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    中国百强科技报刊

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    中国高校百佳科技期刊

    中国最美期刊

    Volume 33 Issue 1
    Jan.  2008
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    Article Contents
    XIE Xian-jun, WANG Yan-xin, SU Chun-li, LIU Huai-qing, DUAN Meng-yu, ZHANG Hong-da, 2008. Environmental Magnetic Properties of Sediments of High Arsenic Groundwater System, Datong Basin. Earth Science, 33(1): 117-123.
    Citation: XIE Xian-jun, WANG Yan-xin, SU Chun-li, LIU Huai-qing, DUAN Meng-yu, ZHANG Hong-da, 2008. Environmental Magnetic Properties of Sediments of High Arsenic Groundwater System, Datong Basin. Earth Science, 33(1): 117-123.

    Environmental Magnetic Properties of Sediments of High Arsenic Groundwater System, Datong Basin

    • Received Date: 2007-03-26
    • Publish Date: 2008-02-25
    • The purpose of the study is to test the possible relationship between magnetic parameters and arsenic in high arsenic aquifer sediment. Magnetic and geochemical study on core sediments from Datong basin suggests that the dominant magnetic mineral is ferrimagnetic. Magnetic measurements and arsenic concentration analysis were carried out to understand the distribution characteristics of magnetic parameters and arsenic in sediments. All core samples with high arsenic content have low saturation isothermal remnant magnetism (SIRM) values, indicating the correlation between arsenic and paramagnetic mineral. The correlation factors between arsenic content and magnetic parameters are very low (R2 < 0.5, α=0.05), but the magnetic susceptibility (χ) is better correlated than the other magnetic parameters with correlation factor of about 0.4 (α=0.05). The low correlation between magnetic proxies and arsenic content is attributed to the dilution of paramagnetic minerals by the ferrimagnetic and anti-ferromagnetic minerals. The occurrence of As-rich groundwater in this region may be due to dissolution of As-bearing Fe mineral (e.g. γFeOOH, 5Fe2O3·9H2O) and subsequent arsenic release.

       

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    • Akai, J., Izumi, K., Fukuhara, H., et al., 2004. Mineralogical and geomicrobiological investigations on groundwater arsenic enrichment in Bangladesh. Applied Geochemistry, 19: 215-230. doi: 10.1016/j.apgeochem.2003.09.008
      Anawar, H. M., Akai, J., Komaki, K., et al., 2003. Geochemical occurrences of arsenic in groundwater of Bangladesh: Sources and mobilisation processes. Journal of Geochemical Exploration, 77: 109-131. doi: 10.1016/S0375-6742(02)00273-X
      Berg, M., Tran, H. C., Nguyen, T. C., et al., 2001. Arsenic contamination of groundwater and drinking water in Vietnam: A human health threat. Environmental Science and Technology, 35: 2621-2626. doi: 10.1021/es010027y
      Bhattacharyya, R., Chatterjee, D., Nath, B., et al., 2003. High arsenic groundwater: Mobilization, metabolism and mitigation—An overviewin the Bengal delta plain. Molecular and Cellular Biochemistry, 253: 347-355. doi: 10.1023/A:1026001024578
      Das, D., Samanta, C., Mandal, B. K., et al., 1996. Arsenic ingroundwater in districts of West Bengal, India. Environmental Geochemistry and Health, 18: 5-15. doi: 10.1007/BF01757214
      Dowling, C. B., Poreda, R. J., Basu, A. R., et al., 2002. Geochemical study of arsenic release mechanisms in theBengal basin groundwater. Water Resources Research, 38: 1-18.
      Guo, H. M., Wang, Y. X., Li, Y. M., 2003. Analysis of factor resulting in anomalous arsenic concentration ingroundwater of Shanyin, Shanxi Province. Environmental Science, 24 (4): 60-67 (in Chinese with English abstract).
      Harvey, C. F., Swartz, C. H., Badruzzaman, A. B. M., et al., 2002. Arsenic mobility and groundwater extraction inBangladesh. Science, 298: 1602-1606. doi: 10.1126/science.1076978
      Harvey, C. F., Swartz, C. H., Badruzzaman, A. B. M., et al., 2005. Groundwater arsenic contaminationin the Gangesdelta: Biogeochemistry, hydrology, human perturbations and human suffering on a large scale. Comptus Rendus Geoscience, 337: 285-296.
      Horneman, A., Van Geen, A., Kent, D. V., et al., 2004. Decoupling of As and Fe release to Bangladesh groundwater under reducing conditions. Part Ⅰ: Evidence fromsediment profiles. Geochimica et Cosmochimica Acta, 68: 3459-3473. doi: 10.1016/j.gca.2004.01.026
      Islam, F. S., Gault, A. G., Boothman, C., et al., 2004. Directevidence of arsenic release from Bengal sediments mediated by indigenous metalreducing bacteria. Nature, 430: 68-71. doi: 10.1038/nature02638
      Klump, S., Kipfer, R., Cirpka, O. A., et al., 2006. Groundwater dynamics and arsenic mobilization in Bangladesh assessed using noble gases and tritium. Environmental Science and Technology, 40: 243-250. doi: 10.1021/es051284w
      McArthur, J. M., Banerjee, D. M., Hudson-Edwards, K. A., et al., 2004. Natural organic matter in sedimentary basins and its relation to arsenic in anoxic groundwater: The example of West Bengal and its worldwide implications. Applied Geochemistry, 19: 1255-1293. doi: 10.1016/j.apgeochem.2004.02.001
      McArthur, J. M., Ravenscroft, P., Safiullah, S., et al., 2001. Arsenic in groundwater: Testing pollution mechanismsfor sedimentary aquifers in Bangladesh. Water Resources Research, 37: 109-117. doi: 10.1029/2000WR900270
      Nickson, R. T., McArthur, J. M., Burgess, W. G., et al., 1998. Arsenic poisoning of Bangladesh groundwater. Nature, 395: 338. doi: 10.1038/26387
      Nickson, R. T., McArthur, J. M., Ravenscroft, P., et al., 2000. Mechanism of arsenic release to groundwater, Bangladesh and West Bengal. Applied Geochemistry, 15: 403-413. doi: 10.1016/S0883-2927(99)00086-4
      Polya, D. A., Gault, A. G., Bourne, N. J., et al., 2003. Coupled HPLC-ICP-MS analysis indicates highly hazardous concentrations of dissolved arsenic species are present inCambodian well waters. Royal Society of Chemistry Special Publication, 288: 127-140.
      Polya, D. A., Gault, A. G., Diebe, N., et al., 2005. Arsenichazard in shallow Cambodian groundwaters. Mineralogical Magazine, 69: 807-823. doi: 10.1180/0026461056950290
      Shen, M. J., Hu, S. Y., Blaha, U., et al, 2006. Magnetic responses to heavy metal pollution and its statistic significance for site722soil vertical profile in eastern Beijing. Earth Science—Journal of University of Geosciences, 31 (3): 399-404 (in Chinese with English abstract).
      Smedley, P. L., Kinniburgh, D. G., 2002. A review of thesource, behaviour and distribution of arsenic in naturalwaters. Applied Geochemistry, 17: 517-568. doi: 10.1016/S0883-2927(02)00018-5
      Smedley, P. L., Zhang, M., Zhang, G., et al., 2003. Mobilisation of arsenic and other trace elements in fluviolacustrine aquifers of the Huhhot basin, Inner Mongolia. Applied Geochemistry, 18: 1453-1477. doi: 10.1016/S0883-2927(03)00062-3
      Smith, A. H., Lingas, E. O., Rahman, M., 2000. Contamination of drinking-water by arsenic in Bangladesh: A public health emergency. Bulletin of the World Health Organisation, 78: 1093-1103.
      Su, C. L., 2006. Regional hydrogeochemistry and genesis of high arsenic groundwater at Datong basin, Shanxi Province, China[Dissertation]. China University of Geosciences, Wuhan (in Chinese with English abstract).
      Swartz, C. H., Blute, N. K., Badruzzman, B., et al., 2004. Mobility of arsenic in a Bangladesh aquifer: Inferences from geochemical profiles, leaching data and mineralogical characterisation. Geochimica et Cosmochimica Acta, 68: 4539-4557. doi: 10.1016/j.gca.2004.04.020
      Thompson, R., OldFeld, F., 1986. Environmental magnetism. Allen and Unwin, London, 1-227.
      US EPA., 2001. Method200.9: Trace elements in water, solids and biosolids by stabilized temperature graphite furnace atomic absorption spectrometry. EPA-821-R-01-011, U. S. A. .
      Wang, J. H., Zhao, L. S., Wu, Y. B., 1998. Environmental geochemical study on arsenic in arseniasis areas in Shanyin and Yingxian, Shanxi Province. Geoscience, 12 (2): 243-248 (in Chinese with English abstract).
      Wang, X. S., Qin, Y., 2006. Relation between sulfur and magnetic parameters in Xuzhou urban topsoils and itsenvironmental significance. Environmental Herald, 24 (7): 48-50 (in Chinese with English abstract).
      World Health Organization (WHO), 1996. Guidelines fordrinking water quality., 2nd ed., Health criteria and other supporting information, vol. 2., Geneva, Switzerland.
      Zhang, W. G., Yu, L. Z., 2002. Relationship between granularity and magnetic properties in intertidal sediments of the Yangtze Estuary, China. Science in China (Seri. D), 32 (9): 783-792 (in Chinese).
      Zhang, W. G., Yu, L. Z., Lu, M., 2003. Relationship betweeniron oxides and magnetic properties in intertidal sediments of the Yangtze Estuary, China. Chinese Journal of Geophysics, 46 (1): 79-85 (in Chinese with Englishabstract).
      Zheng, Y., Stute, M., Van Geen, A., et al., 2004. Redoxcontrol of arsenic mobilisationin Bangladesh groundwater. Applied Geochemistry, 19: 201-214. doi: 10.1016/j.apgeochem.2003.09.007
      郭华明, 王焰新, 李永敏, 2003. 山阴水砷中毒区地下水砷的富集因素分析. 环境科学, 24 (4): 60-67. https://www.cnki.com.cn/Article/CJFDTOTAL-HJKZ200304010.htm
      沈明洁, 胡守云, Blaha, U., 等, 2006. 北京西郊722土壤垂向剖面重金属污染的磁学响应及其统计意义. 地球科学——中国地质大学学报, 31 (3): 399-404. https://www.cnki.com.cn/Article/CJFDTOTAL-DQKX200603018.htm
      苏春利, 2006. 大同盆地区域水文地球化学与高砷地下水成因研究[博士学位论文]. 武汉: 中国地质大学.
      王敬华, 赵伦山, 吴悦斌, 1998. 山西山阴、应县一带砷中毒区砷的环境地球化学研究. 现代地质, 12 (2): 243-248. https://www.cnki.com.cn/Article/CJFDTOTAL-XDDZ802.014.htm
      王学松, 秦勇, 2006. 徐州城市表层土壤中硫与环境磁学参数的关系及其环境意义. 环境导报, 24 (7): 48-50. https://www.cnki.com.cn/Article/CJFDTOTAL-KJDB200607019.htm
      张卫国, 愈立中, 2002. 长江口潮滩沉积物的磁学性质及其与粒度的关系. 中国科学(D辑), 32 (9): 783-792. https://www.cnki.com.cn/Article/CJFDTOTAL-JDXK200209009.htm
      张卫国, 愈立中, 陆敏, 2003. 长江口潮滩沉积物氧化铁与磁性特征和的关系. 地球物理学报, 46 (1): 79-85. doi: 10.3321/j.issn:0001-5733.2003.01.013
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