天山北麓中段绿洲带高砷地下水中砷的迁移转化规律

雷米; 周金龙; 周殷竹; 孙英; 韩双宝; 刘江涛; 鲁涵; 白凡; 闫志雲

doi:10.3799/dqkx.2022.349

Volume 49 Issue 1

Jan. 2024

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Article Navigation > Earth Science > 2024 > 49(1): 253-270

Lei Mi, Zhou Jinlong, Zhou Yinzhu, Sun Ying, Han Shuangbao, Liu Jiangtao, Lu Han, Bai Fan, Yan Zhiyun, 2024. Migration and Transformation Mechanism of High Arsenic Groundwater in Oasis Belt in Middle Part of Northern Piedmont of Tianshan Mountain. Earth Science, 49(1): 253-270. doi: 10.3799/dqkx.2022.349

Citation:

Lei Mi, Zhou Jinlong, Zhou Yinzhu, Sun Ying, Han Shuangbao, Liu Jiangtao, Lu Han, Bai Fan, Yan Zhiyun, 2024. Migration and Transformation Mechanism of High Arsenic Groundwater in Oasis Belt in Middle Part of Northern Piedmont of Tianshan Mountain. Earth Science, 49(1): 253-270. doi: 10.3799/dqkx.2022.349

Citation:

Lei Mi, Zhou Jinlong, Zhou Yinzhu, Sun Ying, Han Shuangbao, Liu Jiangtao, Lu Han, Bai Fan, Yan Zhiyun, 2024. Migration and Transformation Mechanism of High Arsenic Groundwater in Oasis Belt in Middle Part of Northern Piedmont of Tianshan Mountain. Earth Science, 49(1): 253-270. doi: 10.3799/dqkx.2022.349

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Migration and Transformation Mechanism of High Arsenic Groundwater in Oasis Belt in Middle Part of Northern Piedmont of Tianshan Mountain

doi: 10.3799/dqkx.2022.349

Lei Mi^{1, 2, 3
,
,},
Zhou Jinlong^{1, 2, 3
,
,
,},
Zhou Yinzhu⁴,
Sun Ying^{1, 2, 3},
Han Shuangbao⁴,
Liu Jiangtao⁴,
Lu Han^{1, 2, 3},
Bai Fan^{1, 2, 3},
Yan Zhiyun^{1, 2, 3}

1.
College of Water Conservancy and Civil Engineering, Xinjiang Agricultural University, Urumqi 830052, China
2.
Xinjiang Hydrology and Water Resources Engineering Research Center, Urumqi 830052, China
3.
Xinjiang Key Laboratory of Water Conservancy Engineering Safety and Water Disaster Prevention, Urumqi 830052, China
4.
Center for Hydrogeology and Environmental Geology, China Geological Survey, Baoding 071051, China

Received Date: 2022-06-16
Available Online: 2024-01-24
Publish Date: 2024-01-25

Abstract

Abstract

Junggar Basin is a typical inland basin with high arsenic groundwater distribution. Groundwater is an important drinking water source in the basin. Regional water supply safety is at risk. Migration and transformation of high arsenic groundwater need to be further investigated. In this study, the oasis belt in the middle part of the northern piedmont of Tianshan Mountain was taken as the research area. Semivariogram model and UNMIX source analysis model were used to analyze the distribution of arsenic in groundwater and the source contribution rate of groundwater chemical indexes, and influencing factors of arsenic migration. Transformation and enrichment in high arsenic groundwater in the typical profile were analyzed in combination with geological conditions, occurrence environment and hydrogeochemical action. Results show that groundwater in the study area is generally freshwater with weak alkaline and slightly reduced environment. Groundwater As concentration ranges between ND and 887.0 μg·L^-1, with an average of 11.2 μg·L^-1. Hydrochemical types of high arsenic groundwater (ρ (As) > 10 μg·L^-1) are mainly HCO₃·SO₄·Cl⁃Na (HSL⁃N) and HCO₃·SO₄⁃Na (Na·Ca) (HS⁃N (NC)) types. Proportions of high arsenic groundwater in single-structure phreatic water, phreatic water in confined water area, and confined water are 0.4%, 6.4%, and 18.6%, respectively. Contribution rates of native mineral source, rock salt mineral source, soil input-human emission source, sulfuric-carbonate mineral source and environmental source to groundwater hydrochemical indexes are 11.3%, 21.1%, 23.1%, 23.4% and 21.1%, respectively. Arsenic species in 24 groups of a total of 25 groundwater samples of typical profiles is only As (Ⅴ) (96.0% of the sampling sites). From piedmont plain to alluvial plain, along groundwater flow, the variation trend of groundwater total arsenic concentration firstly increased and then decreased. Arsenic enrichment in occurrence environment is affected by groundwater hydrochemical indexes including pH, Eh, HCO₃^- and PO₄^3-, which is also related to geological, hydrogeological conditions, organic matter degradation, and dissolution.
- high arsenic groundwater,
- spatial distribution,
- source apportionment,
- migration and transformation,
- hydrogeology

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Migration and Transformation Mechanism of High Arsenic Groundwater in Oasis Belt in Middle Part of Northern Piedmont of Tianshan Mountain

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