江汉平原砷中毒病区地下水砷形态季节性变化特征

邓娅敏; 王焰新; 李慧娟; 李红梅; 郭伟; 段艳华; 董创举; 甘义群; 刘乃静; 丁旭峰

doi:10.3799/dqkx.2015.168

Volume 40 Issue 11

Nov. 2015

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Article Navigation > Earth Science > 2015 > 40(11): 1876-1886

Deng Yamin, Wang Yanxin, Li Huijuan, Li Hongmei, Guo Wei, Duan Yanhua, Dong Chuangju, Gan Yiqun, Liu Naijing, Ding Xufeng, 2015. Seasonal Variation of Arsenic Speciation in Shallow Groundwater from Endemic Arsenicosis Area in Jianghan Plain. Earth Science, 40(11): 1876-1886. doi: 10.3799/dqkx.2015.168

Citation:

Deng Yamin, Wang Yanxin, Li Huijuan, Li Hongmei, Guo Wei, Duan Yanhua, Dong Chuangju, Gan Yiqun, Liu Naijing, Ding Xufeng, 2015. Seasonal Variation of Arsenic Speciation in Shallow Groundwater from Endemic Arsenicosis Area in Jianghan Plain. Earth Science, 40(11): 1876-1886. doi: 10.3799/dqkx.2015.168

Citation:

Deng Yamin, Wang Yanxin, Li Huijuan, Li Hongmei, Guo Wei, Duan Yanhua, Dong Chuangju, Gan Yiqun, Liu Naijing, Ding Xufeng, 2015. Seasonal Variation of Arsenic Speciation in Shallow Groundwater from Endemic Arsenicosis Area in Jianghan Plain. Earth Science, 40(11): 1876-1886. doi: 10.3799/dqkx.2015.168

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Seasonal Variation of Arsenic Speciation in Shallow Groundwater from Endemic Arsenicosis Area in Jianghan Plain

doi: 10.3799/dqkx.2015.168

Deng Yamin¹,
Wang Yanxin^{2, 3
,
,},
Li Huijuan^{1, 4},
Li Hongmei¹,
Guo Wei³,
Duan Yanhua²,
Dong Chuangju¹,
Gan Yiqun^{2, 3},
Liu Naijing¹,
Ding Xufeng^{1, 4}

1.
Geological Survey, China University of Geosciences, Wuhan430074, China
2.
School of Environmental Studies, China University of Geosciences, Wuhan430074, China
3.
State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan430074, China
4.
Hubei Province Geological Environment Terminus, Wuhan430034, China

Received Date: 2015-01-26
Publish Date: 2015-11-15

Abstract

Abstract

Understanding the seasonal variation of arsenic occurrence in shallow groundwater system is one of the challenges and hot spots concerning the research on high arsenic groundwater, which plays an important role in evaluation of safe groundwater availability and remediation of arsenic-affected aquifer. To investigate the seasonal variation of arsenic speciation in the shallow aquifer from the endemic arsenicosis area in the Jianghan plain, groundwater from shallow phreatic aquifer and unconfined aquifer were monitored for arsenic speciation (As(Ⅲ), As(Ⅴ) and acid-leacheable particulate As) and water level during pre-monsoon (May), monsoon (July-August) and post-monsoon (November-December) seasons. Arsenic concentration and speciation in groundwater varied temporally: the concentration of As(Ⅴ) and particulate As were higher, together with higher particulate Fe in most samples during the pre-monsoon seasons; As(Ⅴ) and particulate As decreased significantly during monsoon seasons, while dissovled As and Fe increased dramatically. Higher As concentrations were associated with an increasing percentage of As(Ⅲ) in rainy season and a decrease towards the end of dry season, indicating a reductive moblization responding to groundwater level fluctuation.
- arsenic speciation,
- seasonal variation,
- water level fluctuation,
- redox,
- Jianghan plain,
- groundwater,
- geochemistry.

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References(48)

References

Aziz, Z., van Geen, A., Versteeg, R., et al., 2008. Impact of Local Recharge on Arsenic Concentrations in Shallow Aquifers Inferred from the Electromagnetic Conductivity of Soils in Araihazar, Bangladesh. Water Resources Research, 44: W07416. doi: 10.1029/2007WR00600

Benner, S.G., Polizzotto, M.L., Kocar, B.D., et al., 2008. Groundwater Flow in an Arsenic-Contaminated Aquifer, Mekong Delta, Cambodia. Applied Geochemistry, 23(11): 3072-3087. doi: 10.1016/j.apgeochem.2008.06.013

Berg, M., Tran, H.C., Nguyen, T.C., et al., 2001. Arsenic Contamination of Groundwater and Drinking Water in Vietnam: A Human Health Threat. Environmental Science & Technology, 35(13): 2621-2626. doi: 10.1021/es010027y

Cheng, Z., van Geen, A., Seddique, A.A., et al., 2005. Limited Temporal Variability of Arsenic Concentrations in 20 Wells Monitored for 3 Years in Araihazar, Bangladesh. Environmental Science & Technology, 39(13): 4759-4766. doi: 10.1021/es048065f

Deng, Y.M., 2008. Geochemical Processes of High Arsenic Groundwater System at Western Hetao Basin (Dissertation). China University of Geosciences, Wuhan (in Chinese with English abstract).

Dhar, R.K., Zheng, Y., Stute, M., et al., 2008. Temporal Variability of Groundwater Chemistry in Shallow and Deep Aquifers of Araihazar, Bangladesh. Journal of Contaminant Hydrology, 99(1-4): 97-111. doi: 10.1016/j.jconhyd.2008.03.007

Farooq, S.H., Chandrasekharam, D., Berner, Z., et al., 2010. Influence of Traditional Agricultural Practices on Mobilization of Arsenic from Sediments to Groundwater in Bengal Delta. Water Research, 44(19): 5575-5588. doi: 10.1016/j.watres.2010.05.057

Fendorf, S., Michael, H.A., van Geen, A., 2010. Spatial and Temporal Variations of Groundwater Arsenic in South and Southeast Asia. Science, 328(5982): 1123-1127. doi: 10.1126/science.1172974

Gan, Y.Q., Wang, Y.X., Duan, Y.H., et al., 2014. Dynamic Changes of Groundwater Arsenic Concentration in the Monitoring Field Site, Jianghan Plain. Earth Science Frontiers, 21(4): 37-49 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-DXQY201404006.htm

Gan, Y.Q., Wang, Y.X., Duan, Y.H., et al., 2014. Hydrogeochemistry and Arsenic Contamination of Groundwater in the Jianghan Plain, Central China. Journal of Geochemical Exploration, 138: 81-93. doi: 10.1016/j.gexplo.2013.12.013

Gong, Z., Lu, X., Watt, C., et al., 2006. Speciation Analysis of Arsenic in Groundwater from Inner Mongolia with an Emphasis on Acid-Leachable Particulate Arsenic. Analytica Chimica Acta, 555(1): 181-187. doi: 10.1016/j.aca.2005.08.062

Guo, H.M., Guo, Q., Jia, Y.F., 2013. Chemical Characteristics and Geochemical Processes of High Arsenic Groundwater in Different Regions of China. Journal of Earth Sciences and Environment, 35(3): 83-96 (in Chinese with English abstract).

Guo, H.M., Guo, Q., Jia, Y.F., et al., 2013. Dynamic Behaviors of Water Levels and Arsenic Concentration in Shallow Groundwater from the Hetao Basin, Inner Mongolia. Journal of Geochemical Exploration, 135(SI): 130-140. doi: 10.1016/j.gexplo.2012.06.010

Guo, H.M., Yang, S.Z., Shen, Z.L., 2007. High Arsenic Groundwater in the World: Overview and Research Perspectives. Advances in Earth Science, 22(11): 1109-1117 (in Chinese with English abstract). http://www.researchgate.net/publication/281018109_High_arsenic_groundwater_in_the_world_Overview_and_research_perspectives

Guo, X.X., 2014. Hydrogeological Monitoring and Reactive Transport Modeling of Arsenic-Contaminated Aquifer System in Jianghan Plain, Central China (Dissertation). China University of Geosciences, Wuhan (in English with Chinese abstract).

Jia, Y.F., Guo, H.M., 2013. Hot Topics and Trends in the Study of High Arsenic Groudnwater. Advances in Earth Science, 28(1): 51-61 (in Chinese with English Abstract). http://www.researchgate.net/publication/308308294_Hot_topics_and_trends_in_studies_of_high_arsenic_groundwater

Kumar, A.R., Riyazuddin, P., 2012. Seasonal Variation of Redox Species and Redox Potentials in Shallow Groundwater: A Comparison of Measured and Calculated Redox Potentials. Journal of Hydrology, 444: 187-198. doi: 10.1016/j.jhydrol.2012.04.018

Larsen, M.A.D., Pham, N.Q., Dang, N.D., et al., 2008. Controlling Geological and Hydrogeological Processes in an Arsenic Contaminated Aquifer on the Red River Flood Plain, Vietnam. Applied Geochemistry, 23(11): 3099-3115. doi: 10.1016/j.apgeochem.2008.06.014

McArthur, J.M., Ravenscroft, P., Banerjee, D.M., et al., 2008. How Paleosols Influence Groundwater Flow and Arsenic Pollution: A Model from the Bengal Basin and Its Worldwide Implication. Water Resources Research, 44: W11411. doi: 10.1029/2007WR006552.

Munk, L., Hagedorn, B., Sjostrom, D., 2011. Seasonal Fluctuations and Mobility of Arsenic in Groundwater Resources, Anchorage, Alaska. Applied Geochemistry, 26(11): 1811-1817. doi: 10.1016/j.apgeochem.2011.06.005

Neumann, R.B., Ashfaque, K.N., Badruzzaman, A.B., et al., 2010. Anthropogenic Influences on Groundwater Arsenic Concentrations in Bangladesh. Nature Geoscience, 3(1): 46-52. doi: 10.1038/ngeo685

Nordstrom, D.K., 2002. Worldwide Occurrences of Arsenic in Groundwater. Science, 296(5576): 2143-2145. doi: 10.1126/science.1072375

Oinam, J.D., Ramanathan, A., Linda, A., et al., 2011. A Study of Arsenic, Iron and Other Dissolved Ion Variations in the Groundwater of Bishnupur District, Manipur, India. Environmental Science & Technology, 62(6): 1183-1195. doi: 10.1007/s12665-010-0607-2

Planer, F.B., Härtig, C., Lissner, H., et al., 2012. Organic Carbon Mobilization in a Bangladesh Aquifer Explained by Seasonal Monsoon-Driven Storativity Changes. Applied Geochemistry, 27(12): 2324-2334. doi: 10.1016/j.apgeochem.2012.08.005

Romi ć, Ž., Habuda-Stani ć, M., Kalajdži ć, B., et al., 2011. Arsenic Distribution, Concentration and Speciation in Groundwater of the Osijek Area, Eastern Croatia. Applied Geochemistry, 26(1): 37-44. doi: 10.1016/j.apgeochem.2010.10.013

Shen, Z.L., Guo, H.M., Xu, G., et al., 2010. Abnormal Groundwater Chemistry and Endemic Disease. Chinese Journal of Nature, 32(2): 83-89 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-ZRZZ201002006.htm

Shraim, A., Sekaran, N.C., Anuradha, C.D., et al., 2002. Speciation of Arsenic in Tube-Well Water Samples Collected from West Bengal, India, by High-Performance Liquid Chromatography-Inductively Coupled Plasma Mass Spectrometry. Applied Organometallic Chemistry, 16(4): 202-209. doi: 10.1002/aoc.279

Smedley, P.L., Kinniburgh, D.G., 2002. A Review of the Source, Behavior and Distribution of Arsenic in Natural Waters. Applied Geochemistry, 17(5): 517-568. doi: 10.1016/S0883-2927(02)00018-5

Waeles, M., Vandenhecke, J., Salaün, P., et al., 2013. External Sources vs Internal Processes: What Control Inorganic as Speciation and Concentrations in the Penzé Estuary. Journal of Marine Systems, 109-110(Suppl. ): 261-272. doi: 10.1016/j.jmarsys.2011.09.008

Wen, D.G., Zhang, F.C., Zhang, E.Y., et al., 2013. Arsenic, Fluoride and Iodine in Groundwater of China. Journal of Geochemical Exploration, 135(SI): 1-21. doi: 10.1016/j.gexplo.2013.10.012

Williams, M.D., Oostrom, M., 2000. Oxygenation of Anoxic Water in a Fluctuating Water Table System: An Experimental and Numerical Study. Journal of Hydrology, 230(1-2): 70-85. doi: 10.1016/S0022-1694(00)00172-4

Yu, Q., Xie, X.J., Ma, R., et al., 2013. Impact of Groundwater Flow on Arsenic Transport: A Field Observation and Simulation in Datong Basin. Earth Science—Journal of China University of Geosciences, 38(4): 877-886 (in Chinese with English abstract). doi: 10.3799/dqkx.2013.086

Zeng, Z.H., Cai, W.D., Zhang, Z.L., 2004. The Migration Enrichment of Mn Element in Groundwater and the Controlling Factor. Resources Environment & Engineering, 18(4): 39-42 (in Chinese with English abstract).

Zhang, F.C., Wen, D.G., Guo, J.Q., et al., 2010. Research Progress and Prospect of Geological Environment in Main Endemic Disease Area. Geology in China, 37(3): 551-562 (in Chinese with English abstract). http://www.researchgate.net/publication/284852910_Research_progress_and_prospect_of_geological_environment_in_main_endemic_disease_area

Zhao, D.J., 2005. The Three-Dimensional Numerical Simulation for Groundwater System in Jianghan Plain (Dissertation). China University of Geosciences, Wuhan (in Chinese with English abstract).

Zhao, S.J., Liu, G.L., Yang, B.X., et al., 2009. Screening Report on Endemic Arsenism and High Content of Arsenic in Xiantao City, Hubei Province. Chinese Journal of Endemiology, 28(1): 71-74 (in Chinese with English abstract). http://www.researchgate.net/publication/298258131_Screening_report_on_endemic_arsenism_and_high_content_of_arsenic_in_Xiantao_City_Hubei_Province

邓娅敏, 2008. 河套盆地西部高砷地下水系统中的地球化学过程研究(博士学位论文). 武汉: 中国地质大学.

甘义群, 王焰新, 段艳华, 等, 2014. 江汉平原高砷地下水监测场砷的动态变化特征分析. 地学前缘, 21(4): 37-49. https://www.cnki.com.cn/Article/CJFDTOTAL-DXQY201404006.htm

郭华明, 郭琦, 贾永锋, 等, 2013. 中国不同区域高砷地下水化学特征及形成过程. 地球科学与环境学报, 35(3): 83-96. doi: 10.3969/j.issn.1672-6561.2013.03.008

郭华明, 杨素珍, 沈照理, 2007. 富砷地下水研究进展. 地球科学进展, 22(11): 1109-1117. doi: 10.3321/j.issn:1001-8166.2007.11.002

郭欣欣, 2014. 江汉平原浅层含水层系统中砷释放与迁移过程研究(博士学位论文). 武汉: 中国地质大学.

贾永锋, 郭华明, 2013. 高砷地下水研究的热点及发展趋势. 地球科学进展, 28(1): 51-61. https://www.cnki.com.cn/Article/CJFDTOTAL-DXJZ201301007.htm

沈照理, 郭华明, 徐刚, 等, 2010. 地下水化学异常与地方病. 自然杂志, 32(2): 83-89. doi: 10.3969/j.issn.0253-9608.2010.02.006

余倩, 谢先军, 马瑞, 等, 2013. 地下水流动对砷迁移的影响: 大同盆地试验场的观测与模拟. 地球科学——中国地质大学学报, 38(4): 877-886. https://www.cnki.com.cn/Article/CJFDTOTAL-DQKX201304022.htm

曾昭华, 蔡伟娣, 张志良, 2004. 地下水中锰元素的迁移富集及其控制因素. 资源环境与工程, 18(4): 39-42. doi: 10.3969/j.issn.1671-1211.2004.04.008

张福存, 文东光, 郭建强, 等, 2010. 中国主要地方病区地质环境研究进展与展望. 中国地质, 37(3): 551-562. doi: 10.3969/j.issn.1000-3657.2010.03.002

赵德君, 2005. 江汉平原地下水系统三维数值模拟(硕士学位论文). 武汉: 中国地质大学.

赵淑军, 刘甘露, 杨宝霞, 等, 2009. 湖北省仙桃市饮水型地方性砷中毒病区和高砷区水砷筛查报告. 中国地方病学杂志, 28(1): 71-74.

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Seasonal Variation of Arsenic Speciation in Shallow Groundwater from Endemic Arsenicosis Area in Jianghan Plain

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