长江中游河湖平原浅层地下水中砷空间异质性的同位素指示

李典; 邓娅敏; 杜尧; 颜港归; 孙晓梁; 范红晨

doi:10.3799/dqkx.2021.054

Volume 46 Issue 12

Dec. 2021

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Article Navigation > Earth Science > 2021 > 46(12): 4492-4502

Li Dian, Deng Yamin, Du Yao, Yan Ganggui, Sun Xiaoliang, Fan Hongchen, 2021. Isotopic Indication of Spatial Heterogeneity of Arsenic in Shallow Groundwater of Middle Yangtze River Lacustrine Plain. Earth Science, 46(12): 4492-4502. doi: 10.3799/dqkx.2021.054

Citation:

Li Dian, Deng Yamin, Du Yao, Yan Ganggui, Sun Xiaoliang, Fan Hongchen, 2021. Isotopic Indication of Spatial Heterogeneity of Arsenic in Shallow Groundwater of Middle Yangtze River Lacustrine Plain. Earth Science, 46(12): 4492-4502. doi: 10.3799/dqkx.2021.054

Citation:

Li Dian, Deng Yamin, Du Yao, Yan Ganggui, Sun Xiaoliang, Fan Hongchen, 2021. Isotopic Indication of Spatial Heterogeneity of Arsenic in Shallow Groundwater of Middle Yangtze River Lacustrine Plain. Earth Science, 46(12): 4492-4502. doi: 10.3799/dqkx.2021.054

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Isotopic Indication of Spatial Heterogeneity of Arsenic in Shallow Groundwater of Middle Yangtze River Lacustrine Plain

doi: 10.3799/dqkx.2021.054

Li Dian^{1
,
,},
Deng Yamin^{2
,
,
,},
Du Yao²,
Yan Ganggui¹,
Sun Xiaoliang¹,
Fan Hongchen²

1.
Geological Survey of China University of Geosciences, Wuhan 430074, China
2.
School of Environmental Studies, China University of Geosciences, Wuhan 430078, China

Received Date: 2021-04-10
Publish Date: 2021-12-15

Abstract

Abstract

In recent years, it has been reported that high arsenic groundwater is widely distributed in the the middle Yangtze River lacustrine plain. The Poyang Lake plain (PYP) and the Jiangbei plain (ancient Pengli Lake, JBP) are typical lacustrine plains rich in groundwater resources on the northern and southern sides of the middle reach of the Yangtze River. However, the spatial distribution of groundwater arsenic in these regions has not been clearly studied, which posed potential risks to regional water supply security. In this study, 98 shallow groundwater samples and 8 surface water samples were collected in these two regions. The spatial heterogeneity of arsenic in groundwater and its controlling factors were identified by hydrochemistry and stable isotope analysis. The arsenic contents of shallow groundwater in JBP range from 0.65 to 956.72 μg/L (average 210.78 μg/L), and the high arsenic groundwater is mainly distributed in the ancient Yangtze River channel. The arsenic contents of shallow groundwater in PYP range from 0.09 to 267.45 μg/L (average 11.85 μg/L), and the high arsenic groundwater is only distributed in parts of Ganjiang River delta. Stable water isotope composition (δD and δ¹⁸O) of groundwater samples from the JBP is more negative and significantly different from surface water relative to the PYP. Multivariate statistical results of groundwater chemistry data indicate that the differences of provenance and aquifer structure are the key factors affecting arsenic spatial heterogeneity in shallow groundwater in PYP and JBP, the microbially mediated reductive dissolution of arsenic-bearing iron minerals leads to arsenic release in groundwater. Groundwater arsenic in the Jiangbei plain is supposed to be originated from the sediments from ancient Pengli area of Yangtze River provenance. The stable isotopic signatures of hydrogen and oxygen in groundwater indicate that the aquifer environment in JBP is closer and the groundwater circulation and alternation speed is slower compared with the PYP, which is more conducive to arsenic release and enrichment in the groundwater.
- groundwater,
- arsenic,
- hydrogen and oxygen stable isotopes,
- Poyang Lake plain,
- ancient Pengli Lake,
- geochemistry

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References(43)

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Isotopic Indication of Spatial Heterogeneity of Arsenic in Shallow Groundwater of Middle Yangtze River Lacustrine Plain

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