and 2.18-163cm2/s, respectively. The upwelling rates off Zhejiang were calculated using 224Ra vertical distribution, which varied between (8.4-13.3)×10-3cm/s in the summer and (16.3-16.8)×10-3cm/s in the winter.

       

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    • Bollinger, M.S., Moore, W.S., 1984. Radium fluxes from a salt marsh. Nature, 309: 444-446. doi: 10.1038/309444a0
      Chen, X.B., Huang, Y.P., Xie, Y.Z., et al., 1999. Distribution of 224Ra in the Jiulong Estuarine waters and its application. Acta Oceanologica Sinica, 21(4): 54-61 (in Chinese with English abstract). http://qikan.cqvip.com/Qikan/Article/Detail?id=3581451
      Chen, X.B., Xie, Y.Z., Huang, Y.P., et al., 1998. Profiles of 224Ra in the Xiamen bay waters and its application. Acta Oceanologica Sinica, 20(6): 50-57 (in Chinese with English abstract). http://www.hyxb.org.cn/aos/ch/reader/view_abstract.aspx?file_no=19980607
      Cochran, J.K., 1992. The oceanic chemistry of the U- and Th-series nuclides in the ocean. In: Ivanovich, M.I., Harmon, R.S., eds., Uranium-series disequilibrium: application to earth, marine, and environmental science (Second edition). Clarendon Press, Oxford, 364-375.
      Colbert, S.L., Hammond, D.E., 2007. Temporal and spatial variability of radium in the coastal ocean and its impact on computation of nearshore cross-shelf mixing rates. Continental Shelf Research, 27(10-11): 1477-1500. doi: 10.1016/j.csr.2007.01.003
      Elsinger, R.J., Moore, W.S., 1983. 224Ra, 228Ra, and 226Ra in Winyah bay and Delaware bay. Earth and Planetary Science Letters, 64(3): 430-436. doi: 10.1016/0012-821X(83)90103-6
      Hougham, A.L., Moran, S.B., 2007. Water mass ages of coastal ponds estimated using 223Ra and 224Ra as tracers. Marine Chemistry, 105(3-4): 194-207. doi: 10.1016/j.marchem.2007.01.013
      Hu, D.X., Lü, L.H., Xiong, Q.C., et al., 1980. Studies on the upwelling of Zhejiang. Chinese Science Bulletin, (3): 131-133 (in Chinese). http://www.researchgate.net/publication/313708033_Studies_on_the_upwelling_off_Zhejiang
      Hu, D.X., Yang, Z.S., 2001. The key processes for marine fluxes of the East China Sea. China Ocean Press, Bejing (in Chinese).
      Hu, M.N., Zhao, C.F., 2008. Upwelling in Zhejiang coastal areas during summer detected by satellite observations. Journal of Remote Sensing, 12(2): 297-304 (in Chinese with English abstract). http://www.oalib.com/paper/1470423
      Huang, Y.P., Xie, Y.Z., Chen, X.B., et al., 2001. A new method for rapid concentration and determination of 224Ra in seawater. Journal of Xiamen University (Natural Science), 40(3): 699-705 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-XDZK200103010.htm
      Huang, Z.K., Yu, G.Y., Luo, Y.Y., et al., 1996. Numerical modeling of tide induced upwelling in coastal areas of the East China Sea. Journal of Ocean University of Qingdao, 26(4): 405-412 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-QDHY604.002.htm
      Iseki, K., Okamura, K., Kiyomoto, K., 2003. Seasonality and composition of downward particulate fluxes at the continental shelf and Okinawa Trough in the East China Sea. Deep Sea Research Part Ⅱ: Topical Studies in Oceanography, 50(2): 457-473. doi:10.1016/ S0967-0645(02)00468-X
      Krest, J.M., Harvey, J.W., 2003. Using natural distributions of short-lived radium isotopes to quantify groundwater discharge and recharge. Limnology and Oceanography, 48(1): 290-298. doi: 10.4319/lo.2003.48.1.0290
      Krishnaswami, S., 2001. Uranium thorium series isotopes in ocean profiles. In: Steele, J.H., Thorpe, S.A., Turekian, K.K., eds., Encyclopedia of ocean sciences. Academic Press, London, 3146-3156.
      Levy, D.M., Moore, W.S., 1985. 224Ra in continental shelf waters. Earth and Planetary Science Letters, 73(2-4): 226-230. doi: 10.1016/0012-821X(85)90071-8
      Liu, G.S., Yang, W.F., Jia, C.X., et al., 2004. Rapid concentration in-situ and γ spectrum analysis of radium isotopes in large volume seawater. Nuclear Techniques, 27(2): 116-121 (in Chinese with English abstract).
      Liu, X.B., Su, J.L., 1991. The numerical study on the upwelling of Zhejiang and the coastal front. Acta Oceanologica Sinica, 13(3): 305-314 (in Chinese).
      Luo, Y.Y., Yu, G.Y., 1998. Numerical studies of wind and TWC driven upwelling in coastal areas of the East China Sea. Journal Ocean University of Qingdao (Natural Science), 28(4): 536-542 (in Chinese with English abstract). http://www.cnki.com.cn/Article/CJFDTotal-QDHY804.003.htm
      Mao, H.L., Ren, Y.W., Wan, G.M., 1964. A preliminary investigation on the application of using T-S diagrams for a quantitative analysis of the watermasses in the shallow water area. Oceanologia et Limnologia Sinnica, 6(1): 1-21 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTotal-HYFZ196401000.htm
      Men, W., Liu, G.S., Chen, Z.G., et al., 2010. Progress of radium isotopes applications to oceanography research. Advances in Earth Science, 25(1): 33-42 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-DXJZ201001008.htm
      Moore, W.S., 2000. Determining coastal mixing rates using radium isotopes. Continental Shelf Research, 20(15): 1993-2007. doi: 10.1016/S0278-4343(00)00054-6
      Moore, W.S., Todd, J.F., 1993. Radium isotopes in the Orinoco Estuary and eastern Caribbean Sea. Journal of Geophysical Research, 98(C2): 2233-2244. doi: 10.1029/92JC02760
      Nozaki, Y., Kasemsupaya, V., Tsubota, H., 1989. Mean residence time of the shelf water in the East China and the Yellow Seas determined by 228Ra/226Ra measurements. Geophysical Research Letters, 16(11): 1297-1300. doi: 10.1029/GL016i011p01297
      Nozaki, Y., Tsubota, H., Kasemsupaya, V., et al., 1991. Residence times of surface water and particle-reactive 210Pb and 210Po in the East China and Yellow seas. Geochimica et Cosmochimica Acta, 55(5): 1265-1272. doi: 10.1016/0016-7037(91)90305-O
      Pan, Y.Q., Xu, D.R., Xu, J.P., 1985. The front structure, variation and causes of upwelling off Zhejiang. Acta Oceanologica Sinica, 7(4): 401-411 (in Chinese).
      Rama., Todd, J.F., Butts, J.L., et al., 1987. A new method for the rapid measurement of 224Ra in the natural waters. Marine Chemistry, 22(1): 43-54. doi: 10.1016/0304-4203(87)90047-8
      Smith, M.R., Lautensleger, A.W., Laul, J.C., 1988. A new method for the determination of radium-228, thorium-228, and radium-224 in groundwaters via thoron (radon-220). Journal of Radioanalytical and Nuclear Chemistry, 123(1): 107-119. doi: 10.1007/BF02036384
      Sun, X.P., 2006. Regional marine in China offshore. China Ocean Press, Beijing, 106-109 (in Chinese).
      Torgersen, T., Turekian, K.K., Turekian, V.C., et al., 1996. 224Ra distribution in surface and deep water of Long Island Sound: sources and horizontal transport rates. Continental Shelf Research, 16 (12): 1545-1559. doi: 10.1016/0278-4343(96)00003-9
      Webster, I.T., Hancock, G.J., Murray, A.S., et al., 1994. Use of radium isotopes to examine pore-water exchange in an estuary. Limnology and Oceanography, 39(8): 1917-1927. doi: 10.4219/lo.1994.39.8.1917
      Webster, I.T., Hancock, G.J., Murray, A.S., 1995. Modelling the effect of salinity on radium desorption from sediments. Geochimica et Cosmochimica Acta, 59(12): 2469-2476. doi: 10.1016/0016-7037(95)00141-7
      Zhang, J., 2002. Biogeochemistry of Chinese estuarine and coastal waters: nutrients, trace metals and biomarkers. Regional Environmental Change, 3(1-3): 65-76. doi: 10.1007/s10113-001-0039-3
      Zhang, L., Liu, Z., Zhang, J., et al., 2007. Reevaluation of mixing among multiple water masses in the shelf: an example from the East China Sea. Continental Shelf Research, 27(15): 1969-1979. doi: 10.1016/j.csr.2007.04.002
      陈性保, 黄奕普, 谢永臻, 等, 1999. 九龙江河口区水体中224Ra的分布及其应用. 海洋学报, 21(4): 54-61. https://www.cnki.com.cn/Article/CJFDTOTAL-SEAC199904007.htm
      陈性保, 谢永臻, 黄奕普, 等, 1998. 厦门湾海水中的224Ra的深度分布特征及其应用. 海洋学报, 20(6): 50-57. https://www.cnki.com.cn/Article/CJFDTOTAL-SEAC199806006.htm
      胡敦欣, 吕良洪, 熊庆成, 等, 1980. 关于浙江沿岸上升流的研究. 科学通报, (3): 131-133. https://www.cnki.com.cn/Article/CJFDTOTAL-KXTB198003009.htm
      胡敦欣, 杨作升, 2001. 东海海洋通量关键过程. 北京: 海洋出版社.
      胡明娜, 赵朝方, 2008. 浙江近海夏季上升流的遥感观测与分析. 遥感学报, 12(2): 297-304. https://www.cnki.com.cn/Article/CJFDTOTAL-YGXB200802015.htm
      黄奕普, 谢永臻, 陈性保, 等, 2001. 海水中224Ra快速富集和测定的新方法. 厦门大学学报(自然科学版), 40(3): 699-705. doi: 10.3321/j.issn:0438-0479.2001.03.011
      黄祖珂, 俞光耀, 罗义勇, 等, 1996. 东海沿岸潮致上升流的数值模拟. 青岛海洋大学学报, 26(4): 405-412. https://www.cnki.com.cn/Article/CJFDTOTAL-QDHY604.002.htm
      刘广山, 杨伟锋, 贾成霞, 等, 2004. 大体积海水镭同位素现场快速富集与γ谱直接测定. 核技术, 27(2): 116-121. doi: 10.3321/j.issn:0253-3219.2004.02.009
      刘先炳, 苏纪兰, 1991. 浙江沿岸上升流和沿岸锋面的数值研究. 海洋学报, 13(3): 305-314. https://www.cnki.com.cn/Article/CJFDTOTAL-SEAC199103001.htm
      罗义勇, 俞光耀, 1998. 风和台湾暖流引起东海沿岸上升流数值计算. 青岛海洋大学学报(自然科学版), 28(4): 536-542. https://www.cnki.com.cn/Article/CJFDTOTAL-QDHY804.003.htm
      毛汉礼, 任允武, 万国铭, 1964. 应用T-S关系定量地分析浅海水团的初步研究. 海洋与湖沼, 6(1): 1-21. https://www.cnki.com.cn/Article/CJFDTOTAL-HYFZ196401000.htm
      门武, 刘广山, 陈志刚, 等, 2010. 镭同位素在海洋学研究中的应用及进展. 地球科学进展, 25(1): 33-42. https://www.cnki.com.cn/Article/CJFDTOTAL-DXJZ201001008.htm
      潘玉球, 徐端蓉, 许建平, 1985. 浙江沿岸上升流区的锋面结构、变化及其原因. 海洋学报, 7(4): 401-411. https://www.cnki.com.cn/Article/CJFDTOTAL-SEAC198504000.htm
      孙湘平, 2006. 中国近海区域海洋. 北京: 海洋出版社, 106-109.
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