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    二连盆地白音查干凹陷下白垩统湖相沸石成因:来自矿物学、微量元素特征的证据

    杨喆 钟大康 张硕 郭强 路昭

    杨喆, 钟大康, 张硕, 郭强, 路昭, 2018. 二连盆地白音查干凹陷下白垩统湖相沸石成因:来自矿物学、微量元素特征的证据. 地球科学, 43(10): 3733-3748. doi: 10.3799/dqkx.2018.252
    引用本文: 杨喆, 钟大康, 张硕, 郭强, 路昭, 2018. 二连盆地白音查干凹陷下白垩统湖相沸石成因:来自矿物学、微量元素特征的证据. 地球科学, 43(10): 3733-3748. doi: 10.3799/dqkx.2018.252
    Yang Zhe, Zhong Dakang, Zhang Shuo, Guo Qiang, Lu Zhao, 2018. Mineralogical and Trace-Element Constrains on the Genesis of Zeolite in Lower Cretaceous Lacustrine Rocks from Baiyinchagan Sag, Erlian Basin, China. Earth Science, 43(10): 3733-3748. doi: 10.3799/dqkx.2018.252
    Citation: Yang Zhe, Zhong Dakang, Zhang Shuo, Guo Qiang, Lu Zhao, 2018. Mineralogical and Trace-Element Constrains on the Genesis of Zeolite in Lower Cretaceous Lacustrine Rocks from Baiyinchagan Sag, Erlian Basin, China. Earth Science, 43(10): 3733-3748. doi: 10.3799/dqkx.2018.252

    二连盆地白音查干凹陷下白垩统湖相沸石成因:来自矿物学、微量元素特征的证据

    doi: 10.3799/dqkx.2018.252
    基金项目: 

    国家自然科学基金项目 41302108

    国家自然科学基金项目 41472094

    国家自然科学基金项目 41502099

    详细信息
      作者简介:

      杨喆(1989-), 女, 博士研究生, 主要从事储层地质学及沉积学研究

      通讯作者:

      钟大康

    • 中图分类号: P581

    Mineralogical and Trace-Element Constrains on the Genesis of Zeolite in Lower Cretaceous Lacustrine Rocks from Baiyinchagan Sag, Erlian Basin, China

    • 摘要: 二连盆地白音查干凹陷下白垩统暗色沉积物中发育由白色颗粒构成的同沉积纹层、条带,其矿物组合中包含大量成因不明的钠沸石和方沸石.在薄片鉴定和电子探针(EMPA)分析的基础上,通过场发射扫描电镜(FE-SEM)和电感耦合等离子体质谱仪(ICP-MS)法对两种沸石矿物的形貌、微结构、共生矿物组合和微量元素成分进行分析.实验结果表明,钠沸石和方沸石自形程度较高,其中钠沸石为半自形-自形的棱柱状,长轴方向长度最大可达600 μm,集合体为纤维状或块状;方沸石呈自形的四角三八面体,粒径变化较大,介于10~300 μm.钠沸石和方沸石既能独立生长,也能互相交代,与重晶石、含铁白云石、菱镁矿和菱铁矿以及立方体黄铁矿等矿物紧密共生.与地壳及同区和同层位湖相泥岩微量元素配分曲线比较,含沸石岩石的全岩微量元素富集Pb、Sb、Tl、W、Mo、Bi,亏损V、Cr、Co、Ni,暗示了中高温含深源物质的碱性热液流体的加入.在综合分析沸石矿物形态结构、共生矿物组合及微量元素特征的基础上,认为在异常热流驱动下,中高温热液流体沿着断裂等运移通道喷出或溢流至湖底沉积物表面,与冷的湖水混合直接结晶沉淀形成方沸石、钠沸石和其他共生矿物,属于热水沉积成因.

       

    • 图  1  白音查干凹陷构造简图及样品位置(a)和下白垩统地层柱状(b)

      图b改自郭强等(2012)

      Fig.  1.  Simplified structure map of the Baiyinchagan Sag showing samples location (a) and stratigraphic and lithological succession of the Lower Cretaceous in Baiyinchagan Sag (b)

      图  2  白音查干凹陷统腾格尔组含沸石地层展布

      据郭强等(2014)

      Fig.  2.  Isopleth maps about distribution of zeolites-bearing rocks in Tenger Formation of Baiyinchagan Sag

      图  3  沸石及共生矿物岩心照片

      a.网脉状构造,作为热液活动通道,标记处白色颗粒由钠沸石+方沸石+含铁白云石组成,锡3-69井,1 831.45 m;b.网脉状构造横切面,同图a,锡3-69井,1 831.45 m;c.白色颗粒定向分布在暗色沉积物中,且长轴方向随纹层变化,标记处白色颗粒由方沸石+含铁白云石组成,锡3-69井,1 832.15 m;d.白色纹层条带发生塑形变形,标记处白色纹层由钠沸石+含铁白云石组成,锡31井,2 080.04 m;e.白色条带发生撕裂形成不规则颗粒,标记处白色颗粒由钠沸石+菱镁矿+含铁白云石组成,锡3-69井,1 790.5 m;f.白色颗粒呈层状分布,发育微裂缝,微裂缝由方沸石+含铁白云石充填,锡31井,2 035.96 m

      Fig.  3.  Photographs of natrolite and analcime associated with other minerals from cores

      图  4  沸石及共生矿物显微照片

      a.“似斑晶”钠沸石集合体,其边缘白云石化,菱镁矿分布沸石晶粒间,正交偏光,锡26井,1 816.33 m; b.钠沸石交代方沸石共生,两者界线模糊,沸石集合体边缘被含铁白云石交代,正交偏光,锡3-69井,1 772.8 m;c.菱镁矿/菱铁矿呈放射状生长在钠沸石中,正交偏光,锡3-69井,1 772.2 m;d.钠沸石纹层夹在泥岩中,单偏光,锡3-69井,1 776.8 m;e.重晶石充填钠沸石搭建的三角区内,单偏光,锡26井,1 824.3 m;f.板条状钠沸石与菱镁矿、重晶石共生,单偏光,锡26井, 1 818.13 m;g.方沸石颗粒分布于白云质泥岩中,单偏光,锡36井,2 436.94 m;h.“似斑晶”状方沸石集合体,菱镁矿发育在方沸石集合体中,正交偏光,查39井,2 337.32 m;i.方沸石和含铁白云石充填微裂缝,正交偏光,锡26井,1 818.13 m.A.方沸石;B.重晶石;D.含铁白云石;M.菱镁矿;N.钠沸石;Talc.滑石;P.黄铁矿

      Fig.  4.  Microphotographs of natrolite and analcime associated with other minerals

      图  5  沸石矿物及共生矿物扫描电镜二次电子图像

      a.块状钠沸石集合体微形貌特征,锡3-69井,1 785.5 m;b.钠沸石晶粒集合体微形貌特征,锡3-69井,1 792.56 m;c.钠沸石及共生含铁白云石微形貌特征,锡3-69井,1 782.2 m;d.钠沸石中充填立方体黄铁矿微形貌特征,锡32井,1 823.6 m;e.方沸石与钠沸石交代共生,周围分布含铁白云石,锡3-69井,1 770.7 m;f.方沸石与菱镁矿共生,锡3-69井,1 782.2 m;g.钠沸石与重晶石共生微形貌特征,锡3-69井,1 796.8 m;h.放射状菱镁矿和菱铁矿微形貌特征,锡3-69井,1 792.56 m;i.立方体黄铁矿微形貌特征,锡3-69井,1 776.8 m.A.方沸石;B.重晶石;D.含铁白云石;M.菱镁矿;N.钠沸石;Talc.滑石;P.黄铁矿

      Fig.  5.  Scanning electron microscope photos of zeolites associated with other minerals

      图  6  沸石与重晶石含量(a)、黄铁矿含量(b)、菱镁矿含量(c)线性关系图

      Fig.  6.  Content linear graghs between zeolite and barite(a), zeolite and pyrite (b), and zeolite and magnesite (c)

      图  7  含沸石岩石地壳标准化微量元素蛛网图

      标准化值据黎彤(1992)

      Fig.  7.  Continental crust-normalized trace element spider diagram of zeolite-bearing rocks

      表  1  电子探针(EMPA)沸石的主量元素分析结果(%)

      Table  1.   Analysis of main elements of zeolites by EMPA (%)

      矿物类型 样品 样品深度(m) 氧化物含量(%) Na/Al Si/Al
      Na2O Al2O3 SiO2 K2O 总量
      锡26 1 820.6 13.76 29.22 57.02 / 100 0.77 1.66
      锡26 1 818.1 15.71 28.11 55.86 0.32 100 0.92 1.69
      钠沸石 锡3-69 1 772.2 16.8 32.47 50.73 / 100 0.61 1.50
      锡3-69 1 776.8 17.82 32.66 49.52 / 100 0.64 1.46
      查39 2 337.3 15.71 33.16 51.13 / 100 0.56 1.48
      方沸石 锡31 2 076.8 14.07 27.03 58.88 / 99.98 0.61 2.09
      锡3-69 1 772.2 15.72 27.76 56.51 / 100 0.67 1.96
      锡3-69 1 772.2 15.42 27.38 57.20 / 100 0.66 2.01
      锡3-69 1 772.2 15.72 27.31 56.95 / 99.98 0.68 2.00
      下载: 导出CSV

      表  2  含沸石岩石微量元素含量(10-6)

      Table  2.   Trace elements content (10-6) of zeolite-bearing rocks

      岩石类型 样品号 元素含量(10-6)
      Li Be Sc V Cr Co Ni Cu Zn Pb Sb Cd Ga Tl Rb Sr Cs Ba W Mo Bi Y Th U
      沸石质白云岩 X3-69-1 209.0 3.2 23.8 130.0 83.4 16.4 42.4 51.0 111.0 22.0 1.0 0.3 30.2 1.4 99.4 869.0 32.8 572.0 3.6 3.9 0.6 33.3 15.4 6.6
      X3-69-2 163.0 2.5 17.5 147.0 87.2 18.9 42.0 45.4 111.0 35.5 1.0 0.3 16.4 0.7 110.0 444.0 29.9 470.0 3.4 15.8 1.3 32.4 12.6 4.7
      X3-69-3 383.0 3.5 16.7 128.0 89.5 25.4 54.7 59.5 120.0 31.8 1.2 0.3 17.3 0.9 135.0 342.0 28.7 408.0 3.7 8.7 0.9 25.3 5.9 2.3
      X3-69-4 355.0 1.9 15.7 119.0 80.3 16.5 33.7 52.1 117.0 20.8 0.6 0.4 17.2 0.8 89.7 761.0 43.5 217.0 3.7 73.6 0.5 34.8 15.9 7.5
      C39-1 97.0 1.3 14.0 92.1 47.8 17.6 42.3 46.3 103.0 34.2 1.5 0.3 25.6 0.3 48.0 2305.0 31.8 3065.0 2.5 41.7 0.9 34.2 34.8 19.3
      X31-1 546.0 4.8 17.7 154.0 89.2 16.1 31.7 45.7 122.0 24.0 0.7 0.3 20.5 1.0 207.0 407.0 34.6 469.0 4.7 16.7 0.5 18.3 6.6 3.0
      X3-69-5 155.0 1.9 13.8 103.0 74.0 15.7 38.6 46.4 103.0 25.9 0.7 0.3 11.9 0.5 63.6 532.0 47.4 482.0 1.9 15.4 0.8 59.5 10.2 7.1
      X3-69-6 9.2 0.8 11.2 64.0 57.0 15.3 39.3 54.6 81.9 28.4 1.9 0.4 10.9 5.2 69.3 874.0 31.6 433.0 1.8 18.2 0.6 53.5 24.2 16.1
      X3-69-7 516.0 4.2 18.1 141.0 87.5 19.4 39.1 50.3 116.0 25.4 1.1 0.3 21.1 0.8 156.0 500.0 30.0 521.0 3.6 13.4 0.6 25.0 15.9 3.2
      X31-2 516.0 6.2 13.0 124.0 67.8 23.7 43.8 61.6 104.0 48.1 1.1 0.4 21.0 3.3 187.0 355.0 41.0 406.0 7.0 11.0 1.2 17.1 10.5 6.4
      X3-69-8 174.0 2.1 14.4 112.0 71.9 16.1 39.8 48.1 105.0 24.3 0.6 0.3 15.3 0.4 80.7 432.0 39.3 308.0 2.2 10.6 0.8 35.5 11.5 4.6
      X31-3 72.1 1.9 14.3 140.0 57.7 14.8 31.6 46.2 86.9 24.2 0.7 0.4 17.7 0.3 100.0 757.0 24.6 290.0 3.6 44.1 0.5 45.5 12.7 4.7
      X3-69-9 25.0 1.4 17.6 111.0 74.5 18.8 50.4 48.5 96.9 29.8 1.1 0.3 18.6 0.5 41.6 497.0 17.3 225.0 3.5 44.9 0.8 25.9 8.4 6.8
      X3-69-10 259.0 3.8 15.0 115.0 81.2 18.3 47.0 54.1 124.0 27.7 1.1 0.4 19.7 0.6 151.0 390.0 22.6 409.0 4.7 6.0 0.8 17.9 8.1 2.1
      含沸石白云岩 X32-1 30.6 1.5 13.4 95.7 58.9 16.7 40.8 47.7 80.2 21.9 0.5 0.3 11.1 0.4 83.6 928.0 6.5 326.0 5.0 6.4 0.5 31.8 13.4 8.4
      X31-4 67.9 0.4 8.5 57.3 25.7 5.7 20.8 40.4 34.2 8.1 0.5 0.1 11.6 0.1 21.7 5 374.0 16.0 2 204.0 1.6 2.5 0.3 12.3 6.7 4.0
      含沸石白云质泥岩 X26-1 15.0 0.7 15.6 92.1 69.0 23.3 28.8 46.5 101.0 26.5 1.4 0.3 22.7 0.2 44.5 446.0 15.7 139.0 3.8 19.8 0.6 18.7 14.7 4.9
      X26-2 19.4 0.7 12.1 79.1 71.8 14.4 37.7 44.5 99.3 23.8 1.0 0.2 33.0 0.2 12.7 389.0 11.6 656.0 2.8 9.9 0.5 15.7 8.1 1.6
      X3-69-11 421.0 2.7 17.2 120.0 75.0 21.9 51.7 59.6 125.0 32.6 1.4 0.3 25.1 0.6 122.0 305.0 12.5 367.0 4.5 11.1 0.7 19.0 12.2 3.5
      X36-1 460.0 2.3 13.2 106.0 73.2 16.5 37.8 48.3 101.0 26.2 0.6 0.3 24.5 0.3 188.0 438.0 27.1 775.0 3.6 3.8 0.7 27.0 19.8 8.8
      X31-5 127.0 1.9 13.4 118.0 83.7 20.4 42.9 54.5 124.0 27.1 1.1 0.3 30.5 0.4 75.7 379.0 18.8 330.0 4.9 12.9 0.9 24.9 30.1 15.2
      X3-69-12 445.0 2.9 14.4 117.0 92.2 20.0 46.6 54.8 101.0 37.4 1.1 0.3 21.6 0.9 142.0 514.0 36.5 478.0 3.8 41.6 0.9 30.8 10.6 5.8
      C39-2 243.0 2.6 13.7 116.0 86.9 17.3 41.0 56.4 103.0 23.5 0.8 0.3 21.3 0.5 173.0 291.0 35.1 261.0 4.0 11.3 0.8 11.9 4.9 2.4
      X3-69-13 204.0 2.9 18.3 128.0 89.9 14.7 32.5 41.6 161.0 20.8 1.1 0.3 31.6 1.0 102.0 589.0 36.5 2 399.0 3.8 2.9 0.4 25.9 19.1 2.8
      含泥沸石质白云岩 X31-6 10.0 1.2 12.0 90.0 61.6 16.3 41.6 46.7 71.8 23.6 2.7 0.4 12.1 1.1 88.0 1 344.0 18.0 351.0 3.4 20.2 0.5 49.2 13.2 4.1
      X3-69-14 136.0 2.4 15.5 98.8 71.3 20.6 67.6 46.2 98.4 48.8 1.7 0.3 20.4 0.6 53.8 575.0 17.4 509.0 3.4 58.4 0.7 33.5 14.9 34.8
      X3-69-15 370.0 4.1 17.5 134.0 83.7 22.5 49.3 54.7 112.0 26.8 1.0 0.3 20.2 0.6 195.0 342.0 31.8 493.0 5.4 7.8 0.8 16.9 4.7 2.3
      沸石质泥岩 X26-3 132.0 0.9 8.5 73.9 58.9 15.8 35.9 38.3 101.0 19.4 0.8 0.2 30.4 0.3 27.5 196.0 30.0 1 596.0 2.4 4.6 0.6 12.5 7.1 1.7
      平均值 220.0 2.4 14.9 110.9 73.2 17.8 41.1 49.6 104.1 27.5 1.1 0.3 20.7 0.9 102.4 770.5 27.5 684.3 3.7 19.2 0.7 28.2 13.3 7.0
      地壳丰度 23.0 1.7 16.0 143.0 127.0 24.7 81.3 56.0 76.3 14.0 0.5 0.2 16.7 0.7 108.0 382.0 1.2 463.0 1.1 1.4 0.2 27.7 7.6 2.1
      富集系数 9.6 1.4 0.9 0.8 0.6 0.7 0.5 0.9 1.4 2.0 2.1 1.7 1.2 1.2 0.9 2.0 22.3 1.5 3.2 13.4 3.7 1.0 1.7 3.4
      泥岩 331.0 7.5 17.4 140.0 91.7 23.4 40.7 55.2 136.0 21.1 0.8 0.3 25.3 0.6 249.0 567.0 83.1 612.0 2.5 3.3 0.5 31.1 17.9 5.2
      注:地壳丰度参考黎彤(1992);富集系数=含沸石岩石微量元素含量/地壳丰度.
      下载: 导出CSV
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    • 收稿日期:  2018-02-15
    • 刊出日期:  2018-10-20

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