渤海东部和黄海北部表层沉积物稀土元素的分布特征与物源判别

蓝先洪; 李日辉; 密蓓蓓; 张志珣; 郭兴伟; 黄龙

doi:10.3799/dqkx.2016.038

渤海东部和黄海北部表层沉积物稀土元素的分布特征与物源判别

doi: 10.3799/dqkx.2016.038

蓝先洪^1,2,,
李日辉^1,2,
密蓓蓓^1,2,
张志珣^1,2,
郭兴伟^1,2,
黄龙^1,2

1.
国土资源部海洋油气资源与环境地质重点实验室，山东青岛 266071
2.
青岛海洋地质研究所，山东青岛 266071

基金项目:

国土资源部海洋区域地质调查项目 GZH201400206

国土资源部海洋区域地质调查项目 GZH200800501

国家自然科学基金项目 41206053

国土资源部海洋区域地质调查项目 GZH201400205

国家自然科学重点基金项目 41330964

详细信息

作者简介:
蓝先洪(1958-)，男，研究员，主要从事海洋沉积和沉积地球化学研究. E-mail: lanxh@qingdaonews.com

中图分类号: P595;P736.4
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出版历程
- 收稿日期: 2015-07-11
- 刊出日期: 2016-03-15

Distribution Characteristics of Rare Earth Elements in Surface Sediment and Their Provenance Discrimination in the Eastern Bohai and Northern Yellow Seas

Lan Xianhong^{1,2
,},
Li Rihui^1,2,
Mi Beibei^1,2,
Zhang Zhixun^1,2,
Guo Xingwei^1,2,
Huang Long^1,2

1.
Key Laboratory of Marine Hydrocarbon Resource and Environmental Geology, Ministry of Land and Resources, Qingdao 266071, China
2.
Qingdao Institute of Marine Geology, Qingdao 266071, China

摘要

摘要: 为了探讨渤海东部和黄海北部稀土元素分布特征及其影响因素，对渤海东部和黄海北部138个表层沉积物样品进行电感耦合等离子体质谱法分析.结果表明：渤海东部和黄海北部沉积物的配分模式与中国黄土的接近，与周边的鸭绿江、黄河等河流输入物质也有相似性，表明研究区沉积物主要来自于周边大陆.沉积物物源判别结果显示：山东半岛近岸及其西南部沉积物主要来源于黄河，该区域沉积物分布受山东半岛沿岸流及近岸潮流影响；研究区东部沉积物稀土元素组成特征与鸭绿江沉积物组成相近，表明研究区东部沉积物可能由鸭绿江供应；研究区西北部沉积物主要来源于黄河及辽宁沿岸物质输入，局部有滦河、六股河物质存在；研究区东南部物质主要来源于黄河.对沉积物稀土元素百分含量及参数特征值进行了Q型聚类分析，将研究海域沉积物划分为4个不同的区域，分别为北黄海东部区域(Ⅰ)、山东半岛近岸周边区域(Ⅱ)、渤海东部中部区域(Ⅲ)及研究区的西北部与东南部分布区(Ⅳ).
- 稀土元素 /
- 分布特征 /
- 表层沉积物 /
- 渤海东部 /
- 黄海北部 /
- 地球化学
Abstract: Rare earth elements (REE) were analyzed by ICP-MS analysis in 138 surface sediments samples collected from in the eastern Bohai and northern Yellow Seas, China. The results indicated that the REE UCC normalization distribution pattern in surface sediments in the eastern Bohai and northern Yellow Seas was similar to that in Chinese loess, and also those of coastal rivers including the Yalu River, the Yellow River and other rivers, indicating that the sediments in study area were mainly derived from the mainland substance. Provenance discrimination results showed that the sediments in the Shandong Peninsula and southwestern shore were mainly derived from the Yellow River, the area affected by the coastal current of the Shandong Peninsula and near shore tidal current; REE composition characteristics of sediment in the eastern part in the study area were similar to the Yalu River sediments, indicating that the sediments of the eastern study area may be supplied by the Yalu River. Sediments of the western part of the study area were mainly derived from the Yellow River and Liaoning coast material input, the local presence of the Luanhe River, Liuguhe River substance. The material of southeast in the study area mainly derived from the Yellow River. The REE contents and parameters of characteristic value were analyzed by the Q cluster analysis, the study area can be divided into four different regions, Namely region in the eastern part of the North Yellow Sea (Ⅰ), the Shandong Peninsula inshore surrounding area (Ⅱ), middle area in the eastern Bohai Sea (Ⅲ) and distributions in the northwest and southeast of the study area (Ⅳ).
- rare earth elements /
- distribution /
- surface sediments /
- eastern Bohai Sea /
- northern Yellow Sea /
- geochemistry

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图 1 渤海东部和黄海北部表层沉积物稀土元素取样站位分布

Fig. 1. Location of the sampling stations of the rare earth elements (REE) in the surface sediment from the eastern Bohai and northern Yellow Seas

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图 2 渤海东部和黄海北部表层沉积物∑REE分布(μg/g)

Fig. 2. Distribution of ∑REE in surface sediments from the eastern Bohai and northern Yellow Seas

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图 3 渤海东部和黄海北部海域沉积物∑LREE/∑HREE分布

Fig. 3. Distribution of ∑LREE/∑HREE in surface sediments from the eastern Bohai and northern Yellow Seas

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图 4 表层沉积物中δEu值分布

Fig. 4. Distribution of δEu in surface sediments

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图 5 黄河、长江、锦江、汉江和表层沉积物上地壳标准化稀土元素配分模式

长江、黄河数据引自Yang et al.(2002)；鸭绿江、汉江、汉江数据引自Yang et al.(2003)

Fig. 5. UCC-normalzed REE distribution patterns of samples in Yellow River, Yangtze River, Keum River, Han River and surface sediments

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图 6 表层沉积物CIA值与∑REE相关关系(a)和∑REE与平均粒径相关关系(b)

Fig. 6. Correlation between ∑REE and CIA in surface sediments (a) and correlation between ∑REE and average grain diameter (b)

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图 7 渤海东部和黄海北部表层沉积物(La/Yb)_UCC值和(Gd/Yb)_UCC值元素物源判别

Fig. 7. Discrimination plots of (La/Yb)_UCC vs (Gd/Yb)_UCC in surface sediments in the eastern Bohai and northern Yellow Seas

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图 8 沉积物分区与物质运移方向

Fig. 8. The subarea and the moving route of the sediment

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图 9 渤海东部和黄海北部表层沉积物δEu_N值与(La/Yb)_N值物源判别

Fig. 9. Discrimination plots of δEu_N vs (La/Yb)_N in surface sediments from the eastern Bohai and northern Yellow Seas

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表 1 渤海东部和黄海北部表层沉积物稀土元素含量(μg/g)

Table 1. Concentrations of REE in surface sediments from the eastern Bohai and northern Yellow Seas (μg/g)

元素	La	Ce	Pr	Nd	Sm	Eu	Gd	Tb	Dy	Ho	Er	Tm	Yb	Lu	Y	∑REE
最大值	48.9	102.0	11.50	41.9	7.14	1.37	6.07	0.92	5.19	1.05	2.97	0.47	2.99	0.47	27.5	247.6
最小值	19.5	38.4	4.65	17.2	3.13	0.70	2.61	0.41	2.33	0.45	1.16	0.16	1.01	0.15	11.6	115.0
平均值	33.5	66.6	7.86	29.2	5.25	1.08	4.56	0.70	3.92	0.80	2.21	0.34	2.20	0.35	21.1	179.7

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表 2 渤海东部和黄海北部表层沉积物各组份的相关关系

Table 2. Correlation coefficients between the elements of surface sediment in the eastern Bohai and northern Yellow Seas

	∑REE	∑LREE/∑HREE	砂	粉砂	黏土	Al₂O₃	CaO	TiO₂	MgO	TFe₂O₃	Zr	Th	Cr	Co	Rb	Sr
∑REE	1.00
∑LREE/∑HREE	0.73^**	1.00
砂	-0.56^**	-0.34^**	1.00
粉砂	0.53^**	0.29^**	-0.98^**	1.00
黏土	0.53^**	0.41^**	-0.87^**	0.76^**	1.00
Al₂O₃	0.64^**	0.56^**	-0.76^**	0.70^**	0.79^**	1.00
CaO	-0.21^*	-0.21^*	-0.10	0.11	0.06	-0.32^**	1.00
TiO₂	0.60^**	0.33^**	-0.92^**	0.93^**	0.73^**	0.77^**	-0.06	1.00
MgO	0.57^**	0.43^**	-0.88^**	0.84^**	0.84^**	0.89^**	0.06	0.84^**	1.00
TFe₂O₃	0.65^**	0.48^**	-0.83^**	0.76^**	0.85^**	0.84^**	0.05	0.77^**	0.95^**	1.00
Zr	-0.09	-0.13	0.30^**	-0.24^**	-0.37^**	-0.43^**	-0.21^*	-0.14	-0.51^**	-0.52^**	1.00
Th	0.91^**	0.73^**	-0.66^**	0.62^**	0.64^**	0.81^**	-0.26^**	0.71^**	0.74^**	0.76 ^**	-0.18^*	1.00
Cr	0.61^**	0.44^**	-0.91^**	0.87^**	0.84^**	0.89^**	-0.05	0.90^**	0.95^**	0.92^**	-0.38^**	0.79^**	1.00
Co	0.66^**	0.50^**	-0.84^**	0.77^**	0.86^**	0.89^**	-0.04	0.79^**	0.94^**	0.97^**	-0.50^**	0.78^**	0.93^**	1.00
Rb	0.66^**	0.59^**	-0.60^**	0.52^**	0.71^**	0.92^**	-0.35^**	0.59^**	0.79^**	0.82^**	-0.52^**	0.80^**	0.78^**	0.87^**	1.00
Sr	-0.32^**	-0.29^**	0.34^**	-0.34^**	-0.28^**	-0.57^**	0.65^**	-0.42^**	-0.41^**	-0.36^**	0.08	-0.47^**	-0.45^**	-0.41^**	-0.54^**	1.00
注：使用PASS统计软件分析；^*代表双侧检验在0.01水平上显著相关；^代表在0.05水平上显著相关

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表 3 Q-型分区稀土元素的特征参数(μg/g)

Table 3. The characteristic parameters of REE (μg/g)

分区	样品数	∑REE	δEu_N	∑LREE	∑HREE	∑LREE/∑HREE	(La/Lu)_UCC	(La/Yb)_UCC
Ⅰ区	19	183.5	0.66	148.6	34.9	4.26	1.32	1.41
Ⅱ区	65	180.9	0.66	144.7	36.2	4.00	0.99	1.07
Ⅲ区	28	154.8	0.69	118.2	36.6	3.23	0.98	1.07
Ⅳ区	26	200.4	0.67	164.0	36.4	4.51	1.02	1.11

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