• 中国出版政府奖提名奖

    中国百强科技报刊

    湖北出版政府奖

    中国高校百佳科技期刊

    中国最美期刊

    Volume 29 Issue 2
    Mar.  2004
    Turn off MathJax
    Article Contents
    QIU Dong-sheng, ZHUANG Da-fang, HU Yun-feng, YAO Rui, 2004. Estimation of Carbon Sink Capacity Caused by Rock Weathering in China. Earth Science, 29(2): 177-182.
    Citation: QIU Dong-sheng, ZHUANG Da-fang, HU Yun-feng, YAO Rui, 2004. Estimation of Carbon Sink Capacity Caused by Rock Weathering in China. Earth Science, 29(2): 177-182.

    Estimation of Carbon Sink Capacity Caused by Rock Weathering in China

    • Received Date: 2003-07-16
    • Publish Date: 2004-03-25
    • Rock weathering caused by the carbonic acid reaction with minerals to produce dissolved bicarbonates carried by rivers to the oceans is an important part in carbon cycle. The process causes significant carbon dioxide consumption, the accurate calculation of which may partly explain the missing sink of carbon. The CO2 uptaken by carbonate dissolution on the continents is counterbalanced by the CO2 release carbonate precipitation in the ocean. The same is not true for silicate weathering. Silicate weathering is more important than carbonate weathering as a long-term control on atmospheric CO2. A global erosion model (GEM-CO2) developed by Amiotte Suchet allows us to calculate the flux of atmospheric/soil CO2 consumed by chemical erosion of continental rocks. In this paper, the CO2 consumption by rock weathering in China is estimated based on GEM-CO2 and the Chinese Resources and Environment Database, whose distribution is shown in a GRID map with a spatial resolution of 1 000 m×1 000 m. The total carbon consumption is about 4.72×107 t/a, about 52.65% of which are caused by carbonate. The model results are close to previous estimation of other researches. The flux of CO2 consumed by rock weathering increases where carbonate rock outcrops are more abundant and when drainage intensity increases. The results show that the main consumption of CO2 is localized in Guangxi, Guizhou and Chongqing provinces, and west Hubei Province and southwest Hunan Province, because of a high proportion of carbonate rocks and high humidity in a large area.

       

    • loading
    • Amiotte, S., Probst J. L., 1993. Flux de CO2 consommé par altération chimique continentale: Influences du drainage et de la lithologie. C. R. Acad. Sci. Paris, 317: 615-622.
      Berner, R. A., 1991. A model for atmospheric CO2 over Phanerozoic time. Amer. J. Sci. , 291: 339-376. doi: 10.2475/ajs.291.4.339
      Berner, R. A., 1997. Weathering, plants and the long-term carbon cycle. Geochimica et Cosmochimica Acta, 56: 3225-3231.
      Dreybrodt, W., Buhmann, D., 1991. A mass transfer model for dissolution and precipitation of calcite from solutions in turbulent motion. Chemical Geology, 90: 107-122. doi: 10.1016/0009-2541(91)90037-R
      Dreybrodt, W., Buhmann, D., Michaelis, J., et al., 1992. Geochemically controlled calcite precipitation by CO2 outgassing: Field measurements of precipitation rates in comparison to theoretical predictions. Chem. Geol. , 97: 285-294. doi: 10.1016/0009-2541(92)90082-G
      Franke, H. W., 1975. Correspondence between sintering and corrosion. Ann. Spélé, 30: 4665-4675.
      Indermuhle, A., Monnin, E., Stauffer, B., et al., 2000. Atmospheric CO2 concentration from 60 to 20 kyrBP from the Taylor Dome ice core, Antarctica. Geophysical Research Letters, 27: 735-738. doi: 10.1029/1999GL010960
      Kennedy, D., 2001. Breakthrough of the year. Science, 294: 2443-2447.
      Li, J. Z., Lin, J. S., Fang, J. F., 1994. Analysis and estimation of the karst solutional intensity. Geographical Research, 13(3): 90-97 (in Chinese with English abstract).
      Liu, Z. H., 2000. Contribution of carbonate rock weathering to the atmosphere CO2 sink. Carsologica Sinica, 19(4): 293-300 (in Chinese with English abstract). doi: 10.1007/s002549900072
      Mahlman, J. D., 1997. Uncertainties in projections of human-caused climate warming. Science, 21(278): 1416-1417.
      Probst, J. L., Amiotte, S. P., Tardy, Y., 1992. Global continental erosion and fluctuations of atmospheric CO2 consumed during the last 100 years. In: Kharaka, Y. K., Maest, A., eds., Proc. 7th Int. Symp. W. R. I., Park City, Utah, U. S. A., July 13-18, 1992. Balkema, Rotterdam, 483-486.
      Schimel, D., House, J., Hibbard, K., et al., 2001. Recent patterns and mechanisms of carbon exchange by terrestrial ecosystems. Nature, 414: 169-172. doi: 10.1038/35102500
      Steven, C. W., 2001. Climate change enhanced: Where has all the carbon gone? Science, 292: 2261-2263. doi: 10.1126/science.1061077
      Wang, M. X., 1998. Global carbon cycle. In: Chen, S. P., ed., Geosystem science—Chinese progresses and century prospects. Chinese Science & Technology Press, Beijing, 780(in Chinese).
      White, W. B., 1977. Role of solution kinetics in the development of karst aquifers. In: Tolson, J. S., Doyle, F. L., eds., Karst hydrology. Intern. Assoc. Hydrogeol. Memoir, 12: 503-517.
      Wigley, T. M. L., Schimel, D. S., 2000. The carbon cycle. Cambridge University Press, Cambridge, 9-10.
      Xu, S. Y., Jiang, Z. C., 1997. Preliminary assessment of the source-sink relationship between karst process and atmospheric green house gases. Chinese Science Bulletin, 42(9): 953-955 (in Chinese). doi: 10.1360/csb1997-42-9-953
      Yuan, D., 1997. The carbon cycle in karst. Z. Geomorph. N. F. , 108: 91-102.
      李钜章, 林钧枢, 房金福, 1994. 喀斯特溶蚀强度分析与估算. 地理研究, 13(3): 90-97. doi: 10.3321/j.issn:1000-0585.1994.03.011
      刘再华, 2000. 碳酸盐岩岩溶作用对大气CO2沉降的贡献. 中国岩溶, 19(4): 293-300. doi: 10.3969/j.issn.1001-4810.2000.04.001
      王明星, 1998. 全球碳循环. 见: 陈述彭. 地球系统科学——中国进展与世纪展望. 北京: 中国科学技术出版社, 780.
      徐胜友, 蒋忠诚, 1997. 我国岩溶作用与大气温室气体CO2源汇关系的初步估算. 科学通报, 42(9): 953-955. doi: 10.3321/j.issn:0023-074X.1997.09.019
    • 加载中

    Catalog

      通讯作者: 陈斌, bchen63@163.com
      • 1. 

        沈阳化工大学材料科学与工程学院 沈阳 110142

      1. 本站搜索
      2. 百度学术搜索
      3. 万方数据库搜索
      4. CNKI搜索

      Figures(1)  / Tables(3)

      Article views (5001) PDF downloads(48) Cited by()
      Proportional views

      /

      DownLoad:  Full-Size Img  PowerPoint
      Return
      Return