江汉平原典型地区季节性水文条件影响下氮的动态变化规律

沈帅; 马腾; 杜尧; 邓娅敏; 於昊天; 罗可文

doi:10.3799/dqkx.2017.055

Volume 42 Issue 5

May 2017

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Article Navigation > Earth Science > 2017 > 42(5): 674-684

Shen Shuai, Ma Teng, Du Yao, Deng Yamin, Yu Haotian, Luo Kewen, 2017. Dynamic Variations of Nitrogen in Groundwater under Influence of Seasonal Hydrological Condition in Typical Area of Jianghan Plain. Earth Science, 42(5): 674-684. doi: 10.3799/dqkx.2017.055

Citation:

Shen Shuai, Ma Teng, Du Yao, Deng Yamin, Yu Haotian, Luo Kewen, 2017. Dynamic Variations of Nitrogen in Groundwater under Influence of Seasonal Hydrological Condition in Typical Area of Jianghan Plain. Earth Science, 42(5): 674-684. doi: 10.3799/dqkx.2017.055

Citation:

Shen Shuai, Ma Teng, Du Yao, Deng Yamin, Yu Haotian, Luo Kewen, 2017. Dynamic Variations of Nitrogen in Groundwater under Influence of Seasonal Hydrological Condition in Typical Area of Jianghan Plain. Earth Science, 42(5): 674-684. doi: 10.3799/dqkx.2017.055

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Dynamic Variations of Nitrogen in Groundwater under Influence of Seasonal Hydrological Condition in Typical Area of Jianghan Plain

doi: 10.3799/dqkx.2017.055

Shen Shuai^{1,2
,},
Ma Teng^{1,2
,
,},
Du Yao^1,2,
Deng Yamin³,
Yu Haotian^1,2,
Luo Kewen^1,2

1.
School of Environmental Studies, China University of Geosciences, Wuhan 430074, China
2.
State Key Laboratory of Biogeology and Environmental Geology, China University of Geosciences, Wuhan 430074, China
3.
Geological Survey, China University of Geosciences, Wuhan 430074, China

Received Date: 2017-01-20
Publish Date: 2017-05-15

Abstract

Abstract

The pollution of NO₃^--N and NH₃-N in groundwater is very serious in the eastern of Jianghan plain, which is characterized by strong interactions between groundwater and surface water and obvious variations of seasonal hydrological condition. Sediment samples along vertical profiles of three boreholes and groundwater samples with different depths in different seasons were sampled to analyze the nitrogen speciation coupled with supporting chemistry in a typical field site. The results show that NO₃^--N with concentrations from 25.8 to 119.48 mg/kg is a dominant speciation of the total exchangeable nitrogen in sediments. The NH₃-N concentrations have a good positive correlation with TOC and TN contents in sediments, implying NH₃-N was mainly influenced by organic matter. The concentration and speciation of nitrogen in the groundwater deeper than 2 m show a significant response to the fluctuation of groundwater level. During the monsoon season, groundwater level increased, enhancing the reducing potential of aquifer media. As a result, NO₃^--N was not liable to be produced and was more likely to be consumed by denitrification. At the same time, with the mineralization enhanced, NH₃-N was gradually becoming the main speciation of dissolved inorganic nitrogen. After the monsoon season, groundwater level declined, enhancing the oxidizing potential of aquifer media.As a result, nitrification was enhanced and denitrification was limited, and the concentration of NO₃^--N increased.Anthropogenic activities near the surface had a significant effect on the concentration and speciation of nitrogen in the groundwater shallower than 2 m. In summary, under the coupled influence of natural and anthropogenic factors, seasonal hydrological change resulted in the variation of redox potential, which was the main trigger for seasonal variation of nitrogen concentration and speciation in the groundwater.
- Jianghan plain,
- three-nitrogen,
- seasonal variation,
- groundwater,
- migration and transformation,
- hydrogeology

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Dynamic Variations of Nitrogen in Groundwater under Influence of Seasonal Hydrological Condition in Typical Area of Jianghan Plain

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