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    Volume 48 Issue 3
    Mar.  2023
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    Article Navigation >  Earth Science  > 2023  >  48(3): 1217-1231
    Wang Qiuxia, Ping Xianquan, Zheng Jianping, Dai Hongkun, 2023. Mineral Ferric Iron Contents of Peridotite Xenoliths by Mössbauer Spectroscopy: Oxygen Fugacity Applications. Earth Science, 48(3): 1217-1231. doi: 10.3799/dqkx.2022.354
    Citation: Wang Qiuxia, Ping Xianquan, Zheng Jianping, Dai Hongkun, 2023. Mineral Ferric Iron Contents of Peridotite Xenoliths by Mössbauer Spectroscopy: Oxygen Fugacity Applications. Earth Science, 48(3): 1217-1231. doi: 10.3799/dqkx.2022.354
    shu

    Mineral Ferric Iron Contents of Peridotite Xenoliths by Mössbauer Spectroscopy: Oxygen Fugacity Applications

    doi: 10.3799/dqkx.2022.354
    • 1.

      School of Earth Sciences, China University of Geosciences, Wuhan 430074, China

    • 2.

      State Key Laboratory of Geological Processes and Mineral Resources, China University of Geosciences, Wuhan 430074, China

    • Received Date: 2022-06-02
      Available Online: 2023-03-27
    • Publish Date: 2023-03-25
      Abstract
    • The redox state of the lithospheric mantle can be estimated by well equilibrated mineral pairs of mantle peridotite xenoliths. Here we explore the mantle redox state of the northwest North China Craton by measuring the mineral Fe3+/∑Fe of the Langshan spinel lherzolite xenoliths using the newly established lab of WSS-10 Mössbauer spectroscopy at China University of Geosciences (Wuhan). The results show that the Fe3+/∑Fe ratios are 0.05-0.11 for orthopyroxene, 0.16-0.25 for clinopyroxene, 0.16-0.22 for spinel, and no Fe3+ was confirmed in olivine. The corresponding mantle oxygen fugacity using the olivine-orthopyroxene-spinel oxy-barometry is FMQ-0.82 to FMQ-0.39 (averaged at FMQ-0.65), slightly higher than the estimates using electron microprobe data (FMQ-1.49 to FMQ-0.8, averaged at FMQ-1.25). This discrepancy may be explained by the non-stoichiometry Fe3+ excess and cation vacancies in the spinel lattice, which is generally ignored in the stoichinometric calculation using electron microprobe data. Compared with global cratonic mantle (averaged at FMQ-0.35), the lithospheric mantle underneath the northwest North China Craton, represent by Langshan mantle xenoliths, is relatively reduced, and likely results from metasomatism by low-fO2 melts from deeper mantle domains.

       

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