地表水-地下水相互作用下NH<sub>4</sub>-N的吸附/解吸行为及其对N迁移转化的影响

张安广; 梁莹; 马瑞

doi:10.3799/dqkx.2023.188

Volume 49 Issue 10

Oct. 2024

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Zhang Anguang, Liang Ying, Ma Rui, 2024. Adsorption/Desorption Behavior of NH4-N under Surface Water-Groundwater Interaction and Its Impact on N Migration and Transformation. Earth Science, 49(10): 3761-3772. doi: 10.3799/dqkx.2023.188

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Zhang Anguang, Liang Ying, Ma Rui, 2024. Adsorption/Desorption Behavior of NH₄-N under Surface Water-Groundwater Interaction and Its Impact on N Migration and Transformation. Earth Science, 49(10): 3761-3772. doi: 10.3799/dqkx.2023.188

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Adsorption/Desorption Behavior of NH₄-N under Surface Water-Groundwater Interaction and Its Impact on N Migration and Transformation

doi: 10.3799/dqkx.2023.188

School of Environmental Studies, China University of Geosciences, Wuhan 430078, China

Received Date: 2023-07-24
Available Online: 2024-11-08
Publish Date: 2024-10-25

Abstract

Abstract

The migration and transformation of NH₄-N are influenced by the interactions between surface water and groundwater. However, the mechanisms remain poorly understood. Continuous monitoring of the water level and its hydrochemical composition was conducted in the Shahu site. Column experiments and reactive transport modeling were applied to identify the migration and transformation of NH₄-N under conditions of both surface water recharge and groundwater discharge. In this study it indicates that most injected NH₄-N is adsorbed on shallow sediment. Infiltration of surface water enhances desorption of NH₄-N from sediment particle and subsequent nitrification reactions. In contrast, adsorption of NH₄-N on sediment is favored during discharge of NH₄-N containing groundwater. Simulating results emphasize the crucial role of cation exchange in NH₄-N mobility. Alterations in the hydrogeochemical environment during surface water-groundwater interactions impact the NH₄-N adsorption/desorption behaviors and associated biogeochemical reactions.
- ammonium nitrogen,
- ion exchange,
- reactive transport modeling,
- surface water,
- groundwater,
- Jianghan Plain,
- hydrogeology

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References(41)

References

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Adsorption/Desorption Behavior of NH4-N under Surface Water-Groundwater Interaction and Its Impact on N Migration and Transformation

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Adsorption/Desorption Behavior of NH₄-N under Surface Water-Groundwater Interaction and Its Impact on N Migration and Transformation