胶州湾北部表层沉积物重金属污染及DOM对其环境行为的影响

安洋; 周松; 苏春利; 王烁一; 张旭; 吕金桥

doi:10.3799/dqkx.2023.039

Volume 49 Issue 8

Aug. 2024

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An Yang, Zhou Song, Su Chunli, Wang Shuoyi, Zhang Xu, Lv Jinqiao, 2024. Heavy Metal Pollution of Sediments in Northern Jiaozhou Bay and the Influence of DOM on Their Environmental Behavior. Earth Science, 49(8): 2901-2913. doi: 10.3799/dqkx.2023.039

Citation:

An Yang, Zhou Song, Su Chunli, Wang Shuoyi, Zhang Xu, Lv Jinqiao, 2024. Heavy Metal Pollution of Sediments in Northern Jiaozhou Bay and the Influence of DOM on Their Environmental Behavior. Earth Science, 49(8): 2901-2913. doi: 10.3799/dqkx.2023.039

Citation:

An Yang, Zhou Song, Su Chunli, Wang Shuoyi, Zhang Xu, Lv Jinqiao, 2024. Heavy Metal Pollution of Sediments in Northern Jiaozhou Bay and the Influence of DOM on Their Environmental Behavior. Earth Science, 49(8): 2901-2913. doi: 10.3799/dqkx.2023.039

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Heavy Metal Pollution of Sediments in Northern Jiaozhou Bay and the Influence of DOM on Their Environmental Behavior

doi: 10.3799/dqkx.2023.039

An Yang^{1
,
,},
Zhou Song²,
Su Chunli^{1
,
,},
Wang Shuoyi¹,
Zhang Xu¹,
Lv Jinqiao³

1.
School of Environmental Studies, China University of Geosciences, Wuhan 430074, China
2.
Qingdao National High-Tech Industrial Development Zone Development Dept., Qingdao 266000, China
3.
Qingdao High-Tech Investment Promotion Group Co., Ltd. Qingdao 266109, China

Received Date: 2023-01-22
Available Online: 2024-08-27
Publish Date: 2024-08-25

Abstract

Abstract

Coastal zone sediments are the main carriers and destinations for the migration and transformation of pollutants. Dissolved organic matter (DOM), as an important medium for heavy metal migration in the environment, plays an important role in controlling the distribution and migration of heavy metals in sediments. The paper used the factor index and ground accumulation index methods to assess the current pollution status of five heavy metals, Cr, Cu, Zn, As and Pb, in the Surface sediment of the northern coastal zone of Jiaozhou Bay, and combined with three-dimensional fluorescence spectroscopy to analyze the spatial partitioning patterns of different DOM components in sediments, to explore the relationship between DOM composition and heavy metal migration behavior in the Surface sediment of the northern Jiaozhou Bay area. The results showed that the overall heavy metals in the coastal zone sediments were lightly contaminated; the natural DOM fractions in the sediments included four types of terrestrial fulvic acid (C1), terrestrial humic substances (C2), microbial-derived humic substances (C3) and tryptophan-like (C4), and the proportion of humic acid fractions was significantly higher than that of protein-like fractions in the whole area, and their sources were influenced by both terrestrial input and biological metabolism. Each heavy metal may have similar pollution sources, but different migration mechanisms cause differences in their distribution; C1 promotes the natural migration of Cr, each DOM fraction influences the distribution of heavy metals in sediments through different adsorption complexation mechanisms, and there are certain mutual transformation processes among DOM fractions.
- Northern Jiaozhou Bay,
- heavy metals,
- risk assessment,
- DOM,
- fluorescence index,
- environmental geology

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Heavy Metal Pollution of Sediments in Northern Jiaozhou Bay and the Influence of DOM on Their Environmental Behavior

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