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| Citation: | Wang Miao, Wu Bailin, Li Yanqing, Liu Chiyang, Hao Xin, Liu Mingyi, Zhang Wanying, Li Qi, Yao Luhang, Zhang Xiaorui, 2022. Experimental Study on Possibility of Deep Uranium-Rich Source Rocks Providing Uranium Source in Ordos Basin. Earth Science, 47(1): 224-239. doi: 10.3799/dqkx.2021.050
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The high quality source rocks of the Chang 7 Member in Yanchang Formation of the Upper Triassic in the Ordos Basin are characterized by uranium enrichment, while the Jurassic-Cretaceous strata of the basin are famous for hosting a large number of sandstone-type uranium deposits. To analyze the possibility of source rocks providing uranium source for shallow sandstone type uranium deposits, the uranium-rich source rocks, oil samples from the Chang 7 Member and representative uranyl carbonate were selected as reactants, and simulation experiments of hydrocarbon generation and expulsion of uranium from source rocks and oil-uranium relationship were carried out respectively under the reduction conditions of medium-high temperature and high pressure. The results show that uranium can be discharged along with the process of hydrocarbon expulsion from source rock, and the increase of temperature and pressure at 30-200 ℃ and 2-5 MPa is conductive to the increase of hydrocarbon generation and uranium discharge. The discharged rate of uranium increases with the increase of hydrocarbon generation and is generally 55%-75%. Among them, the proportion of soluble uranium from itself is about 12%, and the discharged rate of uranium caused by the superposition of hydrocarbon generation is 43%-48%. The uranium migration forms found in this experiment are special, such as tetravalent (UO2), hexavalent (UO3), mixed valence (U3O8) and hydrate colloid form (UO3·H2O, U6O7(OH)2O), which are mainly adsorbed by low-temperature oil-gas fluid, and the uranium adsorption capacity shows an increasing trend with the increase of temperature and the decrease of pressure. Thus, it is beneficial for uranium ore formation when low temperature uranium-bearing oil-hydrothermal fluids migrate to shallow strata. Based on the above analyses, it is considered that the source rocks of Chang 7 Member in the southern Ordos Basin can release or discharge a large amount of uranium, which can be adsorbed by low-temperature oil-gas in the form of tetravalent, hexavalent and mixed valence. Subsequently, the adsorbed uranium moves upwards along with the oil-water fluid through the fracture, providing partial material source for the formation of shallow sandstone-type uranium deposits of the basin.
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