Research Progress and Applications of High⁃Temperature Barium Isotope Geochemistry
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摘要:
过去十余年，钡（Ba）同位素的地球化学研究取得了显著进展，并在示踪壳幔相互作用、俯冲带物质迁移及循环、花岗岩演化、岩浆热液流体及成矿作用、海洋生产力等方面显示出突出的应用潜力.本文系统综述了当前高温地质过程Ba同位素研究进展.已有研究初步查明不同地质储库的Ba同位素变化范围，显示不同来源的表壳物质（沉积物、蚀变洋壳等）的Ba同位素组成与亏损地幔存在差异.基于理论计算、实验研究和地质样品的观测，显示高温平衡条件下含Ba矿物之间的Ba同位素分馏有限，而含水矿物变质脱水、岩浆热液流体出溶、流体岩石反应过程会产生显著的Ba同位素分馏.最后介绍了应用Ba同位素探究表壳物质再循环和花岗岩演化及成矿的研究进展和实例，显示了Ba同位素示踪高温地质过程的应用潜力.
Abstract:Significant advances have been made in the geochemical study of barium (Ba) isotopes over the past decades, demonstrating considerable potential for their application in tracing crust-mantle interactions, crust recycling in subduction zones, granite differentiation, magmatic-hydrothermal fluids and mineralization processes, as well as marine productivity. This paper systematically reviews the current progress in Ba isotope studies related to high-temperature geological processes. Recent research has preliminarily established the range of Ba isotope variations in different geological reservoirs, revealing distinct Ba isotopic compositions between crustal materials of various origins (such as sediments and altered oceanic crust) and the depleted mantle. Theoretical calculations, experimental studies, and observations from geological samples indicate that Ba isotope fractionation among Ba-bearing minerals is limited under high-temperature equilibrium conditions. However, processes such as dehydration of hydrous minerals during metamorphism, exsolution of magmatic-hydrothermal fluids, and fluid-rock interactions can lead to significant Ba isotope fractionation. Finally, this paper presents research progress and case studies on the use of Ba isotopes to investigate crustal-material recycling, granite evolution, and mineralization, highlighting the application potential of Ba isotope in tracing high-temperature geological processes.
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Key words:
- Ba isotope /
- non-traditional stable isotope /
- geochemical tracing /
- isotope fractionation /
- geochemistry
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图 1 全球MORB样品的δ138/134Ba与87Sr/86Sr（a）和143Nd/144Nd（b）相关图解
DMM端元的Sr-Nd同位素参考值来自Workman and Hart（2005）
Fig. 1. Correlation diagrams of global MORB samples δ138/134Ba with 87Sr/86Sr (a) and 143Nd/144Nd (b)
图 2 与俯冲带岩浆作用有关的全球不同储库的现有Ba同位素观测结果(未按比例绘制)
修改自Le Pichon et al.（2013）
Fig. 2. The existing Ba isotope observations of global different reservoirs related to subduction zone magma processes (not to scale)
图 3 在高温高压条件下，熔体与水相Ba2+（a）以及矿物与水相Ba2+（b）之间的Δ138/134Ba的平衡Ba同位素分馏因子（103lnβ）随温度变化的情况
修改自Wang et al.（2023）；红点数据来自Guo et al.（2020）
Fig. 3. The equilibrium Ba isotope fractionation factors (103lnβ) of 138Ba/134Ba between melt and aqueous Ba2+ (a) and minerals and aqueous Ba2+(b) as a function of temperature at high T-P
图 4 Mariana岛弧岩浆岩的Sr⁃Nd同位素与Ba/Th比值（a）和δ138/134Ba（b）的相关图解
符号颜色指示了岛弧岩浆岩的Ba/Th比值和δ138/134Ba.修改自Zhang et al.（2024），数据来自Zhang et al.（2024）
Fig. 4. Correlation diagrams of Sr⁃Nd isotopes, Ba/Th ratio (a), and δ138/134Ba (b) for the Mariana Island Arc magmatic rocks
图 5 俯冲带中板片物质运输的两种不同端元模型(未按比例绘制)
a.板片熔流体交代地幔楔；b.混杂岩底辟熔融.修改自Nielsen et al.（2020）
Fig. 5. Two different end⁃member models of material transport in subduction zones (not to scale)
图 6 全球不同地区的OIB的δ138/134Ba值与（a）87Sr/86Sr，（b）206Pb/204Pb和（c）Ba/Th比值的相关图解
数据来自Bai et al.（2022）、Shu et al.（2022）、Yu et al.（2022）
Fig. 6. The δ138/134Ba values of OIB from different global regions and their correlation with (a) 87Sr/86Sr, (b) 206Pb/204Pb, and (c) Ba/Th ratios
图 7 不同地区酸性岩的δ138/134Ba与（a）SiO2、（b）Ba、（c）Rb/Sr及（d）Eu/Eu*的相关图解
主微量数据来自Zhao et al.（2016）、Li et al.（2017）
Fig. 7. Correlation diagrams of δ138/134Ba of acidic rocks from different regions with (a) SiO2, (b) Ba, (c) Rb/Sr, and (d) Eu/Eu*
图 8 酸性岩δ138/134Ba与SiO2、Ba含量的相关图解
数据来源：Deng et al.（2021，
2022 ，2024）；Huang et al.（2021）；Li et al.（2024a）；Nan et al.（2018）；Jiang et al.（2022）.颜色代表样品的Ba含量Fig. 8. Correlation diagram of δ138/134Ba in acid rocks with SiO2 and Ba content
表 1 常见含Ba矿物相之间在不同温度下的分馏系数α
Table 1. Fractionation coefficients α of common Ba-containing minerals at different temperatures
温度（K） 300 500 700 1 000 103lnα重晶石‒毒重石 ‒0.19a ‒0.19b ‒0.07a ‒0.07b ‒0.04a ‒0.04b ‒0.02a ‒0.02b 103lnα白云母‒毒重石 ‒0.09a ‒0.19b ‒0.03a ‒0.07b ‒0.02a ‒0.03b ‒0.01a ‒0.02b 103lnα微斜长石‒毒重石 ‒0.13a ‒0.16b ‒0.05a ‒0.06b ‒0.02a ‒0.03b ‒0.01a ‒0.01b 注：a代表数据来自 Wang et al. (2023) ，b代表数据来自Xiao et al. (2023) .
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